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We report the observation of superconductivity in infinite-layer Ca-doped LaNiO$_2$ (La$_{1-x}$Ca$_x$NiO$_2$) thin films and construct their phase diagram. Unlike the metal-insulator transition in Nd- and Pr-based nickelates, the undoped…

Superconductivity · Physics 2022-02-25 S. W. Zeng , C. J. Li , L. E. Chow , Y. Cao , Z. T. Zhang , C. S. Tang , X. M. Yin , Z. S. Lim , J. X. Hu , P. Yang , A. Ariando

Several reports about infinite-layer nickelate thin films suggest that the superconducting critical temperature versus chemical doping phase diagram has a dome-like shape, similar to cuprates. Here, we demonstrate a highly reproducible…

To understand the superconductivity recently discovered in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, we carried out LDA+DMFT (local density approximation plus dynamical mean-field theory) and magnetic force response calculations. The on-site correlation…

Superconductivity · Physics 2020-02-25 Siheon Ryee , Hongkee Yoon , Taek Jung Kim , Min Yong Jeong , Myung Joon Han

High-temperature unconventional superconductivity quite generically emerges from doping a strongly correlated parent compound, often (close to) an antiferromagnetic insulator. The recently developed dynamical vertex approximation is a…

Superconductivity · Physics 2024-06-04 Simone Di Cataldo , Paul Worm , Jan Tomczak , Liang Si , Karsten Held

The correlated electronic structure of the infinite-layer compounds NdNiO$_2$ and SrCuO$_2$ at stoichiometry and with finite hole doping is compared. Key differences are elucidated from an advanced first-principles many-body perspective.…

Strongly Correlated Electrons · Physics 2020-03-06 Frank Lechermann

The difficulty of determining cation concentrations and oxygen stoichiometry in infinite-layer nickelate thin films has so far prevented clear experimental identification of the nickel electron configuration in the superconducting phase. We…

Since the discovery of superconductivity in infinite-layer nickelates RNiO$_2$ (R=La, Pr, Nd), great research efforts have been paid to unveil its underlying superconducting mechanism. However, the physical origin of the intriguing…

Strongly Correlated Electrons · Physics 2022-07-20 T. Y. Xie , Z. Liu , Chao Cao , Z. F. Wang , J. L. Yang , W. Zhu

The discovery of nickelate superconductivity provided the first example of a non-copper-based material with superconductivity strongly analogous to the cuprates, but recent findings raise questions and inconsistencies around the electron…

Superconductivity · Physics 2024-11-05 Y. N. Huang , D. J. Singh

The observation of superconductivity in infinite layer nickelate (Nd,Sr)NiO$_{2}$ thin films has led to rapid theoretical and experimental investigations of these copper-oxide-analogue systems [1-15]. Superconductivity has also been found…

The recent discovery of high-T$_{c}$ superconductivity (HTS) in Sr-doped NdNiO$_2$ has sparked a renewed interest in investigating nickelates as cuprate counterparts. Parent cuprates [Cu$^{2+}$: d$^9$] are antiferromagnetic charge-transfer…

Superconductivity · Physics 2021-01-04 Jyoti Krishna , Harrison LaBollita , Adolfo O. Fumega , Victor Pardo , Antia S. Botana

The novel nickelate superconductors of infinite-layer type feature challenging electronic pecularities in the normal-state phase diagram with doping. Distinct many-body behavior and different dispersion regimes of the entangled…

Strongly Correlated Electrons · Physics 2021-04-29 Frank Lechermann

Using first-principles density functional theory calculations, we investigated the effect of charge doping in a LaNiO$_3$/SrTiO$_3$ superlattice. The detailed analysis based on two different simulation methods for doping clearly shows that…

Strongly Correlated Electrons · Physics 2015-06-04 Heung-Sik Kim , Myung Joon Han

Rare-earth nickelates R$^{3+}$Ni$^{3+}$O$_3$ (R=Lu-Pr, Y) show a striking metal-insulator transition in their bulk phase whose temperature can be tuned by the rare-earth radius. These compounds are also the parent phases of the newly…

Materials Science · Physics 2021-07-21 Lucia Iglesias , Manuel Bibes , Julien Varignon

The recent and exciting discovery of superconductivity in the hole-doped infinite-layer nickelate Nd 1-{\delta} Sr {\delta} NiO 2 draws strong attention to correlated quantum materials. From a theoretical view point, this new class of…

Strongly Correlated Electrons · Physics 2021-01-05 Byungkyun Kang , Corey Melnick , Patrick Semon , Siheon Ryee , Myung Joon Han , Gabriel Kotliar , Sangkook Choi

We report the phase diagram of Nd$_{1-x}$Sr$_x$NiO$_2$ infinite layer thin films grown on SrTiO$_3$. A superconducting dome spanning $0.125 < x < 0.25$ is found, remarkably similar to cuprates, albeit over a narrower doping window. However,…

The superconducting infinite-layer (IL) nickelates offer a new platform for investigating the long-standing problem of high-temperature superconductivity. Many models were proposed to understand its superconducting mechanisms based on the…

Progress in the study of infinite-layer nickelates has always been highly linked to materials advances. In particular, the recent development of superconductivity via hole-doping was predicated on the controlled synthesis of Ni in a very…

The ambient-pressure superconductivity in $\mathrm{La}_{3}\mathrm{Ni}_{2}\mathrm{O}_{7}$ thin films via compressive epitaxial strain provides a highly accessible platform for diverse characterization techniques, facilitating the studies of…

Superconductivity · Physics 2026-02-11 Maosen Wang , Bo Hao , Wenjie Sun , Shengjun Yan , Shengwang Sun , Hongyi Zhang , Zhengbin Gu , Yuefeng Nie

The discovery of superconductivity in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ [1] introduced a new family of layered nickelate superconductors that has now been extended to include a range of Sr-doping [2, 3], Pr or La in place of Nd [4-6], and the…

Significant magnetic exchange interactions have been observed in infinite-layer nickelates RNiO2 (R = La, Pr, Nd), which exhibit unconventional superconductivity upon hole doping. Despite their structural and Fermi surface similarities to…

Superconductivity · Physics 2025-05-15 Yanbing Zhou , Dan Zhao , Boyun Zeng , Chengliang Xia , Yu Wang , Hanghui Chen , Tao Wu , Xianhui Chen
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