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We demonstrate the feasibility of quantum computing for large-scale, realistic chemical systems through the development of a new interface using a quantum circuit simulator and CP2K, a highly efficient first-principles calculation software.…

Chemical Physics · Physics 2025-06-24 Tomoya Shiota , Klaas Gunst , Toshio Mori , Toru Shiozaki , Wataru Mizukami

Machine learning has emerged recently as a powerful tool for predicting properties of quantum many-body systems. For many ground states of gapped Hamiltonians, generative models can learn from measurements of a single quantum state to…

Quantum Physics · Physics 2024-03-05 Haoxiang Wang , Maurice Weber , Josh Izaac , Cedric Yen-Yu Lin

We propose a scheme for the construction of one-particle Green's function (GF) of an interacting electronic system via statistical sampling on a quantum computer. Although the non-unitarity of creation and annihilation operators for the…

Quantum Physics · Physics 2020-02-19 Taichi Kosugi , Yu-ichiro Matsushita

Constrained Hamiltonian description of the classical limit is utilized in order to derive consistent dynamical equations for hybrid quantum-classical systems. Starting with a compound quantum system in the Hamiltonian formulation conditions…

Quantum Physics · Physics 2012-06-08 M. Radonjic , S. Prvanovic , N. Buric

Quantum algorithms on the noisy intermediate-scale quantum (NISQ) devices are expected to simulate quantum systems that are classically intractable to demonstrate quantum advantages. However, the non-negligible gate error on the NISQ…

Quantum Physics · Physics 2021-12-06 Joseph C. Aulicino , Trevor Keen , Bo Peng

Quantum Hamiltonian Computing is a recent approach that uses quantum systems, in particular a single molecule, to perform computational tasks. Within this approach, we present explicit methods to construct logic gates using two different…

Quantum Physics · Physics 2019-06-18 Omid Faizy Namarvar , Olivier Giraud , Bertrand Georgeot , Christian Joachim

In this work we propose an approach for implementing time-evolution of a quantum system using product formulas. The quantum algorithms we develop have provably better scaling (in terms of gate complexity and circuit depth) than a naive…

We present an approach to simulating quantum computation based on a classical model that directly imitates discrete quantum systems. Qubits are represented as harmonic functions in a 2D vector space. Multiplication of qubit representations…

Quantum Physics · Physics 2009-06-30 Steven Peil

Exponentiation of Hamiltonians refers to a mathematical operation to a Hamiltonian operator, typically in the form e^(-i.t.H), where H is the Hamiltonian and t is a time parameter. This operation is fundamental in quantum mechanics,…

Quantum Physics · Physics 2025-02-11 Gerard Fleury , Philippe Lacomme

This work provides a rigorous and self-contained introduction to numerical methods for Hamiltonian simulation in quantum computing, with a focus on high-order product formulas for efficiently approximating the time evolution of quantum…

Quantum Physics · Physics 2025-07-16 Javier Lopez-Cerezo

The optimal use of quantum and classical computational techniques together is important to address problems that cannot be easily solved by quantum computations alone. This is the case of the ground state problem for quantum many-body…

Quantum Physics · Physics 2022-05-03 Patrick Huembeli , Giuseppe Carleo , Antonio Mezzacapo

We describe a simple formalism for generating classes of quantum circuits that are classically efficiently simulatable and show that the efficient simulation of Clifford circuits (Gottesman-Knill theorem) and of matchgate circuits…

Quantum Physics · Physics 2008-12-25 Richard Jozsa

A methodology for solving two-point boundary value problems in phase space for Hamiltonian systems is presented. Using Hamilton-Jacobi theory in conjunction with the canonical transformation induced by the phase flow, we show that the…

Dynamical Systems · Mathematics 2007-05-23 Vincent M Guibout , Daniel J Scheeres

The method of many-body Green's functions is developed for arbitrary systems of electrons and nuclei starting from the full (beyond Born-Oppenheimer) Hamiltonian of Coulomb interactions and kinetic energies. The theory presented here…

Other Condensed Matter · Physics 2020-06-23 Ville J. Härkönen , Robert van Leeuwen , E. K. U. Gross

We revisit quantum phase estimation algorithms for the purpose of obtaining the energy levels of many-body Hamiltonians and pay particular attention to the statistical analysis of their outputs. We introduce the mean phase direction of the…

Quantum Physics · Physics 2020-08-20 P. M. Q. Cruz , G. Catarina , R. Gautier , J. Fernández-Rossier

Quantum Imaginary-Time Evolution (QITE) is a powerful method for preparing ground states on quantum hardware. However, executing QITE has costly measurement budgets for general Hamiltonians. Both fidelity and computational cost are strongly…

Quantum Physics · Physics 2025-12-12 Julio Del Castillo , Mats Granath , Evert van Nieuwenburg

Expectation value estimation is ubiquitous in quantum algorithms. The expectation value of a Hamiltonian, which is essential in various practical applications, is often estimated by measuring a large number of Pauli strings on quantum…

The quantum circuit model is the de-facto way of designing quantum algorithms. Yet any level of abstraction away from the underlying hardware incurs overhead. In the era of near-term, noisy, intermediate-scale quantum (NISQ) hardware with…

Quantum Physics · Physics 2021-08-27 Laura Clinton , Johannes Bausch , Toby Cubitt

Without wasting time and effort on philosophical justifications and implications, we write down the conditions for the Hamiltonian of a quantum system for rendering it mathematically equivalent to a deterministic system. These are the…

Quantum Physics · Physics 2020-06-09 Gerard t Hooft

We study some properties of the canonical transformations in classical mechanics and quantum field theory and give a number of practical formulas concerning their generating functions. First, we give a diagrammatic formula for the…

High Energy Physics - Theory · Physics 2016-04-06 Damiano Anselmi
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