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We study dipole interseries transitions between the yellow and green exciton series in cuprous oxide including the complex valence band structure. To this end, we extend previous studies of the spectrum of complex green exciton resonances…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Patric Rommel , Jörg Main , Sjard Ole Krüger , Stefan Scheel

We report experimental and theoretical investigations of interacting excitons of the yellow series in cuprous oxide (Cu$_2$O) with principal quantum numbers up to $n=7$ by means of second harmonic generation (SHG). Using picosecond pulsed…

When an electron in a semiconductor gets excited to the conduction band the missing electron can be viewed as a positively charged particle, the hole. Due to the Coulomb interaction electrons and holes can form a hydrogen-like bound state…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Jan Ertl , Sebastian Rentschler , Jörg Main

We investigate the infrared optical transitions between excitons of the yellow, green and blue series in the cuprous oxide Cu$_{\mathrm{2}}$O. We show that in many cases the dipole approximation is inadequate and, in particular, that it…

Mesoscale and Nanoscale Physics · Physics 2019-08-05 Sjard Ole Krüger , Stefan Scheel

When treating the exchange interaction of Wannier excitons, usually only the leading terms of the analytic and the nonanalytic exchange interaction are considered. However, higher order terms can lead to a splitting of exciton states, for…

Materials Science · Physics 2016-09-13 Frank Schweiner , Jörg Main , Günter Wunner , Christoph Uihlein

We study the absorption spectra of the yellow excitons in Cu$_2$O in high magnetic fields using polarization-resolved optical absorption measurements with a high frequency resolution. We show that the symmetry of the yellow exciton results…

We numerically investigate the odd parity states of the green exciton series in cuprous oxide. Taking into account the coupling to the yellow series and especially to the yellow continuum, the green excitons are quasi-bound resonances with…

Materials Science · Physics 2020-03-02 Patric Rommel , Patrik Zielinski , Jörg Main

Recent high-resolution absorption spectroscopy on excited excitons in cuprous oxide [Nature (London) 514, 343 (2014)] has revealed significant deviations of their spectrum from that of the ideal hydrogen-like series. Here we show that the…

An experimental study of the yellow exciton series in Cu2O in strong magnetic fields up to 32 T shows the optical activation of direct and phonon-assisted paraexciton luminescence due to mixing with the quadruple allowed orthoexciton state.…

Other Condensed Matter · Physics 2009-03-03 D. Fishman , C. Faugeras , M. Potemski , A. Revcolevschi , P. H. M. van Loosdrecht

We report on the observation of the yellow exciton Lyman series up to the fourth term in Cu2O by time-resolved mid-infrared spectroscopy. The dependence of the oscillator strength on the principal quantum number n can be well reproduced…

Materials Science · Physics 2009-11-11 Takeshi Tayagaki , Andre Mysyrowicz , Makoto Kuwata-Gonokami

In $\mathrm{Cu_{2}O}$ parity is a good quantum number and thus the exciton spectrum falls into two parts: The dipole-active exciton states of negative parity and odd angular momentum, which can be observed in one-photon absorption…

Materials Science · Physics 2017-05-08 Frank Schweiner , Jörg Main , Günter Wunner , Christoph Uihlein

The fluctuation exchange, or FLEX, approximation for interacting electrons is applied to study instabilities in the standard three-band model for CuO2 layers in the high-temperature superconductors. Both intra-orbital and near-neigbor…

Superconductivity · Physics 2009-10-30 G. Esirgen , N. E. Bickers

Excitons with a radius of a few lattice constants can be affected by strong central-cell corrections, leading to significant deviations of the optical spectrum from the hydrogen-like Rydberg series, and also to an enhancement of the exciton…

Materials Science · Physics 2018-01-30 Andreas Alvermann , Holger Fehske

Analytical expressions for the exchange interaction between $J$-multiplets of interacting metallic centers are derived on the basis of a complete electronic model. A common belief that this interaction can be approximated by an isotropic…

Strongly Correlated Electrons · Physics 2015-05-29 Naoya Iwahara , Liviu F. Chibotaru

The observation of giant Rydberg excitons in cuprous oxide $\left(\mathrm{Cu_{2}O}\right)$ up to a principal quantum number of $n=25$ by T.~Kazimierczuk \emph{et al.} [Nature \textbf{514}, 343, (2014)] inevitably raises the question whether…

Materials Science · Physics 2017-12-07 Frank Schweiner , Jan Ertl , Jörg Main , Günter Wunner , Christoph Uihlein

We present a method to calculate the exciton spectra of all direct semiconductors with a complex valence band structure. The Schr\"odinger equation is solved using a complete basis set with Coulomb Sturmian functions. This method also…

Materials Science · Physics 2016-05-09 Frank Schweiner , Jörg Main , Matthias Feldmaier , Günter Wunner , Christoph Uihlein

We have used high resolution transmission spectroscopy to study the exciton level spectrum in Cu$_2$O subject to a longitudinal external electric field, i.e., in the geometry where the transmitted light is propagating along the field…

Materials Science · Physics 2017-02-01 J. Heckötter , M. Freitag , D. Fröhlich , M. Aßmann , M. Bayer , M. A. Semina , M. M. Glazov

We propose a microscopical theory of superconductivity in CuO$_2$ layer within the effective two-band Hubbard model in the strong correlation limit. By applying a projection technique for the matrix Green function in terms of the Hubbard…

Superconductivity · Physics 2015-06-24 N. M. Plakida , L. Anton , S. Adam , Gh. Adam

We present a variational method to calculate the exchange interactions among donor clusters in a semiconductor. Such clusters are candidates for a so-called control-qubit architecture for quantum information, where the effective exchange…

Materials Science · Physics 2007-11-02 W. Wu , P. T. Greenland , A. J. Fisher

Excitons, as bound states of electrons and holes, embody the solid state analogue of the hydrogen atom, whose quantum spectrum is explained within a classical framework by the Bohr-Sommerfeld atomic model. In a first hydrogenlike…

Mesoscale and Nanoscale Physics · Physics 2024-04-17 Jan Ertl , Michael Marquardt , Moritz Schumacher , Patric Rommel , Jörg Main , Manfred Bayer
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