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In the first order of perturbation theory, the total energy of a diatomic molecule in the ground state is calculated taking into account the Pauli principle and plasma oscillations of atomic electrons. The Fourier component of the potential…

Mesoscale and Nanoscale Physics · Physics 2021-12-15 V. P. Koshcheev , Yu. N. Shtanov

The physical aspect of a general perturbation theory is explored. Its role as a physical principle for understanding the interaction among the matters with different levels of hierarchy is appreciated. It is shown that the general…

Chemical Physics · Physics 2007-05-23 Liqiang Wei

The physical aspect of a general perturbation theory is explored. Its role as a physical principle for understanding the interaction among matter with different levels of hierarchy is appreciated. It is shown that the generic perturbation…

Chemical Physics · Physics 2007-05-23 Liqiang Wei

An effective method for the quantitative description of the electronic excited states of polyatomic systems is developed by using computer technology. The proposed method allows calculating various properties of matter at the atomic level…

Atomic Physics · Physics 2016-02-22 A. V. Popov

This article covers few selected aspects of quantum theory of molecular rotations and vibrations. Triatomic molecules are the simplest systems, which show qualitative characteristics of larger polyatomic molecules. On the minimal example of…

Chemical Physics · Physics 2022-03-18 Emil J. Zak

Second order perturbative corrections to electron wavefunction are calculated here at generalized temperature, for the first time. This calculation is important to prove the renormalizeability of QED through order by order cancellation of…

High Energy Physics - Phenomenology · Physics 2015-05-28 Mahnaz Q. Haseeb , Samina S. Masood

Shaped laser pulses are a powerful tool to induce population transfer between electronic molecular states, and time-dependent perturbation theory is suitable for a description of such a transfer in weak external fields. The application of…

Mathematical Physics · Physics 2012-05-24 Klaus Renziehausen

In this perspective, we discuss where and how accounting for electronic many-body polarization affects the accuracy of classical molecular dynamics simulations of biomolecules.While the effects of electronic polarization are highly…

Chemical Physics · Physics 2021-03-29 Josef Melcr , Jean-Philip Piquemal

This article continues the series of works by the authors on the approximation of the electronic terms of diatomic molecules by the Morse formula, which is the simplest anharmonic approximation of the real term U(r). Depending on the choice…

Chemical Physics · Physics 2024-11-22 G. S. Denisov , R. E. Asfin

An algorithm, based on numerical description of the terms of many-body perturbation theory (Goldstone diagrams), is presented. The algorithm allows the use of the same piece of computer code to evaluate any particular diagram in any…

Atomic Physics · Physics 2015-05-13 V. A. Dzuba

Low-order perturbation corrections to the electronic grand potential, internal energy, chemical potential, and entropy of a gas of noninteracting, identical molecules at a nonzero temperature are determined numerically as the…

Chemical Physics · Physics 2019-10-21 Punit K. Jha , So Hirata

Based on the special properties of Liouville eigenoperators a perturbation theory for the partition sum is given. It is applicable for any temperature and includes the case of degenerate Hamiltonians. To demonstrate the reliability of the…

Strongly Correlated Electrons · Physics 2007-05-23 R. Schumann

A very efficient large-order perturbation theory is formulated for the nuclear motion of a linear triatomic molecule. To demonstrate the method, all of the experimentally observed rotational energies, with values of $J$ almost up to 100,…

Chemical Physics · Physics 2009-10-30 Andrei A. Suvernev , David Z. Goodson

The exact wave functions, which describe the states of an electron, bound in the image potential, and the magnetic field, which is perpendicular to surface of a metal, are obtained. The correction terms to the energy of an electron in the…

Quantum Physics · Physics 2015-02-24 P. A. Golovinski , M. A. Preobrazhenskiy

We study a general problem of the translational/rotational/vibrational/electronic dynamics of a diatomic molecule exposed to an interaction with an arbitrary external electromagnetic field. The theory developed in this paper is relevant to…

Quantum Physics · Physics 2016-09-28 Milan Sindelka , Nimrod Moiseyev

In the development of equations of state for polyatomic molecules, thermodynamic perturbation theory (TPT) is widely used to calculate the change in free energy due to chain formation. TPT is a simplification of a more general and exact…

Soft Condensed Matter · Physics 2016-07-13 Bennett D. Marshall

One-dimensional ideal diatomic gas is simulated through possible types of motion of a molecule. Energy of each type of its motion is calculated from theory and numerical method. Calculation of kinetic energy of an atom in…

Chemical Physics · Physics 2014-02-11 Siti Nurul Khotimah , Sparisoma Viridi , Widayani , Abdul Waris

The spectra (rotational, rotation-vibrational or electronic) of diatomic molecules due to transitions involving only closed-shell ($^1\Sigma$) electronic states follow very regular, simple patterns and their theoretical analysis is usually…

Chemical Physics · Physics 2016-05-10 Jonathan Tennyson , Lorenzo Lodi , Laura K. McKemmish , Sergei N Yurchenko

Within density-functional theory, perturbation theory~(PT) is the state-of-the-art formalism for assessing the response to homogeneous electric fields and the associated material properties, e.g., polarizabilities, dielectric constants, and…

The ion-electron coupling properties for a ion impurity in an electron gas and for a two component plasma are carried out on the basis of a regularized electron-ion potential removing the short-range Coulomb divergence. This work is largely…

Statistical Mechanics · Physics 2009-11-07 B Talin , E Dufour , A Calisti , M A Gigosos , M A Gonzalez , T del Rio Gaztelurrutia , J Dufty
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