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Conventional methods for modeling thermocatalytic systems are typically based on the Kohn-Sham density functional theory (KS-DFT), neglecting the inhomogeneous distributions of gas molecules in the reactive environment. However, industrial…

Chemical Physics · Physics 2025-08-14 Jikai Sun , Jianzhong Wu

Soft lubricated contacts exhibit complex interfacial behaviours governed by the coupled effects of multiscale surface roughness and non-linear fluid-solid interactions. Accurately capturing this interplay across thin-film flows is…

Soft Condensed Matter · Physics 2025-11-12 Qian Wang , Suhaib Ardah , Tom Reddyhoff , Daniele Dini

A microfluidic device is constructed from PDMS with a single channel having a short section that is a thin flexible membrane, in order to investigate the complex fluid-structure interaction that arises between a flowing fluid and a…

Soft Condensed Matter · Physics 2020-07-03 Debadi Chakraborty , J. Ravi Prakash , Leslie Yeo , James Friend

Coupling between chemical fuel consumption and phase separation can lead to condensation at a nonequilibrium steady state, resulting in phase behaviors that are not described by equilibrium thermodynamics. Theoretical models of such…

Soft Condensed Matter · Physics 2025-05-23 Yongick Cho , William M. Jacobs

Frictional properties of interfaces with dynamic chemical bonds have been the subject of intensive experimental investigation and modeling, as it provides important insights into the molecular origin of the empirical rate and state laws,…

Mesoscale and Nanoscale Physics · Physics 2020-01-24 Wengen Ouyang , Yao Cheng , Ming Ma , Michael Urbakh

Dispersions of immiscible liquids, such as emulsions and polymer blends, are at the core of many industrial applications which makes the understanding of their properties (morphology, stability, etc.) of great interest. A wide range of…

Chemical Physics · Physics 2017-08-10 Anaïs Giustiniani , Wiebke Drenckhan , Christophe Poulard

A macroscopic theory for the molecular or Casimir interaction of dielectric materials with arbitrarily shaped surfaces is developed. The interaction is generated by the quantum and thermal fluctuations of the electromagnetic field which…

Statistical Mechanics · Physics 2009-11-10 Rauno Buescher , Thorsten Emig

Chemo-mechanical coupled systems have been a subject of interest for many decades now. Previous attempts to solve such models have mainly focused on elastic materials without taking into account the plastic deformation beyond yield, thus…

Computational Engineering, Finance, and Science · Computer Science 2020-01-15 Rupesh Kumar Mahendran , Hirshikesh , Ratna Kumar Annabattula , Sundararajan Natarajan

High velocity impact between crystalline surfaces is important for a range of material phenomena, yet a fundamental understanding of the effect of surface structure, energetics and kinetics on the underlying thermo-mechanical response…

Materials Science · Physics 2015-10-14 Zhenqi Yang , Sinan Muftu , Moneesh Upmanyu

The contribution to the free energy for a film of liquid of thickness $h$ on a solid surface, due to the interactions between the solid-liquid and liquid-gas interfaces is given by the binding potential, $g(h)$. The precise form of $g(h)$…

Soft Condensed Matter · Physics 2015-07-08 Adam P. Hughes , Uwe Thiele , Andrew J. Archer

The efficiency of soft particles to stabilize emulsions is examined by measuring their desorption free energy, i.e., the mechanical work required to detach the particle from a fluid interface. Here, we consider rubber-like elastic as well…

Soft Condensed Matter · Physics 2020-08-20 Hadi Mehrabian , Jacco H. Snoeijer , Jens Harting

Suspensions of Active Brownian Particles (ABP) undergo motility induced phase separation (MIPS) over a wide range of mean density and activity strength [1], even in the absence of an explicit attraction. Negative values of the mechanical…

Soft Condensed Matter · Physics 2022-02-07 Enrique Chacon , Francisco Alarcon , Jorge Ramirez , Pedro Tarazona , Chantal Valeriani

Elastic deformation of rigid materials with soft coatings (stratified materials) due to lubrication forces can also alter the interpretation of dynamic surface forces measurements and prevent contact formation between approaching surfaces.…

Soft Condensed Matter · Physics 2017-08-18 Yumo Wang , Matthew R. Tan , Joelle Frechette

Review of selected fundamental topics on the interaction between phase transformations, fracture, and other structural changes in inelastic materials is presented. It mostly focuses on the concepts developed in the author's group over last…

Materials Science · Physics 2021-08-24 Valery I. Levitas

Systems whose underlying classical dynamics are chaotic exhibit signatures of the chaos in their quantum mechanics. We investigate the possibility of using time-dependent density functional theory (TDDFT) to study the case when chaos is…

Other Condensed Matter · Physics 2009-11-13 Adam Wasserman , Neepa T. Maitra , Eric J. Heller

Using as a starting point conservation of momentum, a multiphase mechanical energy balance equation is derived that accounts for multiple material phases and interfaces present within a moving control volume. This balance is applied to a…

Fluid Dynamics · Physics 2022-12-26 Dalton J. E. Harvie

We use density functional theory (DFT) with the generalized gradient approximation (GGA) and our first-principles extrapolation method for accurate chemisorption energies {[Mason {\em et al.}, Phys. Rev. B {\bf 69}, 161401R (2004)]} to…

Materials Science · Physics 2007-05-23 Sara E. Mason , Ilya Grinberg , Andrew M. Rappe

Purely repulsive active particles spontaneously undergo motility-induced phase separation (MIPS) into condensed and dilute phases. Remarkably, the mechanical tension measured along the interface between these phases is negative. In…

Soft Condensed Matter · Physics 2018-10-31 Adam Patch , Daniel Sussman , David Yllanes , M. Cristina Marchetti

Bonding between polymeric interfaces is encountered widely in several industrial applications. Many of these bonding processes rely on time-consuming and temperature-dependent classical mechanism of polymer interdiffusion via reptation in a…

Soft Condensed Matter · Physics 2022-05-10 Nikhil Padhye , Ajay Vallabh

The formation, deformation, and break-up of liquid interfaces are ubiquitous phenomena in nature. In the present article we discuss the deformation of a liquid interface produced by optical radiation forces. Usually, the bending of such an…