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Photoexcitation is an inherent part of any photochemical or spectroscopic experiment, yet its impact on the excited-state dynamics is often overlooked. However, it is the excited molecular state, built upon photoexcitation and shaped by the…

Chemical Physics · Physics 2026-03-09 Jiří Janoš , Federica Agostini , Petr Slavíček , Basile F. E. Curchod

Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…

Photo- and electro-disintegration techniques have been traditionally used for studying giant dipole resonances and through them nuclear structure. Over a long period, detailed theoretical models for the giant dipole resonances were proposed…

Nuclear Theory · Physics 2013-06-24 J. Swain , Y. N. Srivastava , A. Widom

Proposals to determine biomolecular structures from diffraction experiments using femtosecond X-ray free-electron laser (XFEL) pulses involve a conflict between the incident brightness required to achieve diffraction-limited atomic…

Optics · Physics 2015-05-19 Harry M. Quiney , Keith A. Nugent

Recent advancements in electron microscopy have introduced innovative techniques enabling the inelastic interaction of fast electrons with tightly confined and intense light fields. These techniques, commonly summarized under the term…

Mesoscale and Nanoscale Physics · Physics 2024-05-21 Niklas Müller , Soufiane el Kabil , Gerrit Vosse , Lina Hansen , Christopher Rathje , Sascha Schäfer

An important goal of modern condensed matter physics involves the search for states of matter with new emergent properties and desirable functionalities. Although the tools for material design remain relatively limited, notable advances…

Strongly Correlated Electrons · Physics 2023-06-21 Jacqueline Bloch , Andrea Cavalleri , Victor Galitski , Mohammad Hafezi , Angel Rubio

The physics governing electron acceleration by a relativistically intense laser are not confined to the critical density surface, they also pervade the sub-critical plasma in front of the target. Here, particles can gain many times the…

Pushing the limits of precision and reproducibility in ultrafast laser-based nanostructuring requires detailed control over the properties of the illumination. Most traditional methods of laser-based manufacturing rely on the simplicity of…

Optics · Physics 2023-06-13 Camilo Florian , Xiaohan Du , Craig B. Arnold

We study photoinduced optical responses of one-dimensional strongly correlated electron systems. The optical conductivity spectra are calculated for the ground state and a photoexcited state in the one-dimensional Hubbard model at half…

Strongly Correlated Electrons · Physics 2009-11-11 Nobuya Maeshima , Kenji Yonemitsu

In single particle coherent x-ray diffraction imaging experiments, performed at x-ray free-electron lasers (XFELs), samples are exposed to intense x-ray pulses to obtain single-shot diffraction patterns. The high intensity induces…

Atomic and Molecular Clusters · Physics 2013-01-29 U. Lorenz , N. M. Kabachnik , E. Weckert , I. A. Vartanyants

Producing inward orientated streams of energetic electrons by intense laser pulses acting on solid targets is the most robust and accessible way of transferring the laser energy to particles, which underlies numerous applications, ranging…

Plasma Physics · Physics 2017-10-02 Joel Magnusson , Arkady Gonoskov , Mattias Marklund

Manipulating the structure of single photons in the ultrafast domain is enabling new quantum information processing technologies. At the picosecond timescale, quantum information can be processed before decoherence can occur. In this work,…

Using a new technique to directly detect current induced on a nearby electrode, we measure plasma oscillations in ultracold plasmas, which are influenced by the inhomogeneous and time-varying density and changing neutrality. Electronic…

Plasma Physics · Physics 2012-02-10 K. A. Twedt , S. L. Rolston

We study the ultrafast structural dynamics, in response to electronic excitations, in heterostructures composed of Au$_{923}$ nanoclusters on thin-film substrates with the use of femtosecond electron diffraction. Various forms of atomic…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

The desire to exert active optical control over matter is a unifying theme across multiple scientific disciplines, as exemplified by all-optical magnetic switching, light-induced metastable or exotic phases of solids and the coherent…

Strongly Correlated Electrons · Physics 2021-04-28 Jan Gerrit Horstmann , Bareld Wit , Gero Storeck , Claus Ropers

The electronic and structural properties of a material are strongly determined by its symmetry. Changing the symmetry via a photoinduced phase transition offers new ways to manipulate material properties on ultrafast timescales. However, in…

Strongly Correlated Electrons · Physics 2015-09-25 Simon Wall , Daniel Wegkamp , Laura Foglia , Joyeeta Nag , Richard F. Haglund , Julia Staehler , Martin Wolf

Important advances have recently been made in the search for materials with complex multi-phase landscapes that host photoinduced metastable collective states with exotic functionalities. In almost all cases so far, the desired phases are…

Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…

Optics · Physics 2026-02-05 Nelin Laštovičková Streshkova , Martin Kozák

The soft character of organic materials leads to strong coupling between molecular nuclear and electronic dynamics. This coupling opens the way to control charge transport in organic electronic devices by inducing molecular vibrational…