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Frequency-modulated (FM) combs feature flat intensity spectra with a linear frequency chirp, useful for metrology and sensing applications. Generating FM combs in semiconductor lasers generally requires a fast saturable gain, usually…

The advancement of technologies for the precise interrogation of molecules offers exciting possibilities for new studies in the realms of precision spectroscopy and quantum technologies. Experiments in these domains often address molecular…

Optics · Physics 2022-09-15 Mudit Sinhal , Anatoly Johnson , Stefan Willitsch

One salient characteristic of Quantum Cascade Laser (QCL) is its very shor gain recovery time that so far thwarted the attempts to achieve self-mode locking of the device into a train of single pulses. We show theoretically that four wave…

Optics · Physics 2014-03-21 Jacob Khurgin , Yamac Dikmelik , Andreas Hugi , Jerome Faist

Due to its fast and high resolution characteristics, dual-comb spectroscopy has attracted an increasing amount of interest since its first demonstration. In the terahertz frequency range where abundant absorption lines (finger prints) of…

We demonstrate simple optical frequency combs based on semiconductor quantum well laser diodes. The frequency comb spectrum can be tailored by choice of material properties and quantum-well widths, providing spectral flexibility. Finally,…

Optics · Physics 2020-07-21 Mark Dong , Matthew W. Day , Herbert G. Winful , Steven T. Cundiff

Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multi-heterodyne…

The recent demonstration of a terahertz (THz) molecular gas laser pumped by a mid-infrared quantum cascade laser (QCL) has opened up new perspectives for this family of sources, traditionally relying on CO2-laser pumping. A so far open…

The frequency noise power spectral density of a free-running quantum cascade laser frequency comb is investigated. A plateau is observed at high frequencies, attributed to the quantum noise limit set by the Schawlow-Townes formula for the…

Optics · Physics 2015-11-18 Francesco Cappelli , Gustavo Villares , Sabine Riedi , Jerome Faist

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch

Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

Harmonic frequency combs, in which the lasing modes are separated by a period of tens of free spectral ranges from each other, have been recently discovered in quantum cascade lasers (QCLs). There is an ongoing debate how the harmonic combs…

Optics · Physics 2020-08-05 Yongrui Wang , Alexey Belyanin

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

We report the coherent phase-locking of a quantum cascade laser (QCL) at 10-$\mu$m to the secondary frequency standard of this spectral region, a CO2 laser stabilized on a saturated absorption line of OsO4. The stability and accuracy of the…

Dual-comb sources with equally spaced and low phase noise frequency lines are of great importance for high resolution spectroscopy and metrology. In the terahertz frequency range, electrically pumped semiconductor quantum cascade lasers…

Single-section quantum dash semiconductor lasers have attracted much attention as an integrated and simple platform for the generation of THz-wide and flat optical frequency combs in the telecom C-band. In this work, we present an…

We calculate the quantum-limited shape of the comb lines from a mode-locked Ti:sapphire laser using experimentally-derived parameters for the linear response of the laser to perturbations. The free-running width of the comb lines is found…

Optics · Physics 2009-11-13 J. K. Wahlstrand , J. T. Willits , C. R. Menyuk , S. T. Cundiff

Optical frequency combs establish a rigid phase-coherent link between microwave and optical domains and are emerging as high-precision tools in an increasing number of applications. Frequency combs with large intermodal spacing are employed…

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

We demonstrate a powerful tool for high-resolution mid-IR spectroscopy and frequency metrology with quantum cascade lasers (QCLs). We have implemented frequency stabilization of a QCL to an ultra-low expansion (ULE) reference cavity, via…