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We use second and third harmonic generation microscopy to investigate the nonlinear optical response of GaAs nanocavities embedded in a gold film and compare them to bare GaAs nanocavities. Our results reveal that the surrounding metallic…

In whispering gallery mode (WGM) resonators light is guided by continuous total internal reflection along a curved surface. Fabricating such resonators from an optically nonlinear material one takes advantage of their exceptionally high…

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

We report on nonlinear frequency conversion from the telecom range via second harmonic generation (SHG) and third harmonic generation (THG) in suspended gallium nitride slab photonic crystal (PhC) cavities on silicon, under continuous-wave…

The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar…

To date, second-harmonic generation (SHG) at nanoscale has been concentrated on employing high-refractive-index nanostructures, owing to the strong field confinement at deep subwavelength scales based on optically resonant effects. However,…

Directional harmonic generation is an important property characterizing the ability of nonlinear optical antennas to diffuse the signal in well-defined region of space. Herein, we show how sub-wavelength facets of an organic molecular…

Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…

Optics · Physics 2020-01-10 Xuexue Guo , Xingjie Ni

Second-harmonic generation (SHG) is a well-known nonlinear spectroscopy method to probe electronic structure, specifically, in transition metal dichalcogenide (TMDC) monolayers. This work investigates the nonlinear dynamics of a strongly…

In recent years resonant semiconductor and all-dielectric nanophotonics offered a lot of possibilities for thermally-induced light manipulation at the nanoscale. Owing to high-quality resonant states, such nanostructures allow for efficient…

Optics · Physics 2022-04-13 Olesiya Pashina , Kristina Frizyuk , George Zograf , Mihail Petrov

Second-order nonlinear optical responses, including photogalvanic effect (PGE) and second harmonic generation (SHG), are important physical phenomena in nonlinear optics. The PGE (SHG) related to linearly and circularly polarized light are…

Mesoscale and Nanoscale Physics · Physics 2023-06-01 Yuan Liu , Zhen-Gang Zhu , Gang Su

Transition metal dichalcogenides (TMDCs) have demonstrated significant potential as versatile quantum materials for light absorption and emission. Their unique properties are primarily governed by exciton-photon interactions, which can be…

We report the simultaneous generation of second-harmonic generation (SHG) and Brillouin microlaser in a high-quality thin-film lithium niobate (TFLN) microdisk resonator. The microdisk is fabricated with ultrahigh-Q factor of 4X10(6) by…

The ability to engineer nonlinear optical processes in all-dielectric nanostructures is both of fundamental interest and highly desirable for high-performance, robust, and miniaturized nonlinear optical devices. Herein, we propose a novel…

Optics · Physics 2021-11-25 Tingting Liu , Xinyuan Fang , Shuyuan Xiao

Metallic nanostructures exhibit strong nonlinear-optical response at surface plasmon resonances, where the light-matter coupling efficiency is enhanced. An active modulation of this response can be realized by means of an external magnetic…

Mesoscale and Nanoscale Physics · Physics 2020-05-29 Ilya Razdolski , Gaspar Armelles , Alfonso Cebollada , Andrey Kirilyuk

As the rapid development of nonlinear optics, the enhancement of optical third harmonic generation becomes a pop research realm in the fields of physics, chemistry, biology, materials science, information science and other fields. In this…

Optics · Physics 2017-11-28 Wenbo Zang , Lingling Fan , Xin Yang , Mingyu Ma , Peng Zhan , Zhuo Chen , Zhenlin Wang

The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

Thin-film lithium niobate (TFLN) enables extremely high-efficiency second-order nonlinear optical effects due to large nonlinear coefficient d33 and strong optical field localization. Here, we first designed and fabricated a…

Optics · Physics 2023-12-13 Xiao Wu , Zhenzhong Hao , Li Zhang , Di Jia , Rui Ma , Fang Bo , Feng Gao , Guoquan Zhang , Jingjun Xu

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…