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Related papers: Ultrafast Dynamics of Gallium Vacancy Charge State…

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Gallium selenide (GaSe) is a 2D material with a thickness-dependent gap, strong non-linear optical coefficients and uncommon interband optical selection rules, making it interesting for optoelectronic and spintronic applications. In this…

Materials Science · Physics 2017-06-15 Alaric Bergeron , John Ibrahim , Richard Leonelli , Sébastien Francoeur

Understanding excited carrier dynamics in semiconductors is crucial for the development of photovoltaics and efficient photonic devices. However, overlapping spectral features in optical/NIR pump-probe spectroscopy often render assignments…

Recently reported remarkably high radiation tolerance of $\gamma$/$\beta$-Ga$_2$O$_3$ double-polymorphic structure brings this ultrawide bandgap semiconductor to the frontiers of power electronics applications that are able to operate in…

Materials Science · Physics 2024-09-25 Ru He , Junlei Zhao , Jesper Byggmästar , Huan He , Flyura Djurabekova

In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…

Strongly Correlated Electrons · Physics 2019-05-29 Chen-Yen Lai , Jian-Xin Zhu

Ultrafast electron diffraction/microscopy technique enables us to investigate the nonequilibrium dynamics of crystal structures in the femtosecond-nanosecond time domain. However, the electron diffraction intensities are in general…

Materials Science · Physics 2024-07-10 Toshiya Shiratori , Jumpei Koga , Takahiro Shimojima , Kyoko Ishizaka , Asuka Nakamura

We use density-matrix theory to calculate the ultrafast dynamics of unconventional superconductors from a microscopic viewpoint. We calculate the time evolution of the optical conductivity as well as pump-probe spectra for a d-wave order…

Superconductivity · Physics 2009-11-13 J. Unterhinninghofen , D. Manske , A. Knorr

One of the basic optoelectronic characteristics is the absorption of any optoelectronic device or material. We present the characteristics of pure GaAs and the deviation of ideal spectra. Due to crystal defects, vacancies, impurities, etc.,…

Materials Science · Physics 2024-01-17 Subarna Alam , Mohammad Jahangir Alam

Plasmonic crystals are well known to have band structure including a bandgap, enabling the control of surface plasmon propagation and confinement. The band dispersion relation of bulk crystals has been generally measured by…

Photoinduced non-thermal phase transitions are new paradigms of exotic non-equilibrium physics of strongly correlated materials. An ultrashort optical pulse can drive the system to a new order through complex microscopic interactions that…

Defect energy formation, lattice distortions and electronic structure of cubic In2O3 with Sn, Ga and O impurities were theoretically investigated using density functional theory. Different types of point defects, consisting of 1 to 4 atoms…

Mesoscale and Nanoscale Physics · Physics 2020-02-06 Alexandr I. Cocemasov , Vladimir I. Brinzari , Denis L. Nika

Ultrafast imaging is essential in physics and chemistry to investigate the femtosecond dynamics of nonuniform samples or of phenomena with strong spatial variations. It relies on observing the phenomena induced by an ultrashort laser pump…

Optics · Physics 2021-02-11 Chen Xie , Remi Meyer , Luc Froehly , Remo Giust , Francois Courvoisier

One-dimensional (1D) metal-dielectric (MD) periodic structures take advantage of large refractive index contrast between metal and dielectrics to invoke extremely high nonlinear ultrafast responses of metal. These structures are also…

Ta$_{3}$N$_{5}$ is among the most intensively studied photoanode materials for solar-driven water oxidation, yet its performance often remains limited by short carrier lifetimes and defect mediated recombination. Although transient…

Gallium oxide is a novel advanced material gaining increasing attention for its unique combination of functional properties. It forms in several phases or polymorphs - {\alpha}, {\beta}, {\gamma}, and {\kappa} - having variable properties…

The relationship between the pseudogap and superconductivity remains a central puzzle in the physics of cuprates. Hydrostatic pressure provides a clean tuning parameter free from chemical disorder, yet probing the microscopic energy scales…

Many linked processes occur concurrently in strongly excited semiconductors, such as interband and intraband absorption, scattering of electrons and holes by the heated lattice, Pauli blocking, bandgap renormalization and the formation of…

Supercontinua are broadband spectra that are essential to optical spectroscopy, sensing, imaging, and metrology. They are generated from ultrashort laser pulses through nonlinear frequency conversion in fibers, bulk media, and…

Defects are crucial in determining a variety of material properties especially in low dimensions. In this work, we study point defects in monolayer alpha-phase Ruthenium (III) chloride (alpha-RuCl3), a promising candidate to realize quantum…

Materials Science · Physics 2023-05-31 Wenqi Yang , Linghan Zhu , Yan Lu , Erik Henriksen , Li Yang

Ultrafast phenomena on a femtosecond timescale are commonly examined by pump-probe experiments. This implies multiple measurements where the sample under investigation is pumped with a short light pulse and then probed with a second pulse…

$\beta$-Ga$_2$O$_3$ is an ultra-wide bandgap semiconductor and is thus expected to be optically transparent to light of sub-bandgap wavelengths well into the ultraviolet. Contrary to this expectation, it is found here that free electrons in…