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Efficient polarization of organic molecules is of extraordinary relevance when performing nuclear magnetic resonance (NMR) and imaging. Commercially available routes to dynamical nuclear polarization (DNP) work at extremely…

We analyze electron spin relaxation in electronic transport through coherently coupled double quantum dots in the spin blockade regime. In particular, we focus on hyperfine interaction as the spin relaxation mechanism. We pay special…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Carlos López-Monís , Jesús Iñarrea , Gloria Platero

{\bf Purpose}: Manipulation of the radio-sensitivity of the nucleotide-base driven by the spin blockade mechanism of diffusive free radicals against ionizing radiation. {\bf Materials and methods}: We theoretically propose a mechanism which…

Chemical Physics · Physics 2009-07-28 Ramin M. Abolfath

Dynamic nuclear polarization experiments use microwave irradiation to transfer the larger electron polarization to nuclear spins of interest, and thus enhance the NMR transitions above thermal equilibrium. How the polarization transfer from…

Chemical Physics · Physics 2026-01-12 Gian-Marco Camenisch , Nino Wili , Gunnar Jeschke , Matthias Ernst

Understanding the joint dynamics of electron and nuclear spins is central to core concepts in solid-state magnetic resonance - such as spin-lattice relaxation and dynamic nuclear polarization - but a generalization that capitalizes on…

Quantum Physics · Physics 2021-06-16 Santiago Bussandri , Pablo R. Zangara , Rodolfo H. Acosta , Carlos A. Meriles

The nuclear spin fluctuations (NSF) as well as the dynamic nuclear polarization (DNP) and their effects on the electron spins in negatively charged (In,Ga)As/GaAs quantum dots have been studied by polarized pump-probe and photoluminescence…

We study repeated (noncontinuous) measurements on the electron spin in a quantum dot and find that the measurement technique may lead to a different met$ or mechanism to realize nuclear spin polarization. While it may be used in any case,…

Quantum Physics · Physics 2011-07-28 Lian-Ao Wu

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

We have theoretically analyzed coherent nuclear-spin dynamics induced by electron transport through a quantum-dot spin valve. The hyperfine interaction between electron and nuclear spins in a quantum dot allows for the transfer of angular…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Stefano Chesi , W. A. Coish

Hyper-polarization of nuclear spins is crucial for advancing nuclear magnetic resonance (NMR) and quantum information technologies, as nuclear spins typically exhibit extremely low polarization at room temperature due to their small…

Quantum Physics · Physics 2025-05-20 Haiyang Li , Hao Liao , Ping Wang

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be…

Effects of both the dynamic nuclear polarization (DNP) created by circularly polarized light and the fluctuations of average nuclear spin in a quantum dot (QD) on the electron spin orientation are studied for singly negatively charged InP…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 S. Yu. Verbin , B. Pal , M. Ikezawa , I. V. Ignatiev , Y. Masumoto

Nuclear spin ensembles in diamond are promising candidates for quantum sensing applications, including rotation sensing. Here we perform a characterization of the optically detected nuclear-spin transitions associated with the 14N nuclear…

Optical and electrical control of the nuclear spin system allows enhancing the sensitivity of NMR applications and spin-based information storage and processing. Dynamic nuclear polarization in semiconductors is commonly achieved in the…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 G. Sallen , S. Kunz , T. Amand , L. Bouet , T. Kuroda , T. Mano , D. Paget , O. Krebs , X. Marie , K. Sakoda , B. Urbaszek

Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a…

Mesoscale and Nanoscale Physics · Physics 2014-10-03 A. Högele , M. Kroner , C. Latta , M. Claassen , I. Carusotto , C. Bulutay , A. Imamoglu

Among the possible types of magnetic dipole interactions in molecular systems, couplings between nuclear motion and the nuclear spin have probably received the least attention in molecular spectroscopy. Although very small in comparison to…

Chemical Physics · Physics 2026-04-22 Matthias Diez , Johannes K. Krondorfer , Albert Hirtenfelder , Andreas W. Hauser

Nuclear magnetism in n-doped semiconductors with positive hyperfine constant is revisited. Two kinds of nuclear magnetic ordering can be induced by resident electrons in a deeply cooled nuclear spin system. At positive nuclear spin…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 M. Vladimirova , D. Scalbert , M. S. Kuznetsova , K. V. Kavokin

We demonstrate methods to locally control the spin rotation of moving electrons in a GaAs channel. The Larmor frequency of optically-injected spins is modulated when the spins are dragged through a region of spin-polarized nuclei created at…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 M. E. Nowakowski , G. D. Fuchs , S. Mack , N. Samarth , D. D. Awschalom

Color centers that enable nuclear-spin control without RF fields offer a powerful route towards simplified and scalable quantum devices. Such capabilities are especially valuable for quantum sensing and computing platforms that already find…

We present a general method to realize resonant coupling between spins even though their energies are of different scales. Applying the method to the electron and nuclear spin systems such as a nitrogen-vacancy (NV) center with its nearby…

Quantum Physics · Physics 2023-11-20 Sichen Xu , Chanying Xie , Zhen-Yu Wang