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The Zhang-Rice (ZR) singlet is an intriguing quantum state offering potential to realize a spin-orbit-entangled bosonic quasiparticle, which gives rise to the Zhang-Rice exciton. Its formation is attributed to the correlation between a…

Other Condensed Matter · Physics 2025-07-30 Nasaru Khan , Yuliia Shemerliuk , Sebastian Selter , Bernd Büchner , Saicharan Aswartham , Pradeep Kumar

Monolayer and few-layer phosphorene are anisotropic quasi-two-dimensional (quasi-2D) van der Waals (vdW) semiconductors with a linear-dichroic light-matter interaction and a widely-tunable direct-band gap in the infrared frequency range.…

The recently discovered two-dimensional (2D) van der Waals magnet NiPS$_3$ provides a new route to examine many-body quasiparticles under 2D confinement. Excitons are of particular interest due to their strong coupling to the magnetic…

Strongly Correlated Electrons · Physics 2022-10-07 Christopher Lane , Jian-Xin Zhu

Two-dimensional (2D) van der Waals (vdW) heterostructures (HSs) provide a versatile platform for tailoring electronic, optical, and magnetic properties via proximity effects at their interfaces. In this work, we explore the optical response…

Collective excitations of bound electron-hole pairs -- known as excitons -- are ubiquitous in condensed matter, emerging in systems as diverse as band semiconductors, molecular crystals, and proteins. Recently, their existence in strongly…

Semi-metallic graphene and semiconducting monolayer transition metal dichalcogenides (TMDCs) are the two-dimensional (2D) materials most intensively studied in recent years. Recently, black phosphorus emerged as a promising new 2D material…

Mesoscale and Nanoscale Physics · Physics 2014-11-07 Xiaomu Wang , Aaron M. Jones , Kyle L. Seyler , Vy Tran , Yichen Jia , Huan Zhao , Han Wang , Li Yang , Xiaodong Xu , Fengnian Xia

Two-dimensional antiferromagnets are promising materials for spintronics. The van der Waals antiferromagnet NiPS$_3$ has attracted extensive interest due to its ultra-narrow exciton feature which is closely linked with the magnetic…

Strongly Correlated Electrons · Physics 2025-04-09 Jacob A. Warshauer , Huyongqing Chen , Qishuo Tan , Jing Tang , Xi Ling , Wanzheng Hu

The interplay between dimensionality and electronic correlations in van der Waals (vdW) materials offers a powerful toolkit for engineering light-matter interactions at the nanoscale. Excitons, bound electron-hole pairs, are central to this…

Topological band theory has expanded into various domains in applied physics, offering significant potential for future technologies. Recent developments indicate that unique bulk band topology perceived for electrons can be realized in a…

Layered magnetic and strongly correlated materials present a rich platform for condensed matter physics with intrinsic properties intertwined by magnetism and low-dimensionality. A suspended light-emitting 2D antiferromagnetic membrane…

Van der Waals materials and heterostructures manifesting strongly bound room temperature exciton states exhibit emergent physical phenomena and are of a great promise for optoelectronic applications. Here, we demonstrate that nanostructured…

2D magnetic semiconductor CrSBr exhibits unique magneto-optical properties, yet its electronic structure and photophysical mechanisms remain unclear at high magnetic field and low temperature. Through comprehensive spectroscopic…

Materials Science · Physics 2024-11-28 Xiaodong Shen , Jiajun Cao , Weizheng Liang , Borong Cong , Bao Ke , Jialong Zhao , Bingsuo Zou

Ultrafast and coherent generation of magnons is of great significance for high-speed antiferromagnetic spintronics. One possible route is by exciton-magnon pairwise optical excitation. To date, such exciton-magnon transitions have been…

Strongly Correlated Electrons · Physics 2023-12-04 Ziqian Wang , Xiao-Xiao Zhang , Yuki Shiomi , Taka-hisa Arima , Naoto Nagaosa , Yoshinori Tokura , Naoki Ogawa

Van der Waals heterostructures assembled from layers of 2D materials have attracted considerable interest due to their novel optical and electrical properties. Here we report a scattering-type scanning near field optical microscopy study of…

The observation of magnetic ordering in atomically thin CrI$_3$ and Cr$_2$Ge$_2$Te$_6$ monolayers has aroused intense interest in condensed matter physics and material science. Studies of van de Waals two-dimensional (2D) magnetic materials…

Materials Science · Physics 2023-11-14 Tian-Xiang Qian , Ju Zhou , Tian-Yi Cai , Sheng Ju

We study the energies and optical spectra of excitons in twisted bilayers of anisotropic van der Waals semiconductors exhibiting moir\'e patterns, taking phosphorene as a case study. Following the electronic Hamiltonian introduced by us in…

Mesoscale and Nanoscale Physics · Physics 2023-08-08 Isaac Soltero , David A. Ruiz-Tijerina

Van der Waals (vdW) layered materials with long-range magnetic order have the potential to enable novel optoelectronic and spintronic applications. Among these, CrSBr is an air-stable, direct band gap semiconductor that hosts interlayer…

Layered van der Waals materials offer novel opportunities for on-chip waveguiding and development of integrated photonic circuits. In the strong light-matter coupling regime, their nonlinear response can be significantly enhanced, which is…

The unique discovery of magnetic exciton in van der Waals antiferromagnet NiPS3 arises between two quantum many-body states of a Zhang-Rice singlet excited state and a Zhang-Rice triplet ground state. Simultaneously, the spectral width of…

The ability to assemble layers of two-dimensional (2D) materials to form permutations of van der Waals heterostructures provides significant opportunities in materials design and synthesis. Interlayer interactions provide a path to new…

Mesoscale and Nanoscale Physics · Physics 2023-01-09 Zachariah Hennighausen , Jisoo Moon , Kathleen M. McCreary , Connie H. Li , Olaf M. J. van `t Erve , Berend T. Jonker
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