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Carbonic acid (H2CO3) is a weak acid relevant to astrobiology which, to date, remains undetected in space. Experimental work has shown that the beta-polymorph of H2CO3 forms under space relevant conditions through energetic (UV photon,…

Instrumentation and Methods for Astrophysics · Physics 2021-02-24 S. Ioppolo , Z. Kanuchová , R. L. James , A. Dawes , A. Ryabov , J. Dezalay , N. C. Jones , S. V. Hoffmann , N. J. Mason , G. Strazzulla

The study and quantification of UV photon-induced desorption of frozen molecules furthers our understanding of the chemical evolution of cold interstellar regions. Nitric oxide (NO) is an important intermediate species in both gas-phase and…

Astrophysics of Galaxies · Physics 2017-10-05 R. Dupuy , G. Féraud , M. Bertin , X. Michaut , T. Putaud , P. Jeseck , L. Philippe , C. Romanzin , V. Baglin , R. Cimino , J. -H. Fillion

Isoprene and its oligomers, terpenes, are expected to be present, along with other complex organic molecules, in the diverse environments of the ISM and in our solar system. Due to insufficient spectral information of these molecules at low…

Astrophysics of Galaxies · Physics 2025-09-26 R Ramachandran , S Pavithraa , J K Meka , K K Rahul , J -I Lo , S -L Chou , B -M Cheng , B N Rajasekhar , Anil Bhardwaj , N J Mason , B Sivaraman

At the high densities and low temperatures found in star forming regions, all molecules other than H2 should stick on dust grains on timescales shorter than the cloud lifetimes. Yet these clouds are detected in the millimeter lines of…

The HDO/H2O ratio in interstellar gas is often used to draw conclusions on the origin of water in star-forming regions and on Earth. In cold cores and in the outer regions of protoplanetary disks, gas-phase water comes from photodesorption…

Astrophysics of Galaxies · Physics 2015-03-11 Carina Arasa , Jesper Koning , Geert-Jan Kroes , Catherine Walsh , Ewine F. van Dishoeck

Wavelength dependent photodesorption rates have been determined using synchrotron radiation, for condensed pure and mixed methanol ice in the 7 -- 14 eV range. The VUV photodesorption of intact methanol molecules from pure methanol ices is…

Laboratory results of the optical properties of vapor-deposited water ice, specifically the refractive index and extinction coefficient, are available mainly for a selective set of wavelengths and a limited number of deposition…

Instrumentation and Methods for Astrophysics · Physics 2022-02-09 Jiao He , Sharon J. M. Diamant , Siyu Wang , Haochuan Yu , Will R. M. Rocha , Marina Rachid , Harold Linnartz

Under cosmic irradiation, the interstellar water ice mantles evolve towards a compact amorphous state. Crystalline ice amorphisation was previously monitored mainly in the keV to hundreds of keV ion energies. We experimentally investigate…

Ice mantles detected on the surface of dust grains toward the coldest regions of the interstellar medium can be photoprocessed by the secondary ultraviolet (UV) field present in dense cloud interiors. In this work, we present UV-irradiation…

Astrophysics of Galaxies · Physics 2017-11-15 R. Martin-Domenech , G. A. Cruz-Diaz , G. M. Munoz Caro

The photodesorption efficiencies of the hydroxyl (OH) radical from the water ice surface were measured in the range of 310-700 nm for the first time. Although isolated H$_2$O molecules and OH radicals do not absorb visible photons, the…

Chemical Physics · Physics 2024-06-06 Ni-En Sie , Masashi Tsuge , Yoichi Nakai , Naoki Watanabe

Context. Methane is among the main components of the ice mantles of insterstellar dust grains, where it is at the start of a rich solid-phase chemical network. Quantification of the photon-induced desorption yield of these frozen molecules…

The evaporation of water is ubiquitous in nature and industrial technologies. The known mechanism for evaporation is "thermal evaporation" which highlights the energy input for evaporation is via heat. Due to the weak absorption of water to…

Atomic and Molecular Clusters · Physics 2024-04-24 Yaodong Tu , Gang Chen

Ice mantles that formed on top of dust grains are photoprocessed by the secondary ultraviolet (UV) field in cold and dense molecular clouds. UV photons induce photochemistry and desorption of ice molecules. Experimental simulations…

Solar and Stellar Astrophysics · Physics 2015-10-20 R. Martín-Doménech , J. Manzano-Santamaría , G. M. Muñoz Caro , G. A. Cruz-Díaz , Y. -J. Chen , V. J. Herrero , I. Tanarro

This paper describes a near-UV/VIS study of a pyrene:H_2O interstellar ice analogue at 10 K using optical absorption spectroscopy. A new experimental approach makes it possible to irradiate the sample with vacuum ultraviolet (VUV) light…

Instrumentation and Methods for Astrophysics · Physics 2009-08-05 J. Bouwman , D. M. Paardekooper , H. M. Cuppen , H. Linnartz , L. J. Allamandola

The overabundance of gas molecules in the coldest regions of space point to a non-thermal desorption process. Laboratory simulations show an efficient desorption of CO ice exposed to ultraviolet radiation, known as photodesorption, which…

Instrumentation and Methods for Astrophysics · Physics 2022-09-20 N. -E. Sie , Y. -T. Cho , C. -H. Huang , G. M. Muñoz Caro , L. -C. Hsiao , H. -C. Lin , Y. -J. Chen

We made near infrared multicolor imaging observations of a disk around Herbig Be star HD100546 using Gemini/NICI. K (2.2\,$\mu$m), H$_2$O ice (3.06\,$\mu$m), and L'(3.8\,$\mu$m) disk images were obtained and we found the 3.1\,$\mu$m…

Earth and Planetary Astrophysics · Physics 2016-04-13 M. Honda , T. Kudo , S. Takatsuki , A. K. Inoue , T. Nakamoto , M. Fukagawa , M. Tamura , H. Terada , N. Takato

Water (H2O) ice is an important solid constituent of many astrophysical environments. To comprehend the role of such ices in the chemistry and evolution of dense molecular clouds and comets, it is necessary to understand the freeze-out,…

Solid-phase photo-processes involving icy dust grains greatly affect the chemical evolution of the interstellar medium by leading to the formation of complex organic molecules and by inducing photodesorption. So far, the focus of laboratory…

Ultraviolet irradiation of ice is of great interest for understanding the chemistry in both atmospheric and astrophysical environments. In interstellar space, photodissociation of H2O molecules can be a driving force behind the chemistry on…

Astrophysics · Physics 2016-08-30 Stefan Andersson , Geert-Jan Kroes , Ewine F. van Dishoeck

Molecular dynamics calculations have been performed to study the ultraviolet photodissociation of D2O in an amorphous D2O ice surface at 10-90 K, in order to investigate the influence of isotope effects on the photodesorption processes. As…

Chemical Physics · Physics 2011-05-06 C. Arasa , S. Andersson , H. M. Cuppen , E. F. van Dishoeck , G. J. Kroes