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We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

The advent of visible-infrared laser pulses carrying a substantial fraction of their energy in a single field oscillation cycle has opened a new era in the experimental investigation of ultrafast processes in semiconductors and dielectrics…

Quantum Physics · Physics 2018-05-09 Stanislav Yu. Kruchinin , Ferenc Krausz , Vladislav S. Yakovlev

Phase-of-the-phase spectroscopy using two-color colinearly polarized laser pulses has been introduced and experimentally applied to strong-field tunneling ionization in S. Skruszewicz et al., Phys. Rev. Lett. 115, 043001 (2015) and recently…

Atomic Physics · Physics 2018-12-05 V. Tulsky , M. A. Almajid , D. Bauer

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

In few-cycle pulses, the exact value of the carrier-envelope phase difference (CEPD) has a pronounced influence on the ionization dynamics of atoms and molecules. We show that for atoms in circularly polarized light, a change in the CEPD is…

Atomic Physics · Physics 2009-11-13 Christian Per Juul Martiny , Lars Bojer Madsen

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

Permanent electric dipole moments (EDMs) of fundamental particles such as the electron are signatures of parity and time-reversal violation due to physics beyond the standard model. EDM measurements probe new physics at energy scales well…

Atomic Physics · Physics 2020-10-09 Mohit Verma , Andrew M. Jayich , Amar C. Vutha

Quantum calculations of tunneling in strong-field ionization (SFI) predict intricate momentum distributions due to sub-laser-cycle attosecond electron dynamics. These are obscured in most experiments by the dominance of inter-cycle…

Atomic Physics · Physics 2021-06-03 Nicholas Werby , Adi Natan , Ruaridh Forbes , Philip Bucksbaum

We describe the results of experiments and simulations performed with the aim of extending photoelectron spectroscopy with intense laser pulses to the case of molecular compounds. Dimer frame photoelectron angular distributions generated by…

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

We consider atomic strong-field ionization in the long-pulse limit for linearly polarized infrared laser fields. We show how nondipole effects in the plane formed by the propagation and polarization directions lead to (i) a shift of the…

Atomic Physics · Physics 2021-11-10 Mads Middelhede Lund , Lars Bojer Madsen

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

Chemical Physics · Physics 2016-03-03 Bo Y. Chang , Ignacio R. Sola , Seokmin Shin

Orbit-based methods are widespread in strong-field laser-matter interaction. They provide a framework in which photoelectron momentum distributions can be interpreted as the quantum interference between different semi-classical pathways the…

Atomic Physics · Physics 2024-10-03 T. Rook , D. Habibović , C. Figueira de Morisson Faria

We investigate the ionization dynamics of atoms irradiated by an intense laser field using a semiclassical model that includes magnetic Lorentz force in the rescattering process. We find that, the electrons tunneled with different initial…

Atomic Physics · Physics 2017-01-25 J. F. Tao , Q. Z. Xia , J. Cai , L. B. Fu , J. Liu

The electron nondipole dynamics in tunneling ionization in an elliptically polarized laser field is investigated theoretically using a relativistic Coulomb-corrected strong-field approximation (SFA) based on the eikonal approximation of the…

Atomic Physics · Physics 2022-07-07 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…

We report the breakdown of the electric dipole approximation in the long-wavelength limit in strong-field ionization with linearly polarized few-cycle mid-infrared laser pulses at intensities on the order of 10$^{13}$ W/cm$^2$.…

Atomic Physics · Physics 2014-12-16 A. Ludwig , J. Maurer , B. W. Mayer , C. R. Phillips , L. Gallmann , U. Keller

A particle, which moves in a crystal, experiences weak interactions with electrons and nuclei alongside with electromagnetic interaction. Measuring the polarization vector and the angular distribution of charged and neutral particles…

High Energy Physics - Phenomenology · Physics 2019-05-17 V. G. Baryshevsky

High-energy spin-polarized electron, positron, and $\gamma$-photon beams have many significant applications in the study of material properties, nuclear structure, particle physics, and high-energy astrophysics. Thus,efficient production of…

Plasma Physics · Physics 2022-05-09 Ting Sun , Qian Zhao , Kun Xue , Zhi-Wei Lu , Liang-Liang Ji , Feng Wan , Yu Wang , Yousef I. Salamin , Jian-Xing Li