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Key to advancing lithium-ion battery technology, and in particular fast charging capabilities, is our ability to follow and understand the dynamic processes occurring in operating materials under realistic conditions, in real time, and on…

Materials Science · Physics 2021-06-28 Alice J. Merryweather , Christoph Schnedermann , Quentin Jacquet , Clare P. Grey , Akshay Rao

Accurate battery lifetime prediction is important for preventative maintenance, warranties, and improved cell design and manufacturing. However, manufacturing variability and usage-dependent degradation make life prediction challenging.…

Machine Learning · Computer Science 2024-04-23 Tingkai Li , Zihao Zhou , Adam Thelen , David Howey , Chao Hu

Fast-charging of lithium-ion batteries is essential for electric vehicle adoption, but aggressive charging can accelerate its degradation and create safety risks. This study investigates a control framework that coordinates charging current…

Systems and Control · Electrical Eng. & Systems 2026-05-26 Frederic Fabry , Alessio Lodge , Robinson Medina , Feye Hoekstra , Steven Wilkins , Madalin Frunzete

This contribution presents a diagnosis scheme for batteries to detect and isolate internal faults in the form of small parameter changes. This scheme is based on an electrochemical reduced-order model of the battery, which allows the…

Systems and Control · Electrical Eng. & Systems 2021-03-19 Luis D. Couto , Jorn M. Reniers , David A. Howey , Michel Kinnaert

The unified 3D phase-field model for the description of the lithium-ion cell as a whole is developed. The model takes into account the realistic distribution of particles in porous electrodes, percolative transport of ions, and the…

Disordered Systems and Neural Networks · Physics 2021-05-11 Pavel E. L'vov , Mikhail Yu. Tikhonchev , Renat T. Sibatov

To develop a high-density and long-life lithium-ion battery, a technology is needed that allows non-destructive visualization of the spatial distribution of deteriorated parts after cycle test. In the present study, we measured the…

Chemical Physics · Physics 2021-05-26 Shogo Suzuki , Hideaki Okada , Kai Yabumoto , Seiju Matsuda , Yuki Mima , Noriaki Kimura , Kenjiro Kimura

Lithium-ion batteries (LIBs) of high energy density and light-weight design, have found wide applications in electronic devices and systems. Degradation mechanisms that caused by lithiation is a main challenging problem for LIBs with high…

Computational Engineering, Finance, and Science · Computer Science 2020-06-26 Masoud Ahmadi

Lithium-ion batteries exhibit complex nonlinear dynamics, resulting from diffusion and phase transformations coupled to ion intercalation reactions. Using the recently developed Cahn-Hilliard reaction (CHR) theory, we investigate a simple…

Chemical Physics · Physics 2014-02-13 Yi Zeng , Martin Z. Bazant

Fracture of lithium-ion battery electrodes is found to contribute to capacity fade and reduce the lifespan of a battery. Traditional fracture models for batteries are restricted to consideration of a single, idealised particle; here,…

In this paper we study a system of partial differential equations which models lithium-ion batteries. The system describes the conservation of Lithium and conservation of charges in the solid and electrolyte phases, together with the…

Analysis of PDEs · Mathematics 2022-02-08 Xiangsheng Xu

The Doyle-Fuller-Newman (DFN) model is a common mechanistic model for lithium-ion batteries. The reaction rate constant and diffusivity within the DFN model are key parameters that directly affect the movement of lithium ions, thereby…

Systems and Control · Electrical Eng. & Systems 2025-04-15 Marc D. Berliner , Minsu Kim , Xiao Cui , Vivek N. Lam , Patrick A. Asinger , Martin Z. Bazant , William C. Chueh , Richard D. Braatz

This letter proposes a lightweight, model-free online diagnostic framework for detecting internal short circuits (ISC) in single lithium-ion cells under dynamic operating conditions. The core of the method lies in computing the first-order…

Systems and Control · Electrical Eng. & Systems 2025-06-17 Yangyang Xu , Chenglin Liao

Lithium-ion (Li-ion) batteries are ubiquitous in electric vehicles (EVs) as efficient energy storage devices. The reliable operation of Li-ion batteries depends critically on the accurate estimation of battery capacity. However,…

Systems and Control · Electrical Eng. & Systems 2025-11-11 Yang Wang , Marta Zagorowska , Riccardo M. G. Ferrari

Compton scattering imaging using high-energy synchrotron x-rays allows the visualization of the spatio-temporal lithiation state in lithium-ion batteries probed in-operando. Here, we apply this imaging technique to the commercial 18650-type…

The complex electrochemical behavior of lithium-ion batteries results in non-linear dynamics and appropriate modeling of this non-linear dynamical system is of interest for better management and control. In this work, we proposed a family…

Systems and Control · Electrical Eng. & Systems 2026-02-25 Khalid Mahmud Labib , Shabbir Ahmed

Parameterisation of coupled degradation mechanisms in lithium-ion batteries is a major challenge. Interactions between the mechanisms depend on usage conditions: C-rate, rest state-of-charge (SoC), depth-of-discharge (DoD) and temperature.…

Materials Science · Physics 2026-04-13 Ganesh Madabattula

Higher energy density and longer lifetime are the requirements for next-generation lithium-ion batteries. A promising anode material is silicon, which offers high specific capacity, but its significant volume change during lithiation and…

Ultrahigh rate performance of active particles used in lithium-ion battery electrodes has been revealed by single-particle measurements, which indicates a huge potential for developing high-power batteries. However, the charging/discharging…

Chemical Physics · Physics 2022-07-25 Ruoyu Xiong , Mengyuan Zhou , Longhui Li , Jia Xu , Maoyuan Li , Bo Yan , Dequn Li , Yun Zhang , Huamin Zhou

This work optimizes a lithium-ion battery charging schedule while considering a joint revenue and battery degradation model. The study extends the work of Meheswari et. al. to encourage battery usage/charging at optimal intervals depending…

Optimization and Control · Mathematics 2022-06-01 Jacob Azoulay , Nico Carballal

This paper presents a combination of machine learning techniques to enable prompt evaluation of retired electric vehicle batteries as to either retain those batteries for a second-life application and extend their operation beyond the…

Systems and Control · Electrical Eng. & Systems 2023-04-10 Aki Takahashi , Anirudh Allam , Simona Onori