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A generalized class of ultra-long-range Rydberg molecules is proposed which consist of a multichannel Rydberg atom whose outermost electron creates a chemical bond with a distant ground state atom. Such multichannel Rydberg molecules…

Atomic Physics · Physics 2015-11-11 Matthew T. Eiles , Chris H. Greene

We propose to create superposition states of over 100 Strontium atoms being in a ground state or metastable optical clock state, using the Kerr-type interaction due to Rydberg state dressing in an optical lattice. The two components of the…

Quantum Physics · Physics 2016-08-17 Mohammadsadegh Khazali , Hon Wai Lau , Adam Humeniuk , Christoph Simon

Rydberg atom arrays are a leading platform for quantum computing and simulation, combining strong interactions with highly coherent operations and flexible geometries. However, the achievable fidelities are limited by the finite lifetime of…

Quantum Physics · Physics 2021-08-11 Sam R. Cohen , Jeff D. Thompson

Rydberg atoms with principal quantum number n >> 1 have exaggerated atomic properties including dipole-dipole interactions that scale as n^4 and radiative lifetimes that scale as n^3. It was proposed a decade ago to take advantage of these…

Quantum Physics · Physics 2015-03-13 M. Saffman , T. G. Walker , K. Molmer

Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, ideally combine long coherence times and strong interactions, a key property of quantum systems, in particular for the development of quantum technologies.…

We perform a comparative analysis of different computational approaches employed to explore the electronic structure of ultralong-range Rydberg molecules. Employing the Fermi pseudopotential approach, where the interaction is approximated…

We study spin-phonon coupled dynamics in the vicinity of a sloped conical intersection created by laser coupling the electronic (spin) and vibrational degrees of freedom of a pair of trapped Rydberg ions. We show that the shape of the…

Atomic Physics · Physics 2025-12-05 Abdessamad Belfakir , Weibin Li

Rydberg atoms provide a wide range of possibilities to tailor interactions in a quantum gas. Here we report on Rydberg excitation of Bose-Einstein condensed 87Rb atoms. The Rydberg fraction was investigated for various excitation times and…

Quantum Physics · Physics 2008-01-23 Rolf Heidemann , Ulrich Raitzsch , Vera Bendkowsky , Björn Butscher , Robert Löw , Tilman Pfau

This paper investigates interaction-induced symmetry breaking in circular quantum dots. We explain that the anisotropic static Wigner molecule ground states frequently observed in simulations are created by interference effects that occur…

Strongly Correlated Electrons · Physics 2024-10-03 Andres Perez Fadon , Gino Cassella , Halvard Sutterud , W. M. C. Foulkes

We study a driven-dissipative system of atoms in the presence of laser excitation to a Rydberg state and spontaneous emission. The atoms interact via the blockade effect, whereby an atom in the Rydberg state shifts the Rydberg level of…

Quantum Gases · Physics 2011-09-14 Tony E. Lee , H. Häffner , M. C. Cross

We study the quantum properties of Rydberg atoms in a magnetic Ioffe-Pritchard trap which is superimposed by a homogeneous electric field. Trapped Rydberg atoms can be created in long-lived electronic states exhibiting a permanent electric…

Atomic Physics · Physics 2007-09-17 Michael Mayle , Bernd Hezel , Igor Lesanovsky , Peter Schmelcher

Non-adiabatic processes near conical intersections are rooted in the stronger coupling between electronic and nuclear degrees of freedom. Using a system of two trapped Rydberg ions, their high polarizability and strong dipolar interactions…

Quantum Physics · Physics 2024-12-04 Manish Chaudhary , Rejish Nath , Weibin Li

Excitons, i.e. the bound states of an electron and a positively charged hole are the solid state analogue of the hydrogen atom. As such they exhibit a Rydberg series, which in cuprous oxide has been observed up to high principal quantum…

Mesoscale and Nanoscale Physics · Physics 2025-11-18 Jan Ertl , Patric Rommel , Jörg Main

The long-range interaction between Rydberg-excited atoms endows a medium with large optical nonlinearity. Here, we demonstrate an optical switch to operate on a single photon from an entangled photon pair under a Rydberg electromagnetically…

Quantum Physics · Physics 2020-11-03 Yi-Chen Yu , Ming-Xin Dong , Ying-Hao Ye , Guang-Can Guo , Dong-Sheng Ding , Bao-Sen Shi

We observe the formation of long-range Cs$_2$ Rydberg molecules consisting of a Rydberg and a ground-state atom by photoassociation spectroscopy in an ultracold Cs gas near 6s$_{1/2}$($F$=3,4)$\rightarrow$np$_{3/2}$ resonances (n=26-34).…

Atomic Physics · Physics 2015-06-23 Heiner Saßmannshausen , Frédéric Merkt , Johannes Deiglmayr

We propose a robust localization of the highly-excited Rydberg atoms, interacting with doughnut-shaped optical vortices. Compared with the earlier standing-wave (SW)-based localization methods, a vortex beam can provide an…

Quantum Physics · Physics 2020-12-30 Ning Jia , Teodora Kirova , Gediminas Juzeliunas , Hamid Reza Hamedi , Jing Qian

Rydberg states of atoms are of great current interest for quantum manipulation of mesoscopic samples of atoms. Long-range Rydberg-Rydberg interactions can inhibit multiple excitations of atoms under the appropriate conditions. These…

Atomic Physics · Physics 2009-11-10 Thad G. Walker , Mark Saffman

We study a novel regime of the Rydberg excitation blockade using highly Stark-shifted, yet long-living, states of Rb atoms subject to electric fields above the classical ionization limit. Such states allow tuning the dipole-dipole…

We report on the formation of ultralong-range Rydberg D-state molecules via photoassociation in an ultracold cloud of rubidium atoms. By applying a magnetic offset field on the order of 10 G and high resolution spectroscopy, we are able to…

The direct observation of non-adiabatic dynamics at conical intersections is a long-standing goal of molecular physics. Novel time-resolved spectroscopies have been proposed which are sensitive to electronic coherences induced by the…

Chemical Physics · Physics 2020-11-16 Simon P. Neville , Albert Stolow , Michael S. Schuurman