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High-energy, local multiplet excitations of the d-electrons are revealed in our inelastic neutron scattering measurements on the prototype magnetic insulator NiO. These become allowed by the presence of both non-zero crystal field and…

Strongly Correlated Electrons · Physics 2012-06-18 Young-June Kim , A. P. Sorini , C. Stock , T. G. Perring , J. van den Brink , T. P. Devereaux

Planned optical spectroscopy experiments in lawrencium (Lr, Z = 103) require accurate theoretical predictions of the location of spectral lines in order to narrow the experimental search window. We present ab initio calculations of the…

Atomic and Molecular Clusters · Physics 2021-12-01 E. V. Kahl , S. Raeder , E. Eliav , A. Borschevsky , J. C. Berengut

Laser beam quality is a key parameter for both industry and science. However, the most common measure, the M2 parameter, requires numerous intensity spatial-profiles for its determination. This is particularly inconvenient for modelling the…

Optics · Physics 2024-01-01 M. H. Griessmann , A. C. Martinez-Becerril , J. S. Lundeen

X-ray absorption spectroscopy measured at the $L$-edge of transition metals (TMs) is a powerful element-selective tool providing direct information about the correlation effects in the $3d$ states. The theoretical modeling of the…

We suggest to include the density of electron charge explicitly in the electron potential of density functional theory, rather than implicitly via exchange-correlation functionals. The advantages of the approach are conceptual and…

Materials Science · Physics 2007-05-23 Werner A. Hofer , Krisztian Palotas

Using local density approximation plus dynamical mean-field theory (LDA+DMFT), we have computed the valence band photoelectron spectra of highly popular multiferroic BiFeO$_{3}$. Within DMFT, the local impurity problem is tackled by exact…

Strongly Correlated Electrons · Physics 2018-03-16 Souvik Paul , Diana Iusan , P. Thunstrom , Y. O. Kvashnin , Johan Hellsvik , Manuel Pereiro , A. Delin , Biplab Sanyal , O. Eriksson

A natural orbital functional for electronic systems with any value of the spin is proposed. This energy functional is based on a new reconstruction for the two-particle reduced density matrix (2RDM) of the multiplet, that is, of the mixed…

Chemical Physics · Physics 2019-10-02 Mario Piris

A very popular ab-initio scheme to calculate electronic properties in solids is the use of hybrid functionals in density functional theory (DFT) that mixes a portion of Fock exchange with DFT functionals. In spite of their success, a major…

Materials Science · Physics 2015-05-20 Miguel A. L. Marques , Julien Vidal , Micael J. T. Oliveira , Lucia Reining , Silvana Botti

We study effects of electron-electron interactions and confinement potential on the magneto-optical absorption spectrum in the far-infrared range of lateral quantum dot molecules. We calculate far-infrared (FIR) spectra for three different…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Helle , A. Harju , R. M. Nieminen

We present a method to calculate the Landau levels and the corresponding edge states of two dimensional (2D) crystals using as a starting point their electronic structure as obtained from standard density functional theory (DFT). The DFT…

Mesoscale and Nanoscale Physics · Physics 2016-09-16 J. L. Lado , J. Fernandez-Rossier

The Local Molecular Field Theory (LMF) developed by Weeks and co-workers has proved successful for treating the structure and thermodynamics of a variety of non-uniform liquids. By reformulating LMF in terms of one-body direct correlation…

Soft Condensed Matter · Physics 2015-06-12 A. J. Archer , R. Evans

We study the electronic band-structure and transport properties of a CuO2-plane within the three-band Hubbard model. The Dynamical Mean-Field Theory (DMFT) is used to solve the many particle problem. The calculations show that the optical…

Strongly Correlated Electrons · Physics 2007-05-23 M. B. Zoelfl , Th. Maier , Th. Pruschke , J. Keller

We report on high-resolution photoluminescence (PL) spectroscopic and microscopic study of laterally coupled InAs/GaAs self-assembled quantum dots by using a low-temperature near-field scanning optical microscope. We have observed slightly…

Materials Science · Physics 2007-05-23 Young-Jun Yu , Haneol Noh , Gun Sang Jeon , Yasuhiko Arakawa , Wonho Jhe

Recent advances using Density Functional Theory (DFT) to augment Multiplet Ligand Field Theory (MLFT) have led to ab-initio calculations of many formerly empirical parameters. This development makes MLFT more predictive instead of…

Strongly Correlated Electrons · Physics 2023-05-01 Charles Cardot , Joshua Kas , Jared Abramson , John Rehr , Gerald T. Seidler

A new method for calculation of band structure has been proposed based on the Green's function theory and local sampling. Potential energy in the Hamiltonian of Schrodinger's equation is approximated with a series of sampled Dirac delta…

Mesoscale and Nanoscale Physics · Physics 2010-02-24 Milad Khoshnegar , Sina Khorasani , Amirhossein Hosseinnia

Bound states around an impurity are investigated for a two dimensional electron system in a strong magnetic field. Long-range Coulomb potential and related potentials are considered. Schr\"odinger equation is solved numerically to obtain…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Daijiro Yoshioka

We present a computational scheme to study spin excitations in magnetic materials from first principles. The central quantity is the transverse spin susceptibility, from which the complete excitation spectrum, including single-particle…

Materials Science · Physics 2010-03-04 Ersoy Sasioglu , Arno Schindlmayr , Christoph Friedrich , Frank Freimuth , Stefan Blügel

We present a new method to calculate optical properties of strongly correlated systems. It is based on dynamical mean field theory and it uses as an input realistic electronic structure obtained by local density functional calculations.…

Strongly Correlated Electrons · Physics 2007-05-23 V. S. Oudovenko , G. Palsson , K. Haule , S. Y. Savrasov , G. Kotliar

A new method (NM) for filtering three-dimensional reconstructed densities is proposed. The algorithm is tested with simulated spectra and employed to study the electronic structure of the rare-earth compound LaB6. For this system, momentum…

Materials Science · Physics 2007-05-23 G. Kontrym-Sznajd , M. Samsel-Czekala , M. Biasini , Y. Kubo

LDA+DMFT (Local Density Approximation combined with Dynamical Mean-Field Theory) computation scheme has been used to calculate spectral properties of LaFeAsO -- the parent compound of the new high-T_c iron oxypnictides. The average Coulomb…

Strongly Correlated Electrons · Physics 2009-06-18 V. I. Anisimov , E. Z. Kurmaev , A. Moewes , I. A. Izyumov