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The fragmentation of carbon monoxide dimers induced by collisions with low energy Ar$^{9+}$ ions is investigated using the COLTRIMS technique. The presence of a neighbor molecule in the dimer serves here as a diagnostic tool to probe the…

Atomic and Molecular Clusters · Physics 2021-11-03 A. Méry , X. Fléchard , S. Guillous , V. Kumar , M. Lalande , J. Rangama , W. Wolff , A. Cassimi

We present a combined theoretical and experimental study of primary and post-collision mechanisms involved when colliding low energy multiply charged ions with van der Waals dimers. The collision dynamics is investigated using a classical…

Atomic and Molecular Clusters · Physics 2018-07-11 W. Iskandar , X. Fléchard , J. Matsumoto , A. Leredde , S. Guillous , D. Hennecart , J. Rangama , A. Méry , B. Gervais , H. Shiromaru , A. Cassimi

We report on electron removal calculations for 2.81 keV/amu Li$^{3+}$ and O$^{3+}$ ion collisions with neon dimers. The target is described as two independent neon atoms fixed at the dimer's equilibrium bond length, whose electrons are…

Atomic and Molecular Clusters · Physics 2021-01-04 Dyuman Bhattacharya , Tom Kirchner

We present efficient and reliable molecular dynamics simulations of the photodissociation of dichloromethane followed by Coulomb explosion. These simulations are performed by calculating trajectories on accurate potential energy surfaces of…

Chemical Physics · Physics 2025-07-22 Yijue Ding

Dimers and trimers of carbonyl sulfide (OCS) molecules embedded in helium nanodroplets are aligned by a linearly polarized 160 ps long moderately intense laser pulse and Coulomb exploded with an intense 40 fs long probe pulse in order to…

Chemical Physics · Physics 2018-11-14 James D. Pickering , Benjamin Shepperson , Lars Christiansen , Henrik Stapelfeldt

Femtosecond laser pulses are utilized to drive multiple ionization in gas-phase formic acid dimers and ions are studied using time-of-flight mass spectrometry. The interaction of formic acid dimer with 200 fs linearly polarized laser pulses…

Atomic and Molecular Clusters · Physics 2022-10-12 Shaun F. Sutton , Dane M. Miller , Lenin M. Quiroz , Ananya Sen , Pilarisetty Tarakeshwar , Scott G. Sayres

We have deduced the structure of the \ce{bromobenzene}--\ce{I2} heterodimer and the \ce{(bromobenzene)2} homodimer inside helium droplets using a combination of laser-induced alignment, Coulomb explosion imaging, and three-dimensional ion…

The electron removal and excitation channels in argon dimer target and helium ion projectile collision systems that facilitate interatomic Coulombic decay (ICD) are investigated. We implement an independent-atom and independent-electron…

Atomic and Molecular Clusters · Physics 2026-03-25 Darij Starko , Tom Kirchner

Electron removal in collisions of alpha particles with neon dimers is studied using an independent-atom-independent-electron model based on the semiclassical approximation of heavy-particle collision physics. The dimer is assumed to be…

Atomic Physics · Physics 2022-07-06 Tom Kirchner

We present an efficient theoretical model to simulate observables in the time-resolved coincident three-ion Coulomb explosion experiment of diiodomethane. The model employs two degrees of freedom to describe the C-I bond breaking and the…

Chemical Physics · Physics 2026-02-26 Yijue Ding

We implement an independent-atom and independent-electron model to investigate the collision systems of He$^{2+}$ and He$^{+}$ ion projectiles impinging on a neon dimer target. The dimer is set to be stationary at its equilibrium bond…

Atomic and Molecular Clusters · Physics 2025-05-13 Darij Starko , Tom Kirchner

Using synchrotron radiation we simultaneously ionize and excite one helium atom of a helium dimer (He_2) in a shakeup process. The populated states of the dimer ion (i.e. He^[*+](n = 2; 3)-He) are found to deexcite via interatomic coulombic…

L-shell ionisation and subsequent Coulomb explosion of fully deuterated methyl iodide, CD$_3$I, irradiated with hard x-rays has been examined by a time-of-flight multi-ion coincidence technique. The core vacancies relax efficiently by Auger…

The weak infrared spectrum of CO2-Ar corresponding to the (0111) <-- (0110) hot band of CO2 is detected in the region of the carbon dioxide nu3 fundamental vibration (~2340 cm-1), using a tunable OPO laser source to probe a pulsed…

Atomic and Molecular Clusters · Physics 2020-10-28 T. A. Gartner , A. J. Barclay , A. R. W. McKellar , N. Moazzen-Ahmadi

We demonstrate the experimental realization of impulsive alignment of carbonyl sulfide (OCS) molecules at the Low Density Matter Beamline (LDM) at the free-electron laser FERMI. OCS molecules in a molecular beam were impulsively aligned…

We present a survey of CO(3-2) molecular line emission in the circumnuclear region of M31 with the James Clerk Maxwell Telescope (JCMT), aiming to explore the physical conditions of the molecular gas. Significant CO(3-2) lines are detected…

Astrophysics of Galaxies · Physics 2019-01-16 Zongnan Li , Zhiyuan Li , Ping Zhou , Yu Gao , Xue-Jian Jiang , Hui Dong

Coulomb explosion imaging (CEI) is a powerful experimental technique that maps a molecule's geometric structure onto the momenta of ionic molecular fragments produced by rapid multiple ionization. Here, we apply CEI induced by pulses from…

We solve the orientation recovery of a tumbling protein in the gas phase from single-event measurements of the spatial positions of its ions after an X-ray laser induced explosion. We simulate diffracted X-ray signal and ion dynamics under…

Chemical Physics · Physics 2026-03-26 Tomas André , Alfredo Bellisario , Nicusor Timneanu , Carl Caleman

The gas-phase structures of four difluoroiodobenzene and two dihydroxybromobenzene isomers were identified by correlating the emission angles of atomic fragment ions created following femtosecond laser-induced Coulomb explosion. The…

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