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The enhancement of the spin-space symmetry from the usual $\mathrm{SU}(2)$ to $\mathrm{SU}(N)$ with $N>2$ is promising for finding nontrivial quantum spin liquids, but the realization of $\mathrm{SU}(N)$ spin systems in real materials is…

Strongly Correlated Electrons · Physics 2020-04-07 Masahiko G. Yamada

While the enhancement of the spin-space symmetry from the usual $\mathrm{SU}(2)$ to $\mathrm{SU}(N)$ is promising for finding nontrivial quantum spin liquids, its realization in magnetic materials remains challenging. Here we propose a new…

Strongly Correlated Electrons · Physics 2018-09-12 Masahiko G. Yamada , Masaki Oshikawa , George Jackeli

In addition to low-energy spin fluctuations, which distinguish them from band insulators, Mott insulators often possess orbital degrees of freedom when crystal-field levels are partially filled. While in most situations spins and orbitals…

Strongly Correlated Electrons · Physics 2012-11-28 P. Corboz , M. Lajkó , A. M. Läuchli , K. Penc , F. Mila

The $\mathrm{SU}(4)$ Heisenberg model on the honeycomb lattice is expected to host a quantum spin-orbital liquid at low temperature with an astonishing candidate material, $\alpha$-ZrCl$_3$. We employed the canonical thermal pure quantum…

Strongly Correlated Electrons · Physics 2022-07-15 Masahiko G. Yamada , Satoshi Fujimoto

We study the effective spin-orbital model that describes the magnetism of 4$d^1$ or 5$d^1$ Mott insulators in ideal tricoordinated lattices. In the limit of vanishing Hund's coupling, the model has an emergent SU(4) symmetry which is made…

Strongly Correlated Electrons · Physics 2018-11-21 Willian M. H. Natori , Eric C. Andrade , Rodrigo G. Pereira

We perform large-scale density matrix renormalization group simulations of the $\mathrm{SU}(4)$ Heisenberg model on the honeycomb lattice and resolve the long-standing question of its ground state in an unbiased and quantitatively…

Strongly Correlated Electrons · Physics 2026-02-03 Masahiko G. Yamada

Quantum spin-orbital liquids are elusive strongly correlated states of matter that emerge from quantum frustration between spin and orbital degrees of freedom. A promising route towards the observation of those states is the creation of…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Xu Dou , Valeri N. Kotov , Bruno Uchoa

We study the strong coupling model of $d^1$ transition metal tri-halides in the large spin-orbit coupled limit. By considering ab-initio-calculation-inspired hierarchy of hopping pathways of these compounds, SU(4) symmetry is found to…

Strongly Correlated Electrons · Physics 2025-08-27 Manoj Gupta , Arijit Haldar , Subhro Bhattacharjee , Tanusri Saha-Dasgupta

Motivated by the absence of both spin freezing and a cooperative Jahn-Teller effect at the lowest measured temperatures, we study the ground state of Ba3CuSb2O9. We solve a general spin-orbital model on both the honeycomb and the decorated…

Strongly Correlated Electrons · Physics 2014-10-02 Andrew Smerald , Frederic Mila

The SU(4)-symmetric spin-orbital model on the honeycomb lattice was recently studied in connection to correlated insulators such as the $e_{g}$ Mott insulator Ba$_{3}$CuSb$_{2}$O$_{9}$ and the insulating phase of magic-angle twisted bilayer…

Strongly Correlated Electrons · Physics 2019-11-27 W. M. H. Natori , R. Nutakki , R. G. Pereira , E. C. Andrade

We use a projective symmetry group analysis to determine all symmetric spin liquids on the stuffed honeycomb lattice Heisenberg model. This lattice interpolates between honeycomb, triangular and dice lattices, always preserving hexagonal…

Strongly Correlated Electrons · Physics 2020-03-10 Jyotisman Sahoo , Rebecca Flint

The SU(4) Heisenberg model can serve as a low energy model of the Mott insulating state in materials where the spins and orbitals are highly symmetric, or in systems of alkaline-earth atoms on optical lattice. Recently, it has been argued…

Strongly Correlated Electrons · Physics 2013-06-28 Miklos Lajko , Karlo Penc

Dirac spin liquids represent a class of highly-entangled quantum phases in two dimensional Mott insulators, featuring exotic properties such as critical correlation functions and absence of well-defined low energy quasi-particles. Existing…

Strongly Correlated Electrons · Physics 2021-03-30 Vladimir Calvera , Chong Wang

We report the discovery of a novel gapless quantum spin liquid in the S=1 honeycomb system Cu$_3$LiRu$_2$O$_6$ with Ru$^{4+}$ ($4d^4$) where moments remain dynamic down to 50 mK. Heat capacity measurements show no sign of magnetic ordering…

We construct a tight-binding model of [(C$_2$H$_5$)$_3$NH]$_2$Cu$_2$(C$_2$O$_4$)$_3$ from Wannier orbital overlaps. Including interactions within the Jahn-Teller distorted Cu-centered $e_g$ Wannier orbitals leads to an effective Heisenberg…

Strongly Correlated Electrons · Physics 2022-05-24 A. C. Jacko , B. J. Powell

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

We present a quantu spin liquid state in a spin-1/2 honeycomb lattice with randomness in the exchange interaction. That is, we successfully introduce randomness into the organic radial-based complex and realize a random-singlet (RS) state.…

Strongly Correlated Electrons · Physics 2017-09-26 H. Yamaguchi , M. Okada , Y. Kono , S. Kittaka , T. Sakakibara , T. Okabe , Y. Iwasaki , Y. Hosokoshi

Spiral spin-liquids are correlated paramagnetic states with degenerate propagation vectors forming a continuous ring or surface in reciprocal space. On the honeycomb lattice, spiral spin-liquids present a novel route to realize emergent…

We provide an exact study of dynamical correlations for the quantum spin-orbital liquid phases of an SU(2)-symmetric Kitaev honeycomb lattice model. We show that the spin dynamics in this Kugel-Khomskii type model is exactly the…

Strongly Correlated Electrons · Physics 2020-08-07 Willian M. H. Natori , Johannes Knolle

Quantum spin liquids have been at the forefront of correlated electron research ever since their original proposal in 1973, and the realization that they belong to the broader class of intrinsic topological orders, along with the fractional…

Strongly Correlated Electrons · Physics 2018-04-26 Ioannis Rousochatzakis , Yuriy Sizyuk , Natalia B. Perkins
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