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We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…

While spin polarization from synchrotron radiation is well established, the polarization of orbital angular momentum (OAM) in such radiative processes remains elusive. We study radiation and polarization of relativistic electrons in a…

Accelerator Physics · Physics 2026-04-24 Ziqiang Huang , Qi Meng , Xuan Liu , Wei Ma , Zhen Yang , Liang Lu , Alexander J. Silenko , Pengming Zhang , Liping Zou

Recent advances in the production of twisted electron beams with a subnanometer spot size offer unique opportunities to explore the role of orbital angular momentum (OAM) in basic atomic processes. In the present work, we address one of…

The electron and ion properties observed in a photoionization inherit a symmetry properties of both a target and a radiation. Introducing a symmetry breaking in a photoionization process one can expect to observe a noticeable variation of…

Atomic Physics · Physics 2024-02-09 Maksim D. Kiselev , Elena V. Gryzlova , Alexei N. Grum-Grzhimailo

Ultrafast imaging of molecular chirality is a key step towards the dream of imaging and interpreting electronic dynamics in complex and biologically relevant molecules. Here, we propose a new ultrafast chiral phenomenon exploiting recent…

We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…

We obtain an expression for the matrix element for a twisted (Laguerre-Gaussian profile) photon scattering from a hydrogen atom. We consider photons incoming with an orbital angular momentum (OAM) of $\ell \hbar$, carried by a factor of…

Quantum Physics · Physics 2013-02-06 Basil S. Davis , L. Kaplan , J. H. McGuire

The combination of photoelectron spectroscopy and ultrafast light sources is on track to set new standards for detailed interrogation of dynamics and reactivity of molecules. A crucial prerequisite for further progress is the ability to not…

We show that ionization of noble gas atoms by strong infrared circularly polarized laser field under standard exerimental conditions can yield electrons with up to 100% spin polarization in energy resolved measurements. Spin polarization…

Atomic Physics · Physics 2013-07-18 Ingo Barth , Olga Smirnova

We demonstrate that strong-field ionization of atoms in circularly polarized laser fields generates a photoelectron spin texture with toroidal topology in momentum space. Using time-dependent Schr\"odinger equation simulations,…

Atomic Physics · Physics 2026-04-03 Xiaodan Mao , Feng He , Pei-Lun He

We consider electron-atom scattering in a circularly polarized laser field at sufficiently high electron energies, permitting to describe the scattering process by the first order Born approximation. Assuming the radiation field has…

Atomic Physics · Physics 2013-03-07 Aurelia Cionga , Fritz Ehlotzky , Gabriela Zloh

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

Atomic Physics · Physics 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

It has been known for a century that electromagnetic fields can transport not only energy and linear momentum but also angular momentum. However, it was not until twenty years ago, with the discovery in laser optics of experimental…

Instrumentation and Methods for Astrophysics · Physics 2011-02-01 Bo Thidé , Fabrizio Tamburini , Elettra Mari , Filippo Romanato , Cesare Barbieri

High-energy photons and other particles carrying non-zero orbital angular momentum (OAM) emerge as a new tool in high-energy physics. Recently, it was suggested to generate high-energy photons with non-zero OAM (twisted photons) by the…

High Energy Physics - Phenomenology · Physics 2013-05-29 I. P. Ivanov , V. G. Serbo

The relations among the components of the exit momenta of ultrarelativistic electrons scattered on a strong electromagnetic wave of a low (optical) frequency and linear polarization are established using the exact solutions to the equations…

Plasma Physics · Physics 2015-04-01 O. V. Bogdanov , P. O. Kazinski

We use the $R$-matrix with time-dependence method to study detachment from F$^-$ in circularly-polarized laser fields of infrared wavelength. By decomposing the photoelectron momentum distribution into separate contributions from detached…

Atomic Physics · Physics 2019-11-04 G. S. J. Armstrong , D. D. A. Clarke , A. C. Brown , H. W. van der Hart

We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and…

Atomic Physics · Physics 2017-09-05 Vinay Pramod Majety , Armin Scrinzi

Several experimental groups have recently obtained the so called vortex electrons (electrons with orbital angular momentum (OAM) of l = 100h) with energies of 300 keV. The gyromagnetic ratio of such electrons becomes proportional to the OAM…

Accelerator Physics · Physics 2014-10-16 Anatoly S. Konkov , Alexander P. Potylitsyn , Marina S. Polonskaya

When a strong laser pulse induces the ionization of an atom, momentum conservation dictates that the absorbed photons transfer their momentum $p_{\gamma}=E_{\gamma}/c$ to the electron and its parent ion. Even after 30 years of studying…

The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…