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How liquid transport occurs in confined spaces is relevant to many industrial and lab-scale processes, ranging from enhanced oil recovery to drug delivery systems. In this work, we investigate propelling microdroplets that form from…

Soft Condensed Matter · Physics 2021-06-15 Gilmar F. Arends , John M. Shaw , Xuehua Zhang

Flow transport in confined spaces is ubiquitous in technological processes, ranging from separation and purification of pharmaceutical ingredients by microporous membranes and drug delivery in biomedical treatment to chemical and biomass…

Soft Condensed Matter · Physics 2021-01-01 Xuehua Zhang , Jae Bem You , Gilmar F. Arends , Jiasheng Qian , Yibo Chen , Detlef Lohse , John M. Shaw

Liquid-liquid phase separation has emerged as a fundamental mechanism underlying intracellular organization, with evidence for it being reported in numerous different systems. However, there is a growing concern regarding the lack of…

Soft Condensed Matter · Physics 2022-12-09 Mrityunjay Kothari , Tal Cohen

A recent study has demonstrated that phase separation in binary liquid mixtures is arrested in the presence of elastic networks and can lead to a nearly uniformly-sized distribution of the dilute-phase droplets. At longer timescales, these…

Soft Condensed Matter · Physics 2020-10-28 Mrityunjay Kothari , Tal Cohen

Molecular segregation in methanol-water mixtures is studied across a wide concentration range as a function of temperature and pressure. Cluster distributions obtained from both neutron diffraction and molecular dynamics simulations point…

Soft Condensed Matter · Physics 2009-11-10 L. Dougan , R. Hargreaves , S. P. Bates , J. L. Finney , V. Reat , A. K. Soper , J. Crain

Efficient and sustainable techniques for separating water-methanol mixtures are in high demand in the industry. Recent studies have revealed that membranes and 2D materials could achieve such separation. In our research, we explore the…

Soft Condensed Matter · Physics 2023-06-28 Roger Bellido-Peralta , Fabio Leoni , Carles Calero , Giancarlo Franzese

Phase separation and transitions among different molecular states are ubiquitous in living cells. Such transitions can be governed by local equilibrium thermodynamics or by active processes controlled by biological fuel. It remains largely…

Biological Physics · Physics 2021-11-24 G. Bartolucci , O. Adame-Arana , X. Zhao , C. A. Weber

Liquid-liquid phase separation is key to understanding aqueous two-phase systems (ATPS) arising throughout cell biology, medical science, and the pharmaceutical industry. Controlling the detailed morphology of phase-separating compound…

Soft Condensed Matter · Physics 2023-10-27 Eric W. Hester , Sean P. Carney , Vishwesh Shah , Alyssa Arnheim , Bena Patel , Dino Di Carlo , Andrea L. Bertozzi

The formation of (bio)molecular condensates via liquid-liquid phase separation in cells has received increasing attention, as these coacervates play important functional and regulatory roles within biological systems. However, the majority…

Soft Condensed Matter · Physics 2022-11-24 Arash Nikoubashman , Miho Yanagisawa

Transport of liquid mixtures through porous membranes is central to processes such as desalination, chemical separations and energy harvesting, with ultrathin membranes made from novel 2D nanomaterials showing exceptional promise. Here we…

Soft Condensed Matter · Physics 2019-08-06 Daniel J. Rankin , Lydéric Bocquet , David M. Huang

Using dissipative particle dynamics simulations, we study the effects of an embedding bulk fluid on the phase separation dynamics in a thin planar liquid film. The domain growth exponent is altered from 2D to 3D behavior upon the addition…

Soft Condensed Matter · Physics 2015-05-18 Sanoop Ramachandran , Shigeyuki Komura , Gerhard Gompper

The separation of liquid mixture has been studied for a long time. Separation proceeds based on the difference in physical properties including pore size and electrostatic interaction. Therefore, there are many difficulties in separation of…

Materials Science · Physics 2021-01-26 Kyoung Hwan Choi , Da Young Hwang , Jeong Eon Park , Dong Hack Suh

Hypothesis: Multi-component droplet evaporation has received significant attention in recent years due to the broad range of applications such as material science, environmental monitoring, and pharmaceuticals. The selective evaporation…

Fluid Dynamics · Physics 2023-05-23 Hao Zeng , Yuki Wakata , Xing Chao , Mingbo Li , Chao Sun

We propose a model describing the phase behavior of two-component membranes consisting of binary mixtures of electrically charged and neutral lipids. We take into account the structural phase transition (main-transition) of the hydrocarbon…

Soft Condensed Matter · Physics 2016-07-11 Naofumi Shimokawa , Hiroki Himeno , Tsutomu Hamada , Masahiro Takagi , Shigeyuki Komura , David Andelman

We study theoretically the evaporation-driven phase separation of a binary fluid mixture in a thin film deposited on a moving substrate, as occurs in meniscus-guided deposition for solution-processed materials. Our focus is on rapid…

Soft Condensed Matter · Physics 2024-07-01 René de Bruijn , Anton A. Darhuber , Jasper J. Michels , Paul van der Schoot

We study the thermodynamic behavior of nonpolar liquid mixtures in the vicinity of curved charged objects, such as electrodes or charged colloids. For small enough charge on the object, or equivalently, small potential, the…

Statistical Mechanics · Physics 2009-11-13 Gilad Marcus , Sela Samin , Yoav Tsori

The filtration membranes are often elaborated through a phase separation process where a polymer rich phase and a polymer poor phase spontaneously form through spinodal decomposition. One process that is still not well understood from a…

The solvation structure of protons in aqueous media is highly relevant to electric properties and to proton transport in liquids and membranes. At ambient temperature, polar liquids display structural fluctuations on femto- to picosecond…

Living and engineered systems rely on the stable coexistence of two interspersed liquid phases. Yet surface tension drives their complete separation. Here we show that stable droplets of uniform and tuneable size can be produced through…

Here we investigate how the positions of a condensed phase can be controlled by using concentration gradients of a regulator that influences phase separation. We consider a mean field model of a ternary mixture where a concentration…

Soft Condensed Matter · Physics 2018-08-15 Samuel Krüger , Christoph A. Weber , Jens-UweSommer , Frank Jülicher
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