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The magnetic properties of the alkaline earth oxocuprate BaCu3O4 are investigated. We show that the characteristic Cu3O4 layers of this material can be described with diamond chains of antiferromagnetically coupled Cu 1/2 spins with only a…

Strongly Correlated Electrons · Physics 2012-04-18 Carl-Willem Rischau , Brigitte Leridon , Dorothée Colson , Anne Forget , Philippe Monod

The magnetic excitation spectrum and Hamiltonian of the quantum magnet BaCuTe2O6 is studied by inelastic neutron scattering (INS) and density functional theory (DFT). INS on powder and single crystal samples reveals overlapping spinon…

Strongly Correlated Electrons · Physics 2023-05-19 A. Samartzis , S. Chillal , H. O. Jeschke , D. J. Voneshen , Z. Lu , A. T. M. N. Islam , B. Lake

We report on the crystal structure of the quantum magnet (CuCl)LaNb2O7 that was controversially described with respect to its structural organization and magnetic behavior. Using high-resolution synchrotron powder x-ray diffraction,…

Materials Science · Physics 2015-03-17 Alexander A. Tsirlin , Artem M. Abakumov , Gustaaf Van Tendeloo , Helge Rosner

The structural and magnetic properties of the face-centered cubic double perovskite Ba2MnWO6 were investigated using neutron powder diffraction, DC-magnetometry, muon spin relaxation and inelastic neutron scattering. Ba2MnWO6 undergoes Type…

Magnetization measurements on single-crystal cubic SrCuTe$_2$O$_6$ with an applied magnetic field of along three inequivalent high symmetry directions $[100]$, $[110]$, and $[111]$ reveal weak magnetic anisotropy. The fits of the magnetic…

Strongly Correlated Electrons · Physics 2020-10-14 P. Saeaun , Y. Zhao , P. Piyawongwatthana , T. J. Sato , F. C. Chou , M. Avdeev , G. Gitgeatpong , K. Matan

We performed susceptibility, magnetization, specific heat, and single crystal neutron diffraction measurements on single crystalline BaMn$_2$Si$_2$O$_7$. Based on the results, we revisited its spin structure with a more accurate solution…

Strongly Correlated Electrons · Physics 2019-07-31 G. H. Wang , C. Y. Xu , H. B. Cao , T. Hong , Q. Huang , Q. Y. Ren , J. Q. Xu , H. D. Zhou , W. D. Luo , D. Qian , J. Ma

The complex perovskite Pb2CoTeO6 (PCTO) has been prepared as polycrystalline powders by solid state reaction route, and the crystal structure and magnetic properties have been investigated using a combination of X-ray and neutron powder…

Materials Science · Physics 2010-12-01 S. A. Ivanov , P. Nordblad , R. Mathieu , R. Tellgren , C. Ritter

We performed high-resolution powder neutron diffraction experiments and discovered an elliptic helical incommensurate magnetic structure in the semiconducting rare-earth magnet YbCuS2, featuring effective spin-1/2 Yb$^{3+}$ ions that form a…

Strongly Correlated Electrons · Physics 2025-01-09 T. Onimaru , Y. Ohmagari , S. Mizutani , R. Yamamoto , H. Kaneshima , C. Moriyoshi , D. T. Adroja , D. Khyalyavin , P. Manuel , H. Saito , C. Hotta

New fluoropnictides BaMnPnF with Pn = As, Sb, Bi, are synthesized by stoichiometric reaction of elements with BaF\_2. The compounds crystallize in the tetragonal P4/nmm (No. 129, Z = 2) space group, with the ZrCuSiAs-type structure, as…

Strongly Correlated Electrons · Physics 2013-07-09 Bayrammurad Saparov , David J. Singh , V. Ovidiu Garlea , Athena S. Sefat

Barlowite, Cu$_{4}$(OH)$_{6}$FBr, has attracted much attention as the parent compound of a new series of quantum spin liquid candidates, Zn$_{x}$Cu$_{4-x}$(OH)$_{6}$FBr. While it is known to undergo a magnetic phase transition to a…

Strongly Correlated Electrons · Physics 2018-12-05 K. Tustain , G. J. Nilsen , C. Ritter , I. da Silva , L. Clark

We investigate the structural and magnetic properties of two molecule-based magnets synthesized from the same starting components. Their different structural motifs promote contrasting exchange pathways and consequently lead to markedly…

The antiferromagnetism in $\alpha$-Cu$_3$Mg(OH)$_6$Br$_2$ was studied by magnetic-susceptibility, specific-heat and neutron-diffraction measurements. The crystal structure consists of Cu$^{2+}$ kagome layers with Mg$^{2+}$ ions occupying…

Strongly Correlated Electrons · Physics 2019-10-23 Yuan Wei , Zili Feng , Clarina dela Cruz , Wei Yi , Zi Yang Meng , Jia-Wei Mei , Youguo Shi , Shiliang Li

The magnetic and structural properties of polycrystalline Co$_{4-x}$ Ni$_x$ Nb$_2$ O$_9$ (x=1,2) have been investigated by neutron powder diffraction, magnetization and heat capacity measurements, and density functional theory (DFT)…

The magnetic properties of a new compound, Na5RbCu4(AsO4)4Cl2 are reported. The material has a layered structure comprised of square Cu4O4 tetramers. The Cu ions are divalent and the system behaves as a low-dimensional S=1/2…

Strongly Correlated Electrons · Physics 2009-11-07 J. A. Clayhold , M. Ulutagay-Kartin , S. -J. Hwu , H. -J. Koo , M. -H. Whangbo , A. Voigt , K. Eaiprasertsak

The magnetic structure of the double perovskite compound Sr$_2$CuTeO$_6$ was determined from neutron powder diffraction data. This material is magnetically described as an $S\,{=}\,1/2$ quasi-two-dimensional square-lattice Heisenberg model…

Strongly Correlated Electrons · Physics 2016-03-09 Tomoyuki Koga , Nobuyuki Kurita , Maxim Avdeev , Sergey Danilkin , Taku J. Sato , Hidekazu Tanaka

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

Materials Science · Physics 2007-05-23 Coen de Graaf , Iberio de P. R. Moreira , Francesc Illas , Oscar Iglesias , Amilcar Labarta

The magnetic behavior of the Ca3Co2O6 spin chain compound is characterized by a large Ising-like character of its ferromagnetic chains, set on triangular lattice, that are antiferromagnetically coupled. At low temperature, T < 7K, the 3D…

Strongly Correlated Electrons · Physics 2007-05-23 A. Maignan , V. Hardy , S. Hebert , M. Drillon , M. R. Lees , O. Petrenko , D. Mc K. Paul , D. Khomskii

The magnetic behavior of the compound, Gd3Ru4Al12, which has been reported to crystallize in a hexagonal structure about two decades ago, had not been investigated in the past literature despite interesting structural features (that is,…

Strongly Correlated Electrons · Physics 2016-06-22 Venkatesh Chandragiri , Kartik K Iyer , E. V. Sampathkumaran

A complex magnetic order of the multiferroic compound Co3TeO6 has been revealed by neutron powder diffraction studies on ceramics and crushed single crystals. The compound adopts a monoclinic structure (s.g. C2/c) in the studied temperature…

Materials Science · Physics 2011-11-28 S. A. Ivanov , R. Tellgren , C. Ritter , P. Nordblad , R. Mathieu , G. Andre , N. V. Golubko , E. D. Politova , M. Weil