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Methods for estimating the correlation energy of molecules and other electronic systems are discussed based on the assumption that the correlation energy can be partitioned between atomic regions. In one method, the electron density is…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

Quantum entanglement is a concept commonly used with reference to the existence of certain correlations in quantum systems that have no classical interpretation. It is a useful resource to enhance the mutual information of memory channels…

Quantum Physics · Physics 2009-11-13 Tina A. C. Maiolo , Fabio Della Sala , Luigi Martina , Giulio Soliani

Representing polyether-salt systems by chains of interacting coordination shells, defined by the cation and by its nearest ligands, we derive the interaction potential between closest shells -- the inter-shells potential -- in terms of…

chem-ph · Physics 2009-10-28 L. D. Carlos , A. L. L. Videira

A curious behavior of electron correlation energy is explored. Namely, the correlation energy is the energy that tends to drive the system toward that of the uniform electron gas. As such, the energy assumes its maximum value when a…

Materials Science · Physics 2019-12-17 Teepanis Chachiyo , Hathaithip Chachiyo

The mechanisms of electrostatic interactions between two charged dielectric spheres inside a polarizable medium have been investigated, in terms of hypothetical effective dipoles that depict how the positive and negative charge in each…

Soft Condensed Matter · Physics 2025-02-06 Yanyu Duan , Zecheng Gan , Ho-Kei Chan

In this work, we explore the statistical physics of colloidal particles that interact with electrolytes via ion-specific interactions. Firstly we study particles interact weakly with electrolyte using linear response theory. We find that…

Soft Condensed Matter · Physics 2016-10-12 Mingnan Ding , Yihao Liang , Xiangjun Xing

In this paper, an alternative method to range-separated linear-response time-dependent density-functional theory and perturbation theory is proposed to improve the estimation of the energies of a physical system from the energies of a…

Chemical Physics · Physics 2015-06-24 Elisa Rebolini , Julien Toulouse , Andrew M. Teale , Trygve Helgaker , Andreas Savin

In this work we present a model for the determination of the interaction energy for triplet and singlet states in atoms with incomplete filled shells. Our model includes the modification of the Coulomb's law by the interaction between the…

Strongly Correlated Electrons · Physics 2014-06-03 V. Dolocan , V. O. Dolocan

We make a comparison between the energy levels of the hydrogen atom, calculated by using standard methods, and that by using a modified Coulomb potential due to the interaction between the magnetic moments of the proton and electron. In…

Atomic Physics · Physics 2014-07-09 Voicu Dolocan

The author suggests an approach based on the separation of total energy of multielectron systems into the semi-classical Coulomb part and the non-classical additional part. This approach allows on the one hand to simplify calculations and…

Atomic Physics · Physics 2008-11-04 Vadim Kavera

Ionic liquids offer unique bulk and interfacial characteristics as battery electrolytes. Our continuum approach naturally describes the electrolyte on a macroscale. An integral formulation for the molecular repulsion,which can be…

Chemical Physics · Physics 2022-11-30 Max Schammer , Arnulf Latz , Birger Horstmann

We study the ionic equilibria and interactions of neutral semi-permeable spherical shells immersed in electrolyte solutions, including polyions. Although the shells are uncharged, only one type of ions of the electrolyte can permeate them,…

Soft Condensed Matter · Physics 2012-07-24 Vladimir Lobaskin , Artem N. Bogdanov , Olga I. Vinogradova

General expression for the thermodynamic potential of the model of semi-infinite jellium is obtained. By using this expression, the surface energy for infinite barrier model is calculated. The behavior of the surface energy and of chemical…

Statistical Mechanics · Physics 2015-09-30 P. P. Kostrobij , B. M. Markovych

We describe arrangements of ions capable of producing short-range attractive interactions between pairs of charged colloidal spheres in the low temperature strongly correlated limit. For particles of radius $R$ with bare charge $Z$ and…

Strongly Correlated Electrons · Physics 2007-05-23 Francisco J. Solis , Monica Olvera de la Cruz

We analyze a decomposition of the Coulomb electron-electron interaction into a long-range and a short-range part in the framework of density functional theory, deriving some scaling relations and the corresponding virial theorem. We study…

Chemical Physics · Physics 2015-06-26 Julien Toulouse , Paola Gori-Giorgi , Andreas Savin

From non-linear modification of Maxwell-Einstein theory, considered in (physics/9801031), follows modified Coulomb law for interaction between charged objects. Namely, if $(m, e)$ and $(m', e')$ are masses and charges of two objects, then…

General Physics · Physics 2007-05-23 Dmitriy Palatnik

Describing the Coulomb interactions between electrons in atomic or molecular systems is an important step to help us obtain accurate results for the different observables in the system. One convenient approach is to separate the dynamic…

Chemical Physics · Physics 2025-01-22 Claude Le Sech , Antonio Sarsa

We have calculated the electrostatic interaction between two rod-like charged objects with arbitrary orientations in three dimensions. we obtained a closed form formula expressing the interaction energy in terms of the separation distance…

Soft Condensed Matter · Physics 2015-05-27 M. Askari , J. Abouie

We calculate the short-range exchange-correlation energy of the uniform electron gas with two modified electron-electron interactions. While the short-range exchange functionals are calculated analytically, Coupled-Cluster and…

Materials Science · Physics 2016-08-16 Julien Toulouse , Andreas Savin , Heinz-Jürgen Flad

We have calculated the total energy of the helium atom in higher excited state. The Coulomb and exchange integrals are evaluated via spherical harmonics. The interaction of the magnetic moments of the electrons between them and also with…

Atomic Physics · Physics 2014-06-03 Voicu Dolocan