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Experimentally resolving atomic-scale structural changes of a deformed glass remains challenging owing to the disordered nature of glass structure. Here, we show that the structural anisotropy emerges as a general hallmark for different…

At temperatures well below their glass transition, the deformation properties of bulk metallic glasses are characterised by a sharp transition from elasticity to plasticity, a reproducible yield stress, and an approximately linear decrease…

Soft Condensed Matter · Physics 2013-11-18 P. M. Derlet , R. Maaß

Understanding and controlling physical aging, i.e. the spontaneous temporal evolution of out-of-equilibrium systems, represents one of the greatest tasks in material science. Recent studies have revealed the existence of a complex atomic…

Materials Science · Physics 2016-02-17 V. M. Giordano , B. Ruta

We use coherent X-rays to probe the aging dynamics of a metallic glass directly on the atomic level. Contrary to the common assumption of a steady slowing down of the dynamics usually observed in macroscopic studies, we show that the…

Materials Science · Physics 2015-10-23 Zach Evenson , Beatrice Ruta , Simon Hechler , Moritz Stolpe , Eloi Pineda , Isabella Gallino , Ralf Busch

Dynamic and structural heterogeneities play an important role in glass transition phenomena and in the formation of amorphous structures. Since structure and dynamics are mutually related, it is expected that there exists some relation…

We use X-Ray Photon Correlation Spectroscopy to investigate the structural relaxation process in a metallic glass on the atomic length scale. We report evidence for a dynamical crossover between the supercooled liquid phase and the…

Soft Condensed Matter · Physics 2015-06-11 B. Ruta , Y. Chushkin , G. Monaco , L. Cipelletti , E. Pineda , P. Bruna , V. M. Giordano , M. Gonzalez-Silveira

A fascinating feature of metallic glasses is their ability to explore different configurations under mechanical deformations. This effect is usually observed through macroscopic observables, while little is known on the consequence of the…

Disordered Systems and Neural Networks · Physics 2023-01-09 A. Cornet , G. Garbarino , F. Zontone , Y. Chushkin , J. Jacobs , E. Pineda , T. Deschamps , S. Li , A. Ronca , J. Shen , G. Morard , N. Neuber , M. Frey , R. Busch , I. Gallino , M. Mezouar , G. Vaughan , B. Ruta

Strong changes in bulk properties, such as modulus and viscosity, are observed near the glass transition temperature, T_{g}, of amorphous materials. For more than a century, intense efforts have been made to define a microscopic origin for…

Disordered Systems and Neural Networks · Physics 2024-04-24 Joseph B. Schlenoff , Khalil Akkaoui

To experimentally clarify the changes in structural and dynamic heterogeneities in a metallic glass (MG), Gd65Co35, by rejuvenation with a temperature cycling (cryogenic rejuvenation), high-energy x-ray diffraction (HEXRD), anomalous x-ray…

Cycling of a metallic glass between ambient and cryogenic temperatures can induce higher-energy states characteristic of glass formation on faster cooling. This rejuvenation, unexpected because it occurs at small macroscopic strains and…

Disordered Systems and Neural Networks · Physics 2022-09-22 Baoshuang Shang , Weihua Wang , Alan Lindsay Greer , Pengfei Guan

The structural relaxation, potential energy states, and mechanical properties of a model glass subjected to thermal cycling are investigated using molecular dynamics simulations. We study a non-additive binary mixture which is annealed with…

Soft Condensed Matter · Physics 2018-12-05 Nikolai V. Priezjev

The influence of static stress and alternating loading direction on the potential energy and mechanical properties of amorphous alloys is investigated using molecular dynamics simulations. The model glass is represented via a binary mixture…

Soft Condensed Matter · Physics 2021-02-09 Nikolai V. Priezjev

The yielding transition, structural relaxation, and mechanical properties of metallic glasses subjected to repeated loading are examined using molecular dynamics simulations. We consider a poorly-annealed Cu-Zr amorphous alloy periodically…

Soft Condensed Matter · Physics 2024-08-30 Nikolai V. Priezjev

We examine the structural relaxation of glassy materials at finite temperatures, considering the effect of activated rearrangements and long-range elastic interactions. Our three-dimensional mesoscopic relaxation model shows how the…

Soft Condensed Matter · Physics 2023-12-20 Gieberth Rodriguez-Lopez , Kirsten Martens , Ezequiel E. Ferrero

Using molecular dynamics simulations, we investigate the effect of uniaxial elastostatic compression on the potential energy, structural relaxation, and mechanical properties of binary glasses. We consider the three-dimensional Kob-Andersen…

Soft Condensed Matter · Physics 2019-06-12 Nikolai V. Priezjev

We rejuvenate well-aged quasi-2D binary colloidal glasses by thermal cycling, and systematically measure both the statistical responses and particle-level structural evolutions during rejuvenation. While the moduli and boson peak are…

Soft Condensed Matter · Physics 2018-12-03 Xiunan Yang , Hua Tong , Weihua Wang , Ke Chen

The process of structural relaxation in disordered solids subjected to repeated tension-compression loading is studied using molecular dynamics simulations. The binary glass is prepared by rapid cooling well below the glass transition…

Soft Condensed Matter · Physics 2020-05-04 Pritam Kumar Jana , Nikolai V. Priezjev

We theoretically investigate the temperature dependence of the reversible structural relaxation time and diffusion constant of metallic glasses under pressure. The compression not only changes the glassy dynamics, but also generates a…

Materials Science · Physics 2021-05-28 Nguyen K. Ngan , Anh D. Phan , Alessio Zaccone

Modern detector technology and highly brilliant fourth-generation synchrotrons allow to improve the temporal resolution in time-resolved diffraction studies. Profiting from this, we applied temperature scanning X-ray photon correlation…

Residual stress engineering is very widely used in the design of new advanced lightweight materials. For metallic glasses the attention has been on structural changes and rejuvenation processes. High energy scanning X-ray diffraction strain…

Materials Science · Physics 2022-10-12 D. Şopu , F. Spieckermann , X. L. Bian , S. Fellner , J. Wright , M. Cordill , C. Gammer , G. Wang , M. Stoica , J. Eckert
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