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We show here that the Hamiltonian for an electronic system may be written exactly in terms of fluctuation operators that transition constituent fragments between internally correlated states, accounting rigorously for inter-fragment…

Chemical Physics · Physics 2019-05-24 Anthony D. Dutoi , Yuhong Liu

We derive electronic tight-binding Hamiltonians for strained graphene, hexagonal boron nitride and transition metal dichalcogenides based on Wannier transformation of {\it ab initio} density functional theory calculations. Our microscopic…

Mesoscale and Nanoscale Physics · Physics 2018-08-14 Shiang Fang , Stephen Carr , Miguel A. Cazalilla , Efthimios Kaxiras

We demonstrate how electric fields with arbitrary time profile can be used to control the time-dependent parameters of spin and orbital exchange Hamiltonians. Analytic expressions for the exchange constants are derived from a time-dependent…

Strongly Correlated Electrons · Physics 2017-03-10 Martin Eckstein , Johan H. Mentink , Philipp Werner

We consider an implementation of the adiabatic spin dynamics approach in a tight-binding description of the electronic structure. The adiabatic approximation for spin-degrees of freedom assumes that the faster electronic degrees of freedom…

The correct interpretation of magnetic properties in the weak-exchange regime has remained a challenging task for several decades. In this regime, the effective exchange interaction between local spins is quite weak, of the same order of…

Chemical Physics · Physics 2024-01-10 Dumitru-Claudiu Sergentu , Boris Le Guennic , Rémi Maurice

We present a technique to map an electronic model with local interactions (a generalized multi-orbital Hubbard model) onto an effective model of interacting classical spins, by requiring that the thermodynamic potentials associated to spin…

Strongly Correlated Electrons · Physics 2015-05-27 Andrea Secchi , Alexander I. Lichtenstein , Mikhail I. Katsnelson

We formulate a low-energy theory for the magnetic interactions between electrons in the multi-band Hubbard model under non-equilibrium conditions determined by an external time-dependent electric field which simulates laser-induced spin…

Strongly Correlated Electrons · Physics 2013-04-11 Andrea Secchi , Sergei Brener , Alexander I. Lichtenstein , Mikhail I. Katsnelson

A generalised extraction procedure for magnetic interactions using effective Hamiltonians is presented that is applicable to systems with more than two sites featuring local spins $S_i \geq 1$. To this end, closed, non-recursive expressions…

Chemical Physics · Physics 2025-06-03 Arta A. Safari , Nikolay A. Bogdanov

We developed a method which performs the coupled adiabatic spin and lattice dynamics based on the tight-binding electronic structure model, where the intrinsic magnetic field and ionic forces are calculated from the converged…

A spin Hamiltonian, which characterizes interatomic interactions between spin moments, is highly valuable in predicting and comprehending the magnetic properties of materials. A deeper understanding of the microscopic origin of magnetic…

We present a computational method to determine the exchange constants in isotropic spin models. The method uses the Hamiltonian and overlap matrices computed from density functional schemes that are based on nonorthogonal basis sets. We…

Mesoscale and Nanoscale Physics · Physics 2019-06-19 László Oroszlány , Jaime Ferrer , András Deák , László Udvardi , László Szunyogh

We investigate the problem of determining the Hamiltonian of a locally interacting open-quantum system. To do so, we construct model estimators based on inverting a set of stationary, or dynamical, Heisenberg-Langevin equations of motion…

Quantum Physics · Physics 2020-08-19 Eugene F. Dumitrescu , Pavel Lougovski

We investigate the role of exchange bridges in molecular magnets. We explore their effects on the distribution of the valence electrons and their contribution to the exchange processes. The present study is focused on a spin-half dimer with…

Atomic and Molecular Clusters · Physics 2020-10-12 M. Georgiev , H. Chamati

We propose a framework for the connection between local symmetries of discrete Hamiltonians and the design of compact localized states. Such compact localized states are used for the creation of tunable, local symmetry-induced bound states…

Quantum Physics · Physics 2018-02-09 M. Röntgen , C. V. Morfonios , P. Schmelcher

One-dimensional multi-component Fermi or Bose systems with strong zero-range interactions can be described in terms of local exchange coefficients and mapping the problem into a spin model is thus possible. For arbitrary external confining…

We present a way of partly reincorporate the effects of the localized bonding electrons on the dynamics of their itinerant counterparts in Hubbard-like Hamiltonians. This is done by relaxing the constraint that the former should be entirely…

Strongly Correlated Electrons · Physics 2020-09-23 T. V. Trevisan , Gustavo M. Monteiro , A. O. Caldeira

We discuss the spin excitations in systems with hopping electron conduction and strong position disorder. We focus on the problem in a strong magnetic field when the spin Hamiltonian can be reduced to the effective single-particle…

Disordered Systems and Neural Networks · Physics 2016-08-24 A. V. Shumilin

A local transformation from fermionic operators to spin matrices is proposed and studied in this work. For this purpose, a system of fermions on a lattice is considered and one applies the scheme to replace the fermionic variables with spin…

High Energy Physics - Lattice · Physics 2022-06-22 Adam Wyrzykowski

An investigation on the properties of electronic states of a tight-binding Hamiltonian on the Apollonian network is presented. This structure, which is defined based on the Apollonian packing problem, has been explored both as a complex…

Disordered Systems and Neural Networks · Physics 2009-11-13 Ariston L. Cardoso , Roberto F. S. Andrade , André M. C. Souza

We prove that estimating the ground state energy of a translationally-invariant, nearest-neighbour Hamiltonian on a 1D spin chain is QMAEXP-complete, even for systems of low local dimension (roughly 40). This is an improvement over the best…

Quantum Physics · Physics 2017-11-15 Johannes Bausch , Toby Cubitt , Maris Ozols
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