Related papers: Controlling quantum interference between virtual a…
Interference between multiple distinct paths is a defining property of quantum physics, where "paths" may involve actual physical trajectories, as in interferometry, or transitions between different internal (e.g. spin) states, or both. A…
Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
Photo-induced phase transitions (PIPTs) provide an ultrafast, energy-efficient way for precisely manipulating the topological properties of transition-metal ditellurides, and can be used to stabilize a topological phase in an otherwise…
The optical spectrum of a quantum system is jointly determined by the properties of the emitter and the driving field. All-optical spectral control can hence be a promising method to engineer the properties of single photon emitters for…
Two-photon excited fluorescence (TPEF) microscopy and fluorescence lifetime imaging (FLIM) are powerful imaging techniques in bio-molecular science. The need for elaborate light sources for TPEF and speed limitations for FLIM, however,…
Single photons constitute a main platform in quantum science and technology: they carry quantum information over extended distances in the future quantum internet and can be manipulated in advanced photonic circuits enabling scalable…
In order to study consequences of the differences between the ionic-to-neutral and neutral-to-ionic transitions in the one-dimensional extended Peierls-Hubbard model with alternating potentials for the TTF-CA complex, we introduce a double…
We demonstrate fluorescence generation through a sequential multiphoton process with real intermediary states. Our findings suggest new directions for optical control of previously unexplored molecular excitation pathways.
The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…
Efficient coupling between light and bulk plasmons (BPs) remains a central challenge because of their inherent mode mismatch, limited penetration depth, and pronounced resonant energy mismatch between visible-range photons and BPs. In this…
Polymorphic transitions in layered transition metal dichalcogenides provide an excellent platform for discovering exotic phenomena associated with metastable states, ranging from topological phase transitions to enhanced superconductivity.…
Cathodoluminescence spectroscopy has recently emerged as a novel platform for nanoscale control of nonclassical features of light. Here, we propose a theoretical model for cathodoluminescence from a multi-level quantum emitter. Employing a…
The interference of two independent single-photon pulses impinging on a beam splitter is analysed in a generalised time-resolved manner. Different aspects of the phenomenon are elaborated using different representations of the single-photon…
Accurately controlling the quantum coherence of photons is pivotal for their applications in quantum sensing and quantum imaging. Here, we propose the utilization of quantum entanglement and local phase manipulation techniques to control…
Here we proposed the valley selective excitations via a two-color (\ensuremath{\omega} + \ensuremath{2\omega}) laser field, made by superimposing two linearly polarized pulses at frequencies \ensuremath{\omega} and \ensuremath{2\omega}. We…
Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and the quantum internet on the horizon. Extensive research has been carried out to determine suitable quantum emitters and…
Entangled two-photon absorption (ETPA) could form the basis of nonlinear quantum spectroscopy at very low photon fluxes, since, at sufficiently low photon fluxes, ETPA scales linearly with the photon flux. When different pairs start to…
Ultraintense pulses from X-ray free-electron lasers can drive, within femtoseconds, multiple processes in the inner shells of atoms and molecules in all phases of matter. The ensuing complex ionization pathways of outer-shell electrons from…
We study phonon-assisted dephasing in optically excited semiconductor quantum dots within the frameworks of the independent Boson model and optimal control. Using a realistic description for the quantum dot states and the phonon coupling,…
We study theoretically the properties of a two-level quantum dipole emitter near an ultrathin transdimensional plasmonic film. Our model system mimics a solid-state single-photon source device. Using realistic experimental parameters, we…