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Related papers: Electronic structure and magnetism in UGa2: DFT+DM…

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Originating from a broken spatial inversion symmetry, ferroelectricity is a functionality of materials with an electric dipole that can be switched by external electric fields. Spontaneous polarization is a crucial ferroelectric property,…

Materials Science · Physics 2017-08-03 Yubo Zhang , Jianwei Sun , John P. Perdew , Xifan Wu

The Gutzwiller technique has long been known as a method to include correlations in electronic structure calculations. Here we implement an ab-initio Gutzwiller+LDA calculation, and apply it to a classic problem, the ferromagnetism of bulk…

Strongly Correlated Electrons · Physics 2013-07-23 Giovanni Borghi , Michele Fabrizio , Erio Tosatti

In this article we introduce a generalization of the popular DFT+U method based on the extended Hubbard model that includes on-site and inter-site electronic interactions. The novel corrective Hamiltonian is designed to study systems for…

Strongly Correlated Electrons · Physics 2015-05-13 Vivaldo Leiria Campo , Matteo Cococcioni

Many-body theories such as dynamical mean field theory (DMFT) have enabled the description of the electron exchange-correlation interactions that are missing in current density functional theory (DFT) calculations. However, there has been…

Strongly Correlated Electrons · Physics 2021-01-19 A. D. N. James , E. I. Harris-Lee , A. Hampel , M. Aichhorn , S. B. Dugdale

In heavy-fermion compounds, the dual character of $f$ electrons underlies their rich and often exotic properties like fragile heavy quasipartilces, variety of magnetic orders and unconventional superconductivity. 5$f$-electron actinide…

Strongly Correlated Electrons · Physics 2019-09-13 Q. Y. Chen , X. B. Luo , D. H. Xie , M. L. Li , X. Y. Ji , R. Zhou , Y. B. Huang , W. Zhang , W. Feng , Y. Zhang , X. G. Zhu , Q. Q. Hao , Q. Liu , L. Huang , P. Zhang , X. C. Lai , Q. Si , S. Y. Tan

We present the band structure of CeIr$_3$ superconductor calculated within the dynamical mean field theory (DMFT). Standard GGA and GGA+U methods fail to reproduce the experimental electronic specific heat coefficient $\gamma_{\rm expt.}$…

Strongly Correlated Electrons · Physics 2022-01-05 Sylwia Gutowska , Bartlomiej Wiendlocha

We analyze possible ways to calculate magnetic exchange interactions within the density functional theory plus dynamical mean-field theory (DFT+DMFT) approach in the paramagnetic phase. Using the susceptibilities obtained within the ladder…

Strongly Correlated Electrons · Physics 2023-06-09 A. A. Katanin , A. S. Belozerov , A. I. Lichtenstein , M. I. Katsnelson

We investigate the electronic structure of EuFe$_{2}$As$_{2}$ using optical spectroscopy and first-principles calculations. At low temperature we observe the evolution of \textit{two} gap-like features, one having a BCS mean-field behavior…

The microscopic origin of metamagnetism and metamagnetic transitions in strongly anisotropic antiferromagnets is investigated within a quantum mechanical theory of correlated electrons. To this end the Hubbard model with staggered…

Strongly Correlated Electrons · Physics 2009-10-30 K. Held , M. Ulmke , N. Bl"umer , D. Vollhardt

The fundamental controversy about the electronic structure for 3d-electron states in FeBr2 is discussed. We advocate for the localized electron atomic-like many-electron crystal-field approach that yields the discrete energy spectrum, in…

Strongly Correlated Electrons · Physics 2008-10-08 Z. Ropka , R. J. Radwanski

Elemental rare-earth metals provide a playground for studying novel electron correlation effects and complex magnetism. However, ab initio simulations of these systems remain challenging. Here, we employ fully charge self-consistent density…

Strongly Correlated Electrons · Physics 2024-12-23 Wenjun Ding , Yogesh K. Vohra , Cheng-Chien Chen

The structural and magnetic properties of spinel compounds $CoB_2O_4$ (B=Cr,Mn and Fe) are studied using the DFT+U method and generalized gradient approximation (GGA). We concentrate on understanding the trends in the properties of these…

Strongly Correlated Electrons · Physics 2016-09-21 Debashish Das , Rajkumar Biswas , Subhradip Ghosh

Methods based on the combination of the usual density functional theory (DFT) codes with the Hubbard models are widely used to investigate the properties of strongly correlated materials. Using first-principle calculations we study the…

Materials Science · Physics 2015-08-04 Christos Tsirogiannis , Iosif Galanakis

We calculate the properties of the 4$d$ ferromagnet SrRuO$_3$ in bulk and thin film form with the aim of understanding the experimentally observed metal to insulator transition at reduced thickness. Although the spatial extent of the 4$d$…

Materials Science · Physics 2008-10-08 James M. Rondinelli , Nuala M. Caffrey , Stefano Sanvito , Nicola A. Spaldin

The problem of importance of strong correlations for the electronic structure, transport and magnetic properties of half--metallic ferromagnetic CrO_2 is addressed by performing density functional electronic structure calculations in the…

Strongly Correlated Electrons · Physics 2009-11-10 A. Toropova , G. Kotliar , S. Y. Savrasov , V. S. Oudovenko

The superconductor UCoGe is analyzed with electronic structure calculations using Linearized Augmented Plane Wave method based on Density Functional Theory. Ferromagnetic and antiferromagnetic calculations with and without correlations (via…

Superconductivity · Physics 2009-11-13 Pablo de la Mora , O. Navarro

Positive muon spin relaxation measurements performed on the ferromagnet UGe2 reveal, in addition to the well known localized 5f-electron density responsible for the bulk magnetic properties, the existence of itinerant quasi-static magnetic…

Strongly Correlated Electrons · Physics 2009-11-07 A. Yaouanc , P. Dalmas de Reotier , P. C. M. Gubbens , C. T. Kaiser , A. A. Menovsky , M. Mihalik , S. P. Cottrell

We study magnetic properties of CrO$_2$ within the density functional theory plus dynamical mean-field theory (DFT+DMFT) approach in the paramagnetic phase. We consider the 3-orbital (per Cr site) model, containing only $t_{2g}$ states, the…

Strongly Correlated Electrons · Physics 2024-10-15 A. A. Katanin

Accurate low-order structure factors (Fg) measured by quantitative convergent beam electron diffraction (QCBED) were used for validation of different density functional theory (DFT) approximations. 23 low-order Fg were measured by QCBED for…

Materials Science · Physics 2013-02-26 Xiahan Sang , Andreas Kulovits , Guofeng Wang , Jorg Wiezorek

In this paper we report comprehensive experimental and theoretical investigation of magnetic and electronic properties of the intermetallic compounds Pr2Fe17 and Gd2Fe17. For the first time electronic structure of these two systems was…

Strongly Correlated Electrons · Physics 2007-05-23 Yu. V. Knyazev , A. V. Lukoyanov , Yu. I. Kuz'min , A. G. Kuchin , I. A. Nekrasov