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A new method of computing multipolar exchange interaction in spin-orbit coupled systems is developed using multipolar tensor expansion of the density matrix in LDA+U electronic structure calculation. Within mean-field approximation,…

Strongly Correlated Electrons · Physics 2014-03-06 Shu-Ting Pi , Ravindra Nanguneri , Sergey Savrasov

Focusing on the efficient probe and manipulation of single-particle spin states, we investigate the coupled spin and orbital dynamics of a spin 1/2 particle in a harmonic potential subject to ultrastrong spin-orbit interaction and external…

Mesoscale and Nanoscale Physics · Physics 2014-01-21 C. Echeverria-Arrondo , E. Ya. Sherman

We report high steady-state nuclear polarization of 1 torr $^3$He gas nuclei via metastability-exchange optical pumping at magnetic fields above 2 T. The introduction of highly polarized $^3$He gas into Brookhaven's Electron Beam Ion Source…

Instrumentation and Detectors · Physics 2019-04-15 J. D. Maxwell , J. Alessi , G. Atoian , E. Beebe , C. S. Epstein , R. G. Milner , M. Musgrave , A. Pikin , J. Ritter , A. Zelenski

Low thermal polarization of nuclear spins is a primary sensitivity limitation for nuclear magnetic resonance. Here we demonstrate optically pumped (microwave-free) nuclear spin polarization of $^{13}\mathrm{C}$ and $^{15}\mathrm{N}$ in…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Ben L. Green , Ben G. Breeze , Gregory J. Rees , John V. Hanna , Jyh-Pin Chou , Viktor Ivády , Adam Gali , Mark E. Newton

Irradiating a semiconductor with circularly polarized light creates spin-polarized charge carriers. If the material contains atoms with non-zero nuclear spin, they interact with the electron spins via the hyperfine coupling. Here, we…

Mesoscale and Nanoscale Physics · Physics 2016-09-09 Raphael W. Mocek , Danil O. Tolmachev , Giovanni Cascio , Dieter Suter

The Knight shift of Ga-71 nuclei is measured in two different electron-doped multiple quantum well samples using optically pumped NMR. These data are the first direct measurements of the electron spin polarization,…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 P. Khandelwal , N. N. Kuzma , S. E. Barrett , L. N. Pfeiffer , K. W. West

Dynamic nuclear polarization transfers spin polarization from electrons to nuclei. We have achieved this by a new method, simultaneously exciting transitions of electronic and nuclear spins. The efficiency of this technique improves with…

Quantum Physics · Physics 2008-09-11 G. W. Morley , K. Porfyrakis , A. Ardavan , J. van Tol

We consider the degree of conservation of nuclear spin polarization in the process of optical pumping under typical spin-exchange optical pumping conditions. Previous analyses have assumed that negligible nuclear spin precession occurs in…

Atomic Physics · Physics 2013-05-29 B. Lancor , T. G. Walker

We describe a method to hyperpolarize 3He nuclear spins at high magnetic fields (4.7 Tesla) solely by a magnetized plasma. The conditions for such a magnetized plasma are fulfilled when the mean free path of the free electrons is much…

Atomic Physics · Physics 2018-12-12 A. Maul , P. Blümler , P. -J. Nacher , E. Otten , G. Tastevin , W. Heil

We demonstrate a method which can hyperpolarize both the electron and nuclear spins of 31P donors in Si at low field, where both would be essentially unpolarized in equilibrium. It is based on the selective ionization of donors in a…

Experiments using polarized $^{3}He$ atom beams to search for short range spin dependent forces are proposed. High intensity, high polarization, small beam size $^{3}He$ atom beams have been successfully produced and used in surface science…

Instrumentation and Detectors · Physics 2015-06-22 H. Yan

A highly asymmetric dynamic nuclear spin pumping is observed in a single self assembled InGaAs quantum dot subject to resonant optical pumping of the neutral exciton transition leading to a large maximum polarization of 54%. This dynamic…

Mesoscale and Nanoscale Physics · Physics 2010-09-30 F. Klotz , V. Jovanov , J. Kierig , E. C. Clark , M. Bichler , G. Abstreiter , M. S. Brandt , J. J. Finley , H. Schwager , G. Giedke

We report the hysteresis of optically-pumped nuclear spin polarization and the degree of circular polarization of photoluminescence on the excitation power and electron spin polarization in single InAlAs quantum dots. By increasing (or…

Materials Science · Physics 2009-11-13 R Kaji , S Adachi , H Sasakura , S Muto

Elucidating spin correlations in the parent compounds of high-temperature superconductors is crucial for understanding superconductivity. We used neutron scattering to study spin correlations in Li$_{1-x}$Fe$_x$ODFeSe, an insulating…

Superconductivity · Physics 2025-01-06 Hongliang Wo , Bingying Pan , Die Hu , Yu Feng , A. D. Christianson , Jun Zhao

Coupled pairs of nuclear spins-1/2 support one singlet state and three triplet states. Transitions between the singlet state and one of the triplet states may be driven by an oscillating low-frequency magnetic field, in the presence of…

Quantum Physics · Physics 2021-10-27 Laurynas Dagys , Christian Bengs , Malcolm H. Levitt

Using measured spin-transfer rates from alkali atoms to He-3, combined with spin-relaxation rates of the alkali atoms due to He-3 and He-4, it should be possible to differentiate between isotropic and anisotropic spin-exchange. This would…

Atomic Physics · Physics 2013-05-29 T. G. Walker , I. A. Nelson , S. Kadlecek

Our search for non-magnetic spin-dependent interactions is based on the measurement of free precession of nuclear spin polarized 3He and 129Xe atoms in a homogeneous magnetic guiding field of about 400 nT. We report on our approach to…

High Energy Physics - Phenomenology · Physics 2017-08-23 F. Allmendinger , U. Schmidt , W. Heil , S. Karpuk , A. Scharth , Y. Sobolev , K. Tullney , S. Zimmer

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

We show that optical pumping of electron spins in individual InGaAs quantum dots leads to strong nuclear polarisation that we measure via the Overhauser shift (OHS) in magneto-photoluminescence experiments between 0 and 4T. We find a…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 P. -F. Braun , B. Urbaszek , T. Amand , X. Marie , O. Krebs , B. Eble , A. Lemaitre , P. Voisin

We investigate in micro-photoluminescence experiments the dynamical nuclear polarization in individual InGaAs quantum dots. Experiments carried out in an applied magnetic field of 2T show that the nuclear polarization achieved through the…

Other Condensed Matter · Physics 2009-11-13 B. Urbaszek , P. -F. Braun , X. Marie , O. Krebs , A. Lemaitre , P. Voisin , T. Amand