Related papers: Broadband cavity-enhanced ultrafast spectroscopy
Direct frequency-comb spectroscopy is used to probe the absolute frequencies of $6S_{1/2}$-$8S_{1/2}$ two-photon transitions of atomic cesium in hot vapor environment. By utilizing the coherent control method of temporally splitting the…
A theoretical model of the influence of detection bandwidth properties on observed line shapes in laser absorption spectroscopy is described. The model predicts artificial frequency shifts, extra broadenings and line asymmetries which must…
Processes involving ultrafast laser driven electron-phonon dynamics play a fundamental role in the response of quantum systems in a growing number of situations of interest, as evidenced by phenomena such as strongly driven phase…
High-resolution spectroscopy allows one to probe weak interactions and to detect subtle phenomena. While such measurements are routinely performed on atoms and molecules in the gas phase, spectroscopy of adsorbed species on surfaces is…
Defects in solid-state materials play a central role in determining coherence, stability, and performance in quantum technologies. Although narrowband techniques can probe specific resonances with high precision, a broadband spectroscopic…
A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…
Measuring microcombs in amplitude and phase provides unique insight into the nonlinear cavity dynamics but spectral phase measurements are experimentally challenging. Here, we report a linear heterodyne technique assisted by electro-optic…
Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…
We demonstrate the first cavity-enhanced optical frequency comb spectroscopy in the mid-infrared wavelength region and report the sensitive real-time trace detection of hydrogen peroxide in the presence of a large amount of water. The…
We investigate the limits of intracavity absorption spectroscopy with nonlinear media. Using a common theoretical framework, we compare the detection of a trace gas within an undriven cavity with gain near and above threshold, a driven…
A simple design paradigm for making broad-band ultra-thin plasmonic absorbers is introduced. The absorber's unit cell is composed of sub-units of various sizes, resulting in nearly 100% absorbance at multiple adjacent frequencies and high…
A 20-fold increase over the single path optical absorption is demonstrated with a low loss medium placed in a resonant cavity. This has been applied to laser cooling of Yb:ZBLAN glass resulting in 90% absorption of the incident pump light.…
We have searched for absorption in several common atomic species due to the atmosphere or exosphere of the transiting extrasolar planet HD 209458b, using high precision optical spectra obtained with the Subaru High Dispersion Spectrograph…
A simple perfect absorption structure is proposed to achieve the high efficiency light absorption of monolayer molybdenum disulfide (MoS 2 ) by the critical coupling mechanism of guided resonances. The results of numerical simulation and…
An interleaved, chirped electro-optic dual comb system is demonstrated for rapid, high dynamic range measurements of cavity optomechanical sensors. This approach allows for the cavity displacements to be interrogated at measurement times as…
A tunable diode laser spectrometer has been employed to examine the overtone absorption lines of $^{12}$CH$_4$ in the region around 12780 cm$^{-1}$ (780 nm) at room temperature. The spectrometer sources are commercially available tunable…
In this manuscript, we have demonstrated that the antenna-enhanced infrared vibrational spectroscopy can be a powerful platform for high-sensitivity detection of ultrathin layer of polymer molecules and in situ monitoring of their…
Advances in high-resolution laser spectroscopy have enabled many scientific breakthroughs in physics, chemistry, biology and astronomy. Optical frequency combs have pushed measurement limits with ultrahigh-frequency accuracy and…
We measure the absolute absorption cross section of molecules using a matter-wave interferometer. A nanostructured density distribution is imprinted onto a dilute molecular beam through quantum interference. As the beam crosses the light…
We develop an analytical model to describe sub-bandgap optical absorption in two-dimensional semiconducting transition metal dichalcogenide (s-TMD) nanoflakes. The material system represents an array of few-layer molybdenum disulfide…