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In this work we consider a current carrying molecular junction with both electron-phonon and electron-electron interactions taken into account. After performing Lang-Firsov transformation and considering Markov approximations in accordance…

Mesoscale and Nanoscale Physics · Physics 2019-05-06 Amir Eskandari-asl

We present a simple model of electrical transport through a metal-molecule-metal nanojunction that includes charging effects as well as aspects of the electronic structure of the molecule. The interplay of a large charging energy and an…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Matthias H. Hettler , Herbert Schoeller , Wolfgang Wenzel

The linear conductance of a molecular conductor oscillating between two metallic leads is investigated numerically both for Hubbard interacting and noninteracting electrons. The molecule-leads tunneling barriers depend on the molecule…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 K. A. Al-Hassanieh , C. A. Büsser , G. B. Martins , E. Dagotto

We investigate the electron transport properties of a model magnetic molecule formed by two magnetic centers whose exchange coupling can be altered with a longitudinal electric field. In general we find a negative differential conductance…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Sujeet K. Shukla , Stefano Sanvito

Spin-charge states of correlated electrons in a one-dimensional quantum dot attached to interacting leads are studied in the non-linear transport regime. With non-symmetric tunnel barriers, regions of negative differential conductance…

Strongly Correlated Electrons · Physics 2011-10-10 F. Cavaliere , A. Braggio , J. T. Stockburger , M. Sassetti , B. Kramer

In this work, we have investigated conduction through an artificial molecule comprising two coupled quantum dots. The question addressed is the role of inter-dot coupling on electronic transport. We find that the current through the…

Mesoscale and Nanoscale Physics · Physics 2011-09-22 M. Imran , B. Tariq , M. Tahir , K. Sabeeh

The interaction of metal-molecule-metal junctions with light is considered within a simple generic model. We show, for the first time, that light induced current in unbiased junctions can take place when the bridging molecule is…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan

Using benzene sandwiched between two Au leads as a model system, we investigate from first principles the change in molecular conductance caused by different atomic structures around the metal-molecule contact. Our motivation is the…

Materials Science · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

The influence of an intramolecular proton transfer reaction on the conductance of a molecular junction is investigated employing a generic model, which includes the effects of the electric field of the gate and leads electrodes and the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Chriszandro Hofmeister , Pedro B. Coto , Michael Thoss

We investigate the effect on molecular transport due to the different structural aspects of metal-molecule interfaces. The example system chosen is the prototypical molecular device formed by sandwiching the phenyl dithiolate molecule (PDT)…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yongqiang Xue , Mark Ratner

We generalize our previous theory [Nano Lett. \textbf{18}, 5015-5023 (2018)] to investigate the influence of electron-phonon (e-p) coupling and vibrational relaxation on photoinduced \textit{anomalous Coulomb blockade}, which originates…

Chemical Physics · Physics 2021-06-21 Bo Fu , Liang-Yan Hsu

The conductance of a molecular junction is commonly determined by either charge-transfer-doping, where alignment of the Fermi energy to the molecular levels is achieved, or tunnelling through the tails of molecular resonances within the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 R. Gutierrez , G. Fagas , K. Richter , F. Grossmann , R. Schmidt

Screening effects in nanoscale junctions with strong electron-phonon coupling open new physical scenarios. We propose an accurate many-body approach to deal with the simultaneous occurrence of the Franck-Condon blockade and the…

Mesoscale and Nanoscale Physics · Physics 2013-07-30 E. Perfetto , G. Stefanucci

We consider transport through a vibrating molecular quantum dot contacted to macroscopic leads acting as charge reservoirs. In the equilibrium and nonequilibrium regime, we study the formation of a polaron-like transient state at the…

Strongly Correlated Electrons · Physics 2015-06-04 T. Koch , H. Fehske , J. Loos

Negative differential resistance - a decrease in current with increasing bias voltage - is a counter-intuitive effect that is observed in various molecular junctions. Here, we present a novel mechanism that may be responsible for such an…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Yonatan Dubi

The transport properties of a octane-dithiol (ODT) molecule coupled to Au(001) leads are analyzed using density functional theory and non-equilibrium Green functions. It is shown that a symmetric molecule can turn into a diode under…

Mesoscale and Nanoscale Physics · Physics 2010-02-09 Tomasz Kostyrko , Víctor M. García-Suárez , Colin J. Lambert , Bogdan R. Bułka

We analyze the effect of a gate on the conductance of molecules by separately evaluating the gate-induced polarization and the potential shift of the molecule relative to the leads. The calculations use ab initio density functional theory…

Materials Science · Physics 2007-05-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

We measure the low bias conductance of a series of substituted benzene diamine molecules while breaking a gold point contact in a solution of the molecules. Transport through these substituted benzenes is by means of nonresonant tunneling…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Latha Venkataraman , Young S. Park , Adam C. Whalley Colin Nuckolls , Mark S. Hybertsen , Michael L. Steigerwald

We study coherent phonon transport through organic, \pi-conjugated molecules. Using first principles calculations and Green's function methods, we find that the phonon transmission function in cross-conjugated molecules, like meta-connected…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Troels Markussen

The electronic transport through a triple quantum dot molecule attached in parallel to leads in presence of a magnetic flux is studied. Analytical expressions of the linear conductance and density of states for the molecule in equilibrium…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. L. Ladrón de Guevara , P. A. Orellana
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