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Self-assembly, the process by which interacting components form well-defined and often intricate structures, is typically thought of as a spontaneous process arising from equilibrium dynamics. When a system is driven by external…

Statistical Mechanics · Physics 2021-11-12 Shriram Chennakesavalu , Grant M. Rotskoff

We investigate two-dimensional crystal assemblies formed by a binary mixture of colloidal particles with a size ratio of 0.88 and driven by short-ranged depletion interactions. Our experiments show that the orientational order of the…

Soft Condensed Matter · Physics 2025-08-18 S. k. Tahmid Shahriar , Chris Feltman , Sean Machler , Nabila Tanjeem

We explore the use of templated self-assembly to facilitate the formation of complex target structures made from patchy particles. First, we consider the templating of high-symmetry shell structures around a spherical core particle. We find…

Soft Condensed Matter · Physics 2013-06-25 Alexander J. Williamson , Alex W. Wilber , Jonathan P. K. Doye , Ard A. Louis

Despite intense research, methods for controlling soft matter's spontaneous self-assembly in-to well-defined layers remain a significant challenge. We observed ion-induced structural disconti-nuities of phospholipid vesicles that can be…

Soft Condensed Matter · Physics 2024-04-01 Judith U. De Mel , Sudipta Gupta , Gerald J. Schneider

Understanding protein self-assembly is important for many biological and industrial processes. Proteins can self-assemble into crystals, filaments, gels, and other amorphous aggregates. The final forms include virus capsids and condensed…

Soft Condensed Matter · Physics 2016-04-15 Jennifer J. McManus , Patrick Charbonneau , Emanuela Zaccarelli , Neer Asherie

Molecular building blocks interacting at the nanoscale organize spontaneously into stable mono- layers that display intriguing long-range ordering motifs on the surface of atomic substrates. The patterning process, if appropriately…

Mesoscale and Nanoscale Physics · Physics 2011-02-18 Marta Balbás Gambra , Carsten Rohr , Kathrin Gruber , Bianca Hermann , Thomas Franosch

The fabrication of versatile building blocks that are reliably self-assemble into desired ordered and disordered phases is amongst the hottest topics in contemporary material science. To this end, microscopic units of varying complexity,…

Soft Condensed Matter · Physics 2016-03-23 Lorenzo Rovigatti , Barbara Capone , Christos N. Likos

Manipulating the way in which colloidal particles self-organise is a central challenge in the design of functional soft materials. Meeting this challenge requires the use of building blocks that interact with one another in a highly…

Soft Condensed Matter · Physics 2021-03-30 Joe G Donaldson , Peter Schall , Laura Rossi

Cyanobacteria sequester photosynthetic enzymes into microcompartments which facilitate the conversion of carbon dioxide into sugars. Geometric similarities between these structures and self-assembling viral capsids have inspired models that…

Soft Condensed Matter · Physics 2018-07-10 Grant M. Rotskoff , Phillip L. Geissler

Active matter physics and swarm robotics have provided powerful tools for the study and control of ensembles driven by internal sources. At the macroscale, controlling swarms typically utilizes significant memory, processing power, and…

Algorithmic self-assembly, a generalization of crystal growth processes, has been proposed as a mechanism for autonomous DNA computation and for bottom-up fabrication of complex nanostructures. A `program' for growing a desired structure…

Materials Science · Physics 2010-01-08 Rebecca Schulman , Erik Winfree

The relationship between interactions, flexibility and disorder in proteins has been explored from many angles: folding upon binding, flexibility of the core relative to the periphery, entropy changes, etc. In this work, we provide…

Soft Condensed Matter · Physics 2022-11-21 Beatriz Seoane , Alessandra Carbone

Aggregation is a common behavior by which groups of organisms arrange into cohesive groups. Whether suspended in the air (like honey bee clusters), built on the ground (such as army ant bridges), or immersed in water (such as sludge worm…

Populations and Evolution · Quantitative Biology 2022-06-23 O. Shishkov , O. Peleg

Structural quantities such as order parameters and correlation functions are often employed to gain insight into the physical behavior and properties of condensed matter systems. While standard quantities for characterizing structure exist,…

Soft Condensed Matter · Physics 2017-08-23 Aaron S. Keys , Christopher R. Iacovella , Sharon C. Glotzer

The Self-Assembly of Nano-Objects (SANO) code we implemented demonstrates the ability to predict the molecular self-assembly of different structural motifs by tuning the molecular building blocks as well as the metallic substrate. It…

Computational Physics · Physics 2012-11-26 Thomas Roussel , Lourdes F. Vega

Monolayers of soft colloidal particles confined at fluid interfaces have been attracting increasing interest for fundamental studies and applications alike. However, establishing the relation between their internal architecture, which is…

Soft Condensed Matter · Physics 2021-03-30 Jacopo Vialetto , Fabrizio Camerin , Fabio Grillo , Lorenzo Rovigatti , Emanuela Zaccarelli , Lucio Isa

In this review we discuss recent advances in the self-assembly of self-propelled colloidal particles and highlight some of the most exciting results in this field with a specific focus on dry active matter. We explore this phenomenology…

Soft Condensed Matter · Physics 2021-02-24 S. A. Mallory , C. Valeriani , A. Cacciuto

Controlled micro- to meso-scale porosity is a common materials design goal with possible applications ranging from molecular gas adsorption to particle size selective permeability or solubility. Here, we use inverse methods of statistical…

Soft Condensed Matter · Physics 2016-03-11 Beth A. Lindquist , Ryan B. Jadrich , Thomas M. Truskett

In geometrically frustrated assemblies, equilibrium self-limitation manifests in the form of a minimum in the free energy per subunit at a finite, multi-subunit size which results from the competition between the elastic costs of…

Soft Condensed Matter · Physics 2023-08-15 Michael Wang , Gregory Grason

Mesoscopic molecular dynamics simulations are used to determine the large scale structure of several binary polymer mixtures of various chemical architecture, concentration, and thermodynamic conditions. By implementing an analytical…

Soft Condensed Matter · Physics 2010-04-05 J. McCarty , I. Y. Lyubimov , M. G. Guenza