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We report on a high-power mid-infrared frequency comb source based on a femtosecond Er:fiber oscillator with a stabilized repetition rate at 250 MHz. The mid-infrared frequency comb is produced through difference frequency generation in a…

We provide new measurements of wavenumbers and line identifications of 10 100 UI and UII near-infrared (NIR) emission lines between 2500 cm-1 and 12 000 cm-1 (4000 nm to 850 nm) using archival FTS spectra from the National Solar Observatory…

Instrumentation and Methods for Astrophysics · Physics 2011-12-07 Stephen L. Redman , James E. Lawler , Gillian Nave , Lawrence W. Ramsey , Suvrath Mahadevan

We generate a 200-nm optical frequency comb at 1.5 microns by injecting two single-frequency lasers into a highly nonlinear fiber, and explore its spectral phase properties and high power to demonstrate full nonlinear conversion into its…

We report the upgrade and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer allowing us to combine high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency…

Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…

Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here…

Optics · Physics 2019-02-28 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Photoabsorption spectra of N$_2$ and CO were recorded at 900K, using the vacuum-ultraviolet Fourier-transform spectrometer at the DESIRS beamline of synchrotron SOLEIL. These high-temperature and high-resolution measurements allow for…

A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…

This work presents the rovibrational spectra of the two strongest first overtone bands of the asymmetric stretching mode $\nu_3$ ($2\nu_3^{2+}$ and $2\nu_3^{2-}$) of the hydronium ion, H$_3$O$^+$. The measurements were performed in a…

Atomic Physics · Physics 2025-09-22 Chiara Schleif , Hayley A. Bunn , Miguel Jiménez-Redondo , Paola Caselli , Pavol Jusko

We report on the generation of frequency combs from the recently-discovered phenomenon of high-order sideband generation (HSG). A near-band gap continuous-wave (cw) laser with frequency $f_\text{NIR}$ was transmitted through an epitaxial…

The (2,0) (3,0) and (4,0) bands of the A$^1\Pi-$X$^1\Sigma^+$ system of $^{12}$C$^{16}$O have been re-investigated by high-resolution vacuum ultraviolet absorption spectroscopy. A VUV Fourier-transform spectrometer, illuminated by…

Atomic Physics · Physics 2016-04-20 M. L. Niu , E. J. Salumbides , A. N. Heays , N. de Oliveira , R. W. Field , W. Ubachs

Laser frequency combs are fast becoming critical to reaching the highest radial velocity precisions. One shortcoming is the highly variable brightness of the comb lines across the spectrum (up to 4-5 orders of magnitude). This can result in…

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

Optics · Physics 2017-04-05 Markku Vainio , Juho Karhu

We developed a novel technique for frequency measurement and synthesis, based on the operation of a femtosecond comb generator as transfer oscillator. The technique can be used to measure frequency ratios of any optical signals throughout…

Optics · Physics 2009-11-07 Jörn Stenger , Harald Schnatz , Christian Tamm , Harald R. Telle

Accurate parameters of molecular hot-band transitions, i.e., those starting from vibrationally excited levels, are needed to accurately model high-temperature spectra in astrophysics and combustion, yet laboratory spectra measured at high…

Optical frequency combs, coherent light sources that connect optical frequencies with microwave oscillations, have become the enabling tool for precision spectroscopy, optical clockwork and attosecond physics over the past decades. Current…

Optics · Physics 2017-03-21 S. -W. Huang , J. Yang , M. Yu , B. H. McGuyer , D. -L. Kwong , T. Zelevinsky , C. W. Wong

Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

We use optical-optical double-resonance (OODR) spectroscopy with a continuous wave (CW) pump and a cavity-enhanced frequency comb probe to measure high rotational energy levels of methane in the upper part of the triacontad polyad (P6). A…

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury