English
Related papers

Related papers: Speedup of nuclear-spin diffusion in hyperpolarize…

200 papers

There has been much renewed interest in dynamic nuclear polarization (DNP), particularly in the context of solid state biomolecular NMR and more recently dissolution DNP techniques for liquids. This paper reviews the role of spin diffusion…

Other Condensed Matter · Physics 2009-04-01 Chandrasekhar Ramanathan

We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…

Mesoscale and Nanoscale Physics · Physics 2019-02-04 Thomas Nutz , Edwin Barnes , Sophia E. Economou

The theory of spin diffusion is extended to the case of spin lattice relaxation and spin diffusion in an inhomogeneous field in spin systems with non-equidistant energy spectrum. Two coupled equations describing the mutual relaxation and…

Materials Science · Physics 2007-05-23 Gregory B. Furman , Shaul D. Goren

The hyperpolarization of nuclear spins can enable powerful imaging and sensing techniques provided the hyperpolarization is sufficiently long-lived. Recent experiments on nanodiamond $^{13}$C nuclear spins demonstrate that relaxation times…

Mesoscale and Nanoscale Physics · Physics 2024-02-20 Gargee Sharma , Torsten Gaebel , Ewa Rej , David J. Reilly , Sophia E. Economou , Edwin Barnes

The spin dynamics of localized donor-bound electrons interacting with the nuclear spin ensemble in $n$-doped GaAs epilayers is studied using nuclear spin polarization by light with modulated circular polarization. We show that the observed…

Coherent two-level systems, or qubits, based on electron spins in GaAs quantum dots are strongly coupled to the nuclear spins of the host lattice via the hyperfine interaction. Realizing nuclear spin control would likely improve electron…

Mesoscale and Nanoscale Physics · Physics 2010-06-15 D. J. Reilly , J. M. Taylor , J. R. Petta , C. M. Marcus , M. P. Hanson , A. C. Gossard

Nuclear spin hyperpolarization provides a promising route to overcome the challenges imposed by the limited sensitivity of nuclear magnetic resonance. Here we demonstrate that dissolution of spin-polarized pentacene-doped naphthalene…

Repeated injection of spin polarized carriers in a quantum dot leads to the polarization of nuclear spins, a process known as dynamic nuclear spin polarization (DNP). Here, we report the first observation of p-shell carrier assisted DNP in…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 C. F. Fong , Y. Ota , E. Harbord , S. Iwamoto , Y. Arakawa

Intermediate-energy heavy-ion collisions can produce a spin polarization of the projectile-like species. Spin polarization has been observed for both nucleon removal and nucleon pickup processes. Qualitative agreement with measured spin…

Nuclear Experiment · Physics 2008-11-26 D. E. Groh , J. S. Pinter , P. F. Mantica , T. J. Mertzimekis , A. E. Stuchbery , D. T. Khoa

We exploit spin noise spectroscopy (SNS) to directly observe build-up of dynamic nuclear polarization and relaxation of a perturbed nuclear spin-system to its equilibrium state in a single-shot experiment. The SNS experiments were performed…

We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum…

We theoretically investigate thermalization and spin diffusion driven by a quantum spin bath for a realistic solid-state NMR experiment. We consider polycrystalline L-alanine, and investigate how the spin polarization spreads among several…

Quantum Physics · Physics 2019-01-17 Walter Hahn , V. V. Dobrovitski

We describe a method to hyperpolarize 3He nuclear spins at high magnetic fields (4.7 Tesla) solely by a magnetized plasma. The conditions for such a magnetized plasma are fulfilled when the mean free path of the free electrons is much…

Atomic Physics · Physics 2018-12-12 A. Maul , P. Blümler , P. -J. Nacher , E. Otten , G. Tastevin , W. Heil

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…

Mesoscale and Nanoscale Physics · Physics 2013-06-07 Xiao-Feng Shi

Optically polarizable nitrogen-vacancy (NV) center in diamond enables the hyperpolarization of $^{13}$C nuclear spins at low magnetic field and room temperature. However, achieving a high level of polarization comparable to conventional…

Quantum Physics · Physics 2024-10-01 Vladimir V. Kavtanyuk , Changjae Lee , Keunhong Jeong , Jeong Hyun Shim

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

We report on the dynamic nuclear polarization of a single charge-tunable self-assembled InAs/GaAs quantum dot in a longitudinal magnetic field of $\sim$0.2T. The hyperfine interaction between the optically oriented electron and nuclei spins…

A new method for local dynamic nuclear polarization is demonstrated in a GaAs/AlGaAs heterostructure at the Landau level filling factor $\nu=3$. Using a narrow channel sample, where the width varies stepwise along the electron flow, we find…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yosuke Komori , Tohru Okamoto

The effect of nuclear spins in Fe/GaAs all-electrical spin-injection devices is investigated. At temperatures below 50 K, strong modifications of the non-local spin signal are found that are characteristic for hyperfine coupling between…

Mesoscale and Nanoscale Physics · Physics 2010-04-08 G. Salis , A. Fuhrer , S. F. Alvarado