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This study investigates the ultrafast dynamics of coherent phonons and phonon-polaritons in lithium niobate (LiNbO$_{3}$) crystals using reflective pump-probe spectroscopy with 25-fs time resolution. In addition to several coherent optical…

Materials Science · Physics 2022-08-23 Aizitiaili Abulikemu , Takumi Fukuda , Muneaki Hase

Lead halide perovskite semiconductors are soft, polar, materials. The strong driving force for polaron formation (the dielectric electron-phonon coupling) is balanced by the light band effective-masses, leading to a strongly-interacting…

Materials Science · Physics 2017-11-15 Jarvist Moore Frost

The discovery of localized plasmon polariton resonances has been pivotal in enabling tunability of the optical resonance. Recently, extensive research efforts have aimed to expand these achievements to other polaritonic states that exhibit…

The long carrier lifetime and defect tolerance in metal halide perovskites (MHPs) are major contributors to the superb performance of MHP optoelectronic devices. Large polarons were reported to be responsible for the long carrier lifetime.…

The low-frequency collective excitations, which often occur in the terahertz or multi-terahertz spectral region, play an essential role in many novel emergent phenomena. Despite numerous studies in the bulk, detection of such excitations at…

Materials Science · Physics 2022-08-01 Jiaming Le , Yudan Su , Junying Ma , Long Cheng , Yuen Ron Shen , Xiaofang Zhai , Chuanshan Tian

Using time resolved ultrafast spectroscopy, we have demonstrated that the far infrared (FIR) excitations in ferroelectric crystals may be modified through an arsenal of control techniques from the fields of guided waves, geometrical and…

The advent of monochromated electron energy-loss spectroscopy has enabled atomic-resolution vibrational spectroscopy, which triggered interest in spatially localized or quasi-localized vibrational modes in materials. Here we report the…

Materials Science · Physics 2023-10-13 De-Liang Bao , Mingquan Xu , Ao-Wen Li , Gang Su , Wu Zhou , Sokrates T. Pantelides

This review will deal with several types of free charge localisation in oxides and their consequences on the effective dielectric spectra of such materials. The first one is the polaronic localisation at the unit cell scale on residual…

Materials Science · Physics 2010-06-21 Mario Maglione

Mid-infrared nanophotonics can be realized using sub-diffractional light localization and field enhancement with surface phonon polaritons in polar dielectric materials. We experimentally demonstrate second harmonic generation due to the…

The monolayer of black phosphorous, or phosphorene, has recently emerged as a new 2D semiconductor with intriguing highly anisotropic transport properties. Existing calculations of its intrinsic phonon-limited electronic transport…

Materials Science · Physics 2015-06-24 Bolin Liao , Jiawei Zhou , Bo Qiu , Mildred S. Dresselhaus , Gang Chen

Phonon polaritons in van der Waals crystals offer mid-infrared light confinement deep below the diffraction limit, making them promising for nanophotonics applications. However, the practical use of phonon polaritons remains limited, in…

Polaritons in 2D and van der Waals (vdW) materials have been investigated in several recent works as an innovative platform for light-matter interaction, rich of new physical phenomena.Hexagonal Boron Nitride (h-BN), in particular, is an…

At the 2D limit, hexagonal systems such as monolayer transition metal dichalcogenides (TMDs) and graphene exhibit unique coupled spin and momentum-valley physics (valley pseudospin) owing to broken spatial inversion symmetry and strong…

Materials Science · Physics 2023-06-21 Tristan L Britt , Bradley J. Siwick

Hybrid lattice-light modes, known as phonon-polaritons, represent the backbone of advanced protocols based on THz pumping of infrared modes. Here we provide a theoretical framework able to capture the different roles played by…

Materials Science · Physics 2025-05-02 Niccolò Sellati , Jacopo Fiore , Stefano Paolo Villani , Lara Benfatto , Mattia Udina

The coherence of polaritons plays a fundamental role in numerous recent experimental observations, from strong coupling to Bose-Einstein condensation, but accessing the coherence of polaritons is a difficult task due to the high energy of…

Recently studied hyperbolic materials host unique phonon-polariton (PP) modes. The ultra-short wavelengths of these modes, which can be much smaller than those of conventional exciton-polaritons, are of high interest for extreme…

Mesoscale and Nanoscale Physics · Physics 2015-08-26 Andrea Tomadin , Alessandro Principi , Justin C. W. Song , Leonid S. Levitov , Marco Polini

We report on the exciton formation and relaxation dynamics following photocarrier injection in a single-layer two-dimensional lead-iodide perovskite. We probe the time evolution of four distinct exciton resonances by means of time-resolved…

Surface phonon polaritons (SPhPs) in polar dielectrics offer new opportunities for infrared nanophotonics due to sub-diffraction confinement with low optical losses. Though the polaritonic field confinement can be significantly improved by…

Semi-metallic graphene and semiconducting monolayer transition metal dichalcogenides (TMDCs) are the two-dimensional (2D) materials most intensively studied in recent years. Recently, black phosphorus emerged as a promising new 2D material…

Mesoscale and Nanoscale Physics · Physics 2014-11-07 Xiaomu Wang , Aaron M. Jones , Kyle L. Seyler , Vy Tran , Yichen Jia , Huan Zhao , Han Wang , Li Yang , Xiaodong Xu , Fengnian Xia

Phonon polaritons enable waveguiding and localization of infrared light with extreme confinement and low losses. The spatial propagation and spectral resonances of such polaritons are usually probed with complementary techniques such as…