Related papers: Vacuum-UV photodesorption from compact Amorphous S…
We investigated the behavior of H$_2$, main constituent of the gas phase in dense clouds, after collision with amorphous solid water (ASW) surfaces, one of the most abundant chemical species of interstellar ices. We developed a general…
We model the temperature and chemical structure of molecular clouds as a function of depth into the cloud, assuming a cloud of constant density n illuminated by an external FUV (6 eV < E < 13.6 eV) flux G_0 (scaling factor in multiples of…
We study the photoevaporation of Jeans-unstable molecular clumps by isotropic FUV (6 eV $< {\rm h}\nu$ < 13.6 eV) radiation, through 3D radiative transfer hydrodynamical simulations implementing a non-equilibrium chemical network that…
Methanol is a common component of interstellar and circumstellar ice mantles and is often used as an evolution indicator in star-forming regions. The observations of gas-phase methanol in the interiors of dense molecular clouds at…
We report the discovery of photomolecular effect: cleavage of water clusters off surfaces by photons. This effect is demonstrated through surprising absorption of partially wetted hydrogel in the visible spectrum where both water and…
The x-ray absorption spectra of water and ice are calculated with a many-body approach for electron-hole excitations. The experimental features, including the small effects of temperature change in the liquid, are quantitatively reproduced…
Using a combination of photostimulated desorption and resonance-enhanced multiphoton ionization methods, the behaviors of OH radicals on the surface of interstellar ice analog was monitored at temperatures between 54 and 80 K. The OH number…
Desorption of H2O films ranging from 53 nanometres to 101 micrometre thicknesses have been investigated using a quartz-crystal microbalance (QCM) and temperature-programmed desorption. Three desorption stages are observed belonging to…
Water ice covers the surface of various objects in the outer Solar system. Within the heliopause, surface ice is constantly bombarded and sputtered by energetic particles from the solar wind and magnetospheres. We report a laboratory…
The aim of this work is to draw attention to the processes of radiative charge exchange in non-symmetric ion-atom collisions as a factor of influence on the opacity of stellar atmospheres in VUV region. For that purpose calculations of the…
X-rays emitted from pre-main-sequence stars at the center of protoplanetary disks can induce nonthermal desorption from interstellar ices populating the cold regions. This X-ray photodesorption needs to be quantified for complex organic…
Photoabsorption spectra of N$_2$ and CO were recorded at 900K, using the vacuum-ultraviolet Fourier-transform spectrometer at the DESIRS beamline of synchrotron SOLEIL. These high-temperature and high-resolution measurements allow for…
The depth-dependent abundance of both gas-phase and solid-state water within dense, quiescent, molecular clouds is important to both the cloud chemistry and gas cooling. Where water is in the gas phase, it's free to participate in the…
Photon-stimulated desorption (PSD) is a process of interest for the two seemingly unrelated topics of accelerator vacuum dynamics and astrochemistry. Here we present an approach to studying PSD of interstellar ice analogs, i.e. condensed…
The astrochemistry of CO2 ice analogues has been a topic of intensive investigation due to the prevalence of CO2 throughout the interstellar medium and the Solar System, as well as the possibility of it acting as a carbon feedstock for the…
The standard model of cosmic ray heating-induced desorption of interstellar ices is based on a continuous representation of the sporadic desorption of ice mantle components from classical (0.1 micron) dust grains. This has been re-evaluated…
The mechanisms by which light interacts with ice and the impact of photo-induced reactions are central to our understanding of environmental, atmospheric and astrophysical processes. However, a microscopic description of the photoproducts…
The spectrometers onboard the Infrared Telescope in Space (IRTS) reveal water vapor absorption in early M-type stars, as early as M2. Previous observations detected H_2O vapor absorption only in stars later than M6, with the exception of…
Throughout their lives, short period exoplanets (<100 days) experience X-ray and extreme-UV (XUV) stellar irradiation that can heat and photoionize planets' upper atmospheres, driving transonic outflows. This photoevaporative mass loss…
We search for frozen water and its processing around young stellar objects (YSOs of class I/II). We try to detect potential, regional differences in water ice evolution within YSOs, which is relevant to understanding the chemical structure…