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We describe quantum circuits with only $\widetilde{\cal O}(N)$ Toffoli complexity that block encode the spectra of quantum chemistry Hamiltonians in a basis of $N$ arbitrary (e.g., molecular) orbitals. With ${\cal O}(\lambda / \epsilon)$…

Quantum computing has emerged as a promising platform for simulating strongly correlated systems in chemistry, for which the standard quantum chemistry methods are either qualitatively inaccurate or too expensive. However, due to the…

Chemical Physics · Physics 2024-05-06 Max Rossmannek , Fabijan Pavošević , Angel Rubio , Ivano Tavernelli

Context-aware compression techniques have gained increasing attention as model sizes continue to grow, introducing computational bottlenecks that hinder efficient deployment. A structured encoding approach was proposed to selectively…

Computation and Language · Computer Science 2025-02-13 Barnaby Schmitt , Alistair Grosvenor , Matthias Cunningham , Clementine Walsh , Julius Pembrokeshire , Jonathan Teel

Tensor algebra accelerators have been gaining popularity for running high-performance computing (HPC) workloads. Identifying optimal schedules for individual tensor operations and designing hardware to run these schedules is an active area…

Distributed, Parallel, and Cluster Computing · Computer Science 2025-03-05 Raveesh Garg , Michael Pellauer , Sivasankaran Rajamanickam , Tushar Krishna

Modeling electronic systems is an important application for quantum computers. In the context of materials science, an important open problem is the computational description of chemical reactions on surfaces. In this work, we outline a…

Coupling separately developed codes offers an attractive method for increasing the accuracy and fidelity of the computational models. Examples include the earth sciences and fusion integrated modeling. This paper describes the Framework…

Many critical EDA problems suffer from the curse of dimensionality, i.e. the very fast-scaling computational burden produced by large number of parameters and/or unknown variables. This phenomenon may be caused by multiple spatial or…

Numerical Analysis · Computer Science 2016-11-18 Zheng Zhang , Kim Batselier , Haotian Liu , Luca Daniel , Ngai Wong

Open quantum systems are ubiquitous in the physical sciences, with widespread applications in the areas of chemistry, condensed matter physics, material science, optics, and many more. Not surprisingly, there is significant interest in…

Quantum Physics · Physics 2023-07-13 Isobel A. Aloisio , Gregory A. L. White , Charles D. Hill , Kavan Modi

High-order solvers for compressible flows are vital in scientific applications. Adaptive mesh refinement (AMR) is a key technique for reducing computational cost by concentrating resolution in regions of interest. In this work, we develop…

Distributed, Parallel, and Cluster Computing · Computer Science 2025-08-08 Anjiang Wei , Hang Song , Mert Hidayetoglu , Elliott Slaughter , Sanjiva K. Lele , Alex Aiken

Quantum computers promise to transform our notions of computation by offering a completely new paradigm. To achieve scalable quantum computation, optimizing compilers and a corresponding software design flow will be essential. We present a…

Programming Languages · Computer Science 2018-07-24 Thomas Häner , Damian S. Steiger , Krysta Svore , Matthias Troyer

Running quantum algorithms often involves implementing complex quantum circuits with such a large number of multi-qubit gates that the challenge of tackling practical applications appears daunting. To date, no experiments have successfully…

The computational intensity of detector simulation and event reconstruction poses a significant difficulty for data analysis in collider experiments. This challenge inspires the continued development of machine learning techniques to serve…

High Energy Physics - Experiment · Physics 2024-11-22 Dmitrii Kobylianskii , Nathalie Soybelman , Nilotpal Kakati , Etienne Dreyer , Benjamin Nachman , Eilam Gross

Memcomputing is a novel paradigm of computation that utilizes dynamical elements with memory to both store and process information on the same physical location. Its building blocks can be fabricated in hardware with standard electronic…

Emerging Technologies · Computer Science 2018-07-03 Forrest Sheldon , Pietro Cicotti , Fabio L. Traversa , Massimiliano Di Ventra

Simulation of the dynamics of quantum materials is emerging as a promising scientific application for noisy intermediate-scale quantum (NISQ) computers. Due to their high gate-error rates and short decoherence times, however, NISQ computers…

Geometry optimization is an important part of both computational materials and surface science because it is the path to finding ground state atomic structures and reaction pathways. These properties are used in the estimation of…

Materials Science · Physics 2021-07-07 Yilin Yang , Omar A. Jimenez-Negron , John R. Kitchin

In the era of diminishing returns from Moores Law, heterogeneous computing systems have emerged as a vital approach to enhance computational efficiency. This paper introduces a novel MLIR-based dialect, named hyper, designed to optimize…

Cryptography and Security · Computer Science 2025-06-05 Zhiyuan Tan , Liutong Han , Mingjie Xing , Yanjun Wu

Electronic structure calculations of molecular systems are among the most promising applications for fault-tolerant quantum computing (FTQC) in quantum chemistry and drug design. However, while recent algorithmic advancements such as…

Achieving faster execution with shorter compilation time can foster further diversity and innovation in neural networks. However, the current paradigm of executing neural networks either relies on hand-optimized libraries, traditional…

Machine Learning · Computer Science 2020-01-27 Byung Hoon Ahn , Prannoy Pilligundla , Amir Yazdanbakhsh , Hadi Esmaeilzadeh

We demonstrate the feasibility of quantum computing for large-scale, realistic chemical systems through the development of a new interface using a quantum circuit simulator and CP2K, a highly efficient first-principles calculation software.…

Chemical Physics · Physics 2025-06-24 Tomoya Shiota , Klaas Gunst , Toshio Mori , Toru Shiozaki , Wataru Mizukami

Current quantum programming is dominated by low-level, circuit-centric approaches that limit the potential for compiler optimization. This work presents how a high-level programming construct provides compilers with the semantic information…

Quantum Physics · Physics 2025-10-29 Evandro C. R. Rosa , Jerusa Marchi , Eduardo I. Duzzioni , Rafael de Santiago