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We visualize entanglements in polymer melts using molecular dynamics simulation. A bead at an entanglement interacts persistently for long times with the non-bonded beads (those excluding the adjacent ones in the same chain). The…

Soft Condensed Matter · Physics 2009-11-10 Ryoichi Yamamoto , Akira Onuki

Equilibration of polymer melts containing highly entangled long polymer chains in confinement or with free surfaces is a challenge for computer simulations. We approach this problem by first studying polymer melts based on the soft-sphere…

Soft Condensed Matter · Physics 2020-10-14 Hsiao-Ping Hsu , Kurt Kremer

We simulate entangled linear polymers in free-standing thin film geometries where the confining dimension is on the same scale or smaller than the bulk chain dimensions. We compare both film-averaged and layer-resolved, spatially…

Soft Condensed Matter · Physics 2016-08-24 Daniel M. Sussman

Topologically constrained genome-like polymers often double-fold into tree-like configurations. Here we calculate the exact number of tightly double-folded configurations available to a ring polymer in ideal conditions. For this purpose, we…

Soft Condensed Matter · Physics 2026-03-02 Pieter H. W. van der Hoek , Angelo Rosa , Elham Ghobadpour , Ralf Everaers

Entangled networks of stiff biopolymers exhibit complex dynamic response, emerging from the topological constraints that neighboring filaments impose upon each other. We propose a class of reference models for entanglement dynamics of stiff…

Soft Condensed Matter · Physics 2008-06-23 Felix Höfling , Tobias Munk , Erwin Frey , Thomas Franosch

We present simulations on a binary blend of bead-spring polymer chains. The introduction of monomer size disparity yields very different relaxation times for each component of the blend. Competition between two different arrest mechanisms,…

Soft Condensed Matter · Physics 2007-05-23 Angel J. Moreno , Juan Colmenero

We study stress relaxation in bi-disperse entangled polymer solutions. Shorter chains embedded in a majority of longer ones are known to be oriented by coupling to them. We analyze the mechanism for this both by computer simulation and…

Soft Condensed Matter · Physics 2013-05-29 J. M. Deutsch , J. H. Pixley

We study conformational properties of diluted dumbbell polymers which consist of two rings that are attached to both ends of a linear spacer segment by using analytical methods of field theory and bead-spring coarse-grained molecular…

Soft Condensed Matter · Physics 2023-03-22 Khristine Haydukivska , Viktoria Blavatska , Jaroslaw Paturej

We investigate with numerical simulations the molecular origin of viscosity in melts of flexible and semiflexible oligomer rings in comparison to corresponding systems with linear chains. The strong increase of viscosity with ring stiffness…

Soft Condensed Matter · Physics 2023-07-28 Ranajay Datta , Fabian Berressem , Friederike Schmid , Arash Nikoubashman , Peter Virnau

A model of two interacting polymer chains has been proposed to study the effect of penetration of one chain in to the other. We show that small chain penetrates more in comparison to the long chain. We also find a condition in which both…

Statistical Mechanics · Physics 2009-10-31 Sanjay Kumar

Brownian motion and viscoelasticity of semiflexible polymers is a subject that has been studied for many years. Still, rigorous analysis has been hindered due to the difficulty in handling the constraint that polymer chains cannot be…

Soft Condensed Matter · Physics 2024-05-22 Zhongqiang Xiong , Ryohei Seto , Masao Doi

During the life cycle of bacterial cells the non-mixing of the two ring-shaped daughter genomes is an important prerequisite for the cell division process. Mimicking the environments inside highly crowded biological cells, we study the…

Soft Condensed Matter · Physics 2014-12-24 Jaeoh Shin , Andrey G Cherstvy , Ralf Metzler

The radius of gyration of a polymer chain immersed in a low molecular weight solvent is known to vary monotonically with the solvent quality. Here, we consider the behavior of a chain immersed in a high molecular weight solvent (polymer…

Soft Condensed Matter · Physics 2007-05-23 Cyprien Gay , Elie Raphael

The entanglement entropy of a subsystem of a quantum system is expressed, in the replica approach, through analytic continuation with respect to n of the trace of the n-th power of the reduced density matrix. This trace can be thought of as…

High Energy Physics - Theory · Physics 2008-12-18 Michele Caraglio , Ferdinando Gliozzi

We investigate the chain conformation of ring polymers confined to a cylindrical nanochannel using both theoretical analysis and three dimensional Langevin dynamics simulations. We predict that the longitudinal size of a ring polymer scales…

Soft Condensed Matter · Physics 2012-12-06 Junfang Sheng , Kaifu Luo

The block entanglement entropy and fluctuations are investigated in one dimension in finite size correlated electron systems using the Gutzwiller wave function as a prototype correlated electron state. Entanglement entropy shows logarithmic…

Strongly Correlated Electrons · Physics 2014-07-07 Archak Purkayastha , V. Subrahmanyam

The miscibility of polymer blends, a classical problem in polymer science, may be altered, if one or both of the component do not have chain ends. Based on the idea of {\it topological volume}, we propose a mean-field theory to clarify how…

Soft Condensed Matter · Physics 2016-05-04 Takahiro Sakaue , Chihiro H. Nakajima

Two ring polymers close to each other in space may be either in a segregated phase if there is a strong repulsion between monomers in the polymers, or intermingle in a mixed phase if there is a strong attractive force between the monomers.…

Soft Condensed Matter · Physics 2022-11-23 EJ Janse van Rensburg , E Orlandini , MC Tesi , SG Whittington

Molecular dynamics simulations confirm recent extensional flow experiments showing ring polymer melts exhibit strong extension-rate thickening of the viscosity at Weissenberg numbers $Wi<<1$. Thickening coincides with the extreme elongation…

Soft Condensed Matter · Physics 2020-01-22 Thomas C. O'Connor , Ting Ge , Michael Rubinstein , Gary S. Grest

It is nontrivial whether the average size of a ring polymer should become smaller or larger under a topological constraint. Making use of some knot invariants, we evaluate numerically the mean square radius of gyration for ring polymers…

Statistical Mechanics · Physics 2016-08-31 Miyuki K. Shimamura , Tetsuo Deguchi