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If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…

The two opposite concepts - multiphoton and effective photon - readily describing the photoelectric effect under strong irradiation in the case that the energy of the incident light is essentially smaller than the ionisation potential of…

Quantum Physics · Physics 2007-05-23 Volodymyr Krasnoholovets

How quanta of energy and charge are transported on both atomic spatial and ultrafast time scales is at the heart of modern technology. Recent progress in ultrafast spectroscopy has allowed us to directly study the dynamical response of an…

Other Condensed Matter · Physics 2015-04-28 R. Locher , L. Castiglioni , M. Lucchini , M. Greif , L. Gallmann , J. Osterwalder , M. Hengsberger , U. Keller

Time-resolved photoelectron spectroscopy provides access to the electronic structure and non-equilibrium electron dynamics in matter. At solid surfaces photoemission dynamics can be investigated on its natural time scale by measuring…

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We analyze the time delay between emission of photoelectrons from the outer valence $ns$ and $np$ sub-shells in noble gas atoms following absorption of an attosecond XUV pulse. By solving the time dependent Schr\"odinger equation and…

Atomic Physics · Physics 2010-12-07 A. S. Kheifets , I. A. Ivanov

We investigate theoretically the relative time delay of photoelectrons originating from the different subshells (2s and 2p) of neon. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science…

Atomic Physics · Physics 2017-02-15 J. Wätzel , A. S. Moskalenko , Y. Pavlyukh , J. Berakdar

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

Streaked photoemission metrology allows the observation of an apparent relative time delay between the detection of photoelectrons from different initial electronic states. This relative delay is obtained by recording the photoelectron…

Other Condensed Matter · Physics 2015-05-28 Chang-hua Zhang , Uwe Thumm

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

Over the past few decades, following the first demonstration of ultrafast electron microscopy, numerous research groups have focused on achieving attosecond temporal resolution in electron microscopy with the goal of imaging electron and…

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

Atomic Physics · Physics 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

We perform time- and angle-resolved photoelectron spectroscopy on p-type GaAs(110). We observe an optically excited population in the conduction band, from which the time scales of intraband relaxation and surface photovoltage decay are…

Materials Science · Physics 2013-12-06 Shuolong Yang , Jonathan A. Sobota , Patrick S. Kirchmann , Zhi-Xun Shen

A recent paper by Hui et al. (Ref. [1], Sci. Adv. 10, eadp5805 (2024)) claims the demonstration of 'Attosecond electron microscopy and diffraction' with laser-gated electron pulses. In this comment, we point out a series of physical and…

Materials Science · Physics 2024-11-25 P. Baum , C. Ropers

The dispersion measures of fast radio bursts have been identified as a powerful tool for testing the zero-mass hypothesis of the photon. The classical approach treats the massive photon-induced and plasma-induced time delays as two separate…

High Energy Astrophysical Phenomena · Physics 2024-09-10 Bao Wang , Jun-Jie Wei

We present a time-dependent density-functional method able to describe the photoelectron spectrum of atoms and molecules when excited by laser pulses. This computationally feasible scheme is based on a geometrical partitioning that…

Atomic Physics · Physics 2012-06-28 U. De Giovannini , D. Varsano , M. A. L. Marques , H. Appel , E. K. U. Gross , A. Rubio

We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…

Chemical Physics · Physics 2022-05-31 Y. Tamura , K. Yamazaki , K. Ueda , K. Hatada

We investigate attosecond time delays in the emission of photoelectrons using a hierarchy of models of the $CO_2$ molecule including the strong field approximation, Coulomb-scattering, short-range parts of the molecular potential, Hartree…

Atomic Physics · Physics 2021-03-30 Hakon Volkmann , Vinay P. Majety , Armin Scrinzi

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray
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