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Spin resonance of single spin centers bears great potential for chemical structure analysis, quantum sensing and quantum coherent manipulation. Essential for these experiments is the presence of a two-level spin system whose energy…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Philip Willke , Aparajita Singha , Xue Zhang , Taner Esat , Christopher P. Lutz , Andreas J. Heinrich , Taeyoung Choi

Coherent control of individual atomic and molecular spins on surfaces has recently been demonstrated by using electron spin resonance (ESR) in a scanning tunneling microscope (STM). Here we present a combined experimental and modeling study…

Historically, electron spin resonance (ESR) has provided excellent insight into the electronic, magnetic, and chemical structure of samples hosting spin centers. In particular, the hyperfine interaction between the electron and the nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-11-23 Laëtitia Farinacci , Lukas M. Veldman , Philip Willke , Sander Otte

Electron-spin resonance carried out with scanning tunneling microscopes (ESR-STM) is a recently developed experimental technique that is attracting enormous interest on account of its potential to carry out single-spin on-surface resonance…

Mesoscale and Nanoscale Physics · Physics 2023-04-19 Santiago A. Rodríguez , Sergio S. Gómez , Joaquín Fernández-Rossier , Alejandro Ferrón

Electron spin resonance (ESR) spectroscopy in scanning tunneling microscopy (STM) has enabled probing the electronic structure of single magnetic atoms and molecules on surfaces with unprecedented energy resolution, as well as demonstrating…

The integration of scanning tunneling microscopy (STM) and electron spin resonance (ESR) spectroscopy has emerged as a powerful and innovative tool for discerning spin excitations and spin-spin interactions within atoms and molecules…

Mesoscale and Nanoscale Physics · Physics 2024-11-04 Lyuzhou Ye , Xiao Zheng , Xin Xu

Electron paramagnetic resonance (EPR) performed with a scanning tunneling microscope (STM) allows for probing the spin excitation of single atomic species with MHz energy resolution. One of the basic applications of conventional EPR is the…

Mesoscale and Nanoscale Physics · Physics 2021-11-10 Tom S. Seifert , Stepan Kovarik , Pietro Gambardella , Sebastian Stepanow

Hyperfine interactions between electron and nuclear spins have been widely used in material science, organic chemistry, and structural biology as a sensitive probe to the local chemical environment through spatial identification of nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Jinkyung Kim , Kyungju Noh , Yi Chen , Fabio Donati , Andreas J. Heinrich , Christoph Wolf , Yujeong Bae

The development of electron spin resonance (ESR) combined with scanning tunneling spectroscopy (STM) is undoubtedly one of the main experimental breakthroughs in surface science of the last decade thanks to joining the extraordinarily high…

Strongly Correlated Electrons · Physics 2022-08-31 Fernando Delgado , Nicolás Lorente

Electrically detected electron spin resonance (ESR) is used to study the hyperfine interaction of the two-dimensional electrons and the nuclei of the host lattice in a GaAs/AlGaAs heterostructure. Under the microwave and radio- frequency…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Chris Hillman , H. W. Jiang

In the last decade, detecting spin dynamics at the atomic scale has been enabled by combining techniques like electron spin resonance (ESR) or pump-probe spectroscopy with scanning tunneling microscopy (STM). Here, we demonstrate an…

We report the development of a continuous-wave and pulsed X-band electron spin resonance (ESR) spectrometer for the study of spins on ordered surfaces down to cryogenic temperatures. The spectrometer operates in ultra-high vacuum and…

Coherent spin resonance methods such as nuclear magnetic resonance (NMR) and electron spin resonance (ESR) spectroscopy have led to spectrally highly sensitive, non-invasive quantum imaging techniques with groundbreaking applications in…

Magnetic resonance imaging (MRI) revolutionized diagnostic medicine and biomedical research by allowing a noninvasive access to spin ensembles. To enhance MRI resolution to the nanometer scale, new approaches including scanning probe…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 Philip Willke , Kai Yang , Yujeong Bae , Andreas J. Heinrich , Christopher P. Lutz

The pathway toward the tailored synthesis of materials starts with precise characterization of the conformational properties and dynamics of individual molecules. Electron spin resonance based scanning tunneling microscopy can potentially…

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a…

Instrumentation and Detectors · Physics 2019-01-30 Fabian D. Natterer , François Patthey , Tobias Bilgeri , Patrick R. Forrester , Nicolas Weiss , Harald Brune

We propose a new universal mechanism that makes it possible to drive an individual atomic spin using a spin polarized scanning tunnel microscope (STM) with an oscillating electric signal. We show that the combination of the distance…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 J. L. Lado , A. Ferron , J. Fernandez-Rossier

We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunnelling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 Alejandro Ferrón , Santiago A. Rodríguez , Sergio S. Gómez , Jose L. Lado , Joaquín Fernández-Rossier

Electric control of spins has been a longstanding goal in the field of solid state physics due to the potential for increased efficiency in information processing. This efficiency can be optimized by transferring spintronics to the atomic…

Mesoscale and Nanoscale Physics · Physics 2023-11-30 Piotr Kot , Maneesha Ismail , Robert Drost , Janis Siebrecht , Haonan Huang , Christian R. Ast

Integration of electron spin resonance (ESR) in a scanning tunneling microscope (STM) has enabled an all-electrical control of atomic and molecular spins on solid surfaces with atomic-scale precision and energy resolution beyond thermal…

Mesoscale and Nanoscale Physics · Physics 2025-09-03 Deung-Jang Choi , Soo-hyon Phark , Andreas J. Heinrich , Nicolás Lorente
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