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Polaritonic states arise when a bright optical transition of a molecular ensemble is resonantly matched to an optical cavity mode frequency. Here, we lay the groundwork to study the behavior of polaritons in clean, isolated systems by…

Chemical Physics · Physics 2023-10-20 Adam D. Wright , Jane C. Nelson , Marissa L. Weichman

One important development in interaction potential models, or atomistic force fields, for molecular simulation is the inclusion of explicit polarisation, which represents the induction effects of charged or polar molecules on polarisable…

Soft Condensed Matter · Physics 2017-05-25 Agílio A. H. Pádua

We theoretically study the dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. In our prior work [Phys. Rev. Lett. 104, 226807 (2010)] we identified three regimes of long-term dynamics,…

Mesoscale and Nanoscale Physics · Physics 2014-07-28 M. Gullans , J. J. Krich , J. M. Taylor , B. I. Halperin , M. D. Lukin

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

The acceleration of ions in the interaction of circular polarized laser pulses with overdense plasmas is investigated. For circular polarization laser pulses, the quasi-equilibrium for electrons is established due to the light pressure and…

Accelerator Physics · Physics 2007-12-26 X. Q. Yan , C. Lin , Z. M. Sheng , Z. Y. Guo , B. C. Liu , Y. R. Lu , J. X. Fang , J. E. Chen

The propagation of the arbitrarily polarized pulse of the weak probe field through the resonant medium of Lambda-type three-level atoms with degenerate levels adiabatically driven by the coherent coupling field is considered. It is shown…

Optics · Physics 2014-10-17 V. A. Reshetov , I. V. Meleshko

We use the polarized Fock states to describe the coupled molecule-cavity hybrid system in quantum electrodynamics. The molecular permanent dipoles polarize the photon field by displacing its vector potential, leading to non-orthogonality…

Quantum Physics · Physics 2020-05-04 Arkajit Mandal , Sebastian Montillo Vega , Pengfei Huo

Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 Sahand Tabatabaei , Pritam Priyadarsi , Namanish Singh , Pardis Sahafi , Daniel Tay , Andrew Jordan , Raffi Budakian

Vibrational polaritons are formed by strong coupling of molecular vibrations and photon modes in an optical cavity. Experiments have demonstrated that vibrational strong coupling can change molecular properties and even affect chemical…

Quantum Physics · Physics 2025-01-14 Thomas Schnappinger , Cyril Falvo , Markus Kowalewski

The purpose of this work is to use active particles to study the effect of facilitation on supercooled liquids. To this end we investigate the behavior of a model supercooled liquid doped with intermittently active and intermittently slowed…

Soft Condensed Matter · Physics 2023-08-11 Victor Teboul

Liquid state Overhauser Effect Dynamic Nuclear Polarization (ODNP) has experienced a recent resurgence of interest. In particular, a new manifestation of the ODNP measurement measures the translational mobility of water within 5-10 \AA\ of…

Soft Condensed Matter · Physics 2023-02-23 John M. Franck , Anna Pavlova , Songi Han

Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt…

Quantum Physics · Physics 2007-05-23 Ying-Yen Liao , Yueh-Nan Chen , Der-San Chuu

We investigate the persistent orientation of asymmetric-top molecules induced by time-delayed THz pulses that are either collinearly or cross polarized. Our theoretical and numerical results demonstrate that the orthogonal configuration…

Chemical Physics · Physics 2023-12-05 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

When exposed to intense electromagnetic fields, the quantum vacuum is expected to exhibit properties of a polarisable medium akin to a weakly nonlinear dielectric material. Various schemes have been proposed to measure such vacuum…

High Energy Physics - Phenomenology · Physics 2016-03-08 B. King , T. Heinzl

The lowest energy states in transition metal dichalcogenide (TMD) monolayers follow valley selection rules, which have attracted vast interest due to the possibility of encoding and processing of quantum information. However, these quantum…

Mesoscale and Nanoscale Physics · Physics 2024-03-22 Sergii Morozov , Torgom Yezekyan , Christian Wolff , Sergey I. Bozhevolnyi , N. Asger Mortensen

We report the composite vortex solitons of three-wave mixing propagate stably in a three-dimensional (3D) quasi-phase-matched photonic crystals (QPM-PhC). The modulation of QPM-PhC is designed as a checkerboard pattern. The vortex solitons,…

Optics · Physics 2024-08-20 Chao Kong , Jinqing Li , Xinyi Tang , Xuli Li , Ju Jiao , Jun Cao , Haiming Deng

We perform metastability exchange optical pumping of helium-3 in a strong magnetic field of 1.5 T. The achieved nuclear polarization, from 80% at 1.33 mbar to 25% at 67 mbar, shows a substantial improvement at high pressures with respect to…

Atomic Physics · Physics 2009-09-29 Marie Abboud , Alice Sinatra , Xavier Maitre , Genevieve Tastevin , Pierre-Jean Nacher

Intermixed light-matter quasiparticles - polaritons - possess unique optical properties owned to their compositional nature. These intriguing hybrid states have been extensively studied over the past decades in a wide range of realizations…

We study a mechanism by which nuclear hyperpolarization due to the polarization transfer from a microwave-pulse-controlled electron spin is suppressed. From analytical and numerical calculations of the unitary dynamics of multiple nuclear…

Quantum Physics · Physics 2024-03-12 Kento Sasaki , Eisuke Abe

Group-IV monochalcogenides are a family of two-dimensional puckered materials with an orthorhombic structure that is comprised of polar layers. In this article, we use first principles calculations to show the multistability of monolayer…

Materials Science · Physics 2016-08-12 Paul Z. Hanakata , Alexandra Carvalho , David K. Campbell , Harold S. Park