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In hybrid improper ferroelectric systems, polarization arises from the onset of successive nonpolar lattice modes. In this work, measurements and modeling were performed to determine the spatial symmetries of the phases involved in the…

Materials Science · Physics 2019-07-03 S. Liu , H. Zhang , S. Ghose , M. Balasubramanian , Zhenxian Liu , S. G. Wang , Y-S. Chen , B. Gao , J. Kim , S. -W. Cheong , T. A. Tyson

We performed factor-group analysis of all phonons in possible monoclinic C2/c and C2 structures of BiMnO3 and compared it with our experimental infrared and Raman spectra. We conclude that the crystal structure is centrosymmetric C2/c in…

Materials Science · Physics 2012-10-10 V. Goian , S. Kamba , M. Savinov , D. Nuzhnyy , F. Borodavka , P. Vanek , A. A. Belik

Ferroelectric materials display exotic polarization textures at the nanoscale that could be used to improve the energetic efficiency of electronic components. The vast majority of studies were conducted in two dimensions on thin films, that…

The structural evolution of epitaxial mono-oriented (i.e. with the c-axis perpendicular to the interface) ferroelectric Pb(Zr0.2,Ti0.8)O3 thin film has been investigated, using high resolution, temperature dependent, X-ray diffraction. The…

Materials Science · Physics 2009-11-13 Pierre-Eymeric Janolin , Bernard Fraisse , Francoise Le Marrec , Brahim Dkhil

Sm$_2$Ti$_2$O$_7$, a member of rare-earth titanate pyrochlores, exhibits dipolar-octupolar antiferromagnetism below $T_N$ = 0.35 K. We observed two ferroelectric transitions at 182 ($T_{FE1}$) and 52 K ($T_{FE2}$), significantly higher than…

Materials Science · Physics 2024-07-30 S. Mukherjee , O. Ivashko , S. Majumdar , A. Kumar , S. Giri

\ We combine density functional theory and molecular dynamics simulations to investigate the impact of Sr concentration and atomic ordering on the structural and ferroelectric properties of (Ba, Sr)TiO$_3$. On one hand, the macroscopic…

Materials Science · Physics 2023-08-28 Aris Dimou , Ankita Biswas , Anna Gruenebohm

Room temperature ferroelectricity is observed in lattice-matched ~18% ScAlN/GaN heterostructures grown by molecular beam epitaxy on single-crystal GaN substrates. The epitaxial films have smooth surface morphologies and high crystallinity.…

During the last fifteen years, multiferroic (MF) research communities have been searching for an alternative room temperature MF material with large magnetoelectric (ME) coupling for possible applications in high density electronic…

Pyrochlore dielectric materials such as (Bi$_{1.5}$Zn$_{0.5}$)(Nb$_{1.5}$Zn$_{0.5}$)O$_7$ (BZN) have generated interest because they combine high dielectric constants with small dielectric loss tangents and yet are cubic at all…

Materials Science · Physics 2007-05-23 Ram Seshadri

Mixed-anion compounds, which incorporate multiple types of anions into materials, displays tailored crystal structures and physical/chemical properties, garnering immense interests in various applications such as batteries, catalysis,…

Local structural symmetries play a key role in the functionalities of ferroelectric materials and are often found different from average symmetry. Here, we study the real space nanoscale structure in Pb-free BaZr$_{x}$Ti$_{1-x}$O$_{3}$ (x…

In the framework of Landau--Ginzburg--Devonshire (LGD) phenomenological theory, the influence of misfit strains, surface energy, and finite-size effects on phase diagrams, polar properties, and hysteresis loops has been calculated for…

Materials Science · Physics 2014-07-01 E. A. Eliseev , M. D. Glinchuk , A. N. Morozovska , Ya. V. Yakovenko

Ferroelectric domain walls are a rich source of emergent electronic properties and unusual polar order. Recent studies showed that the configuration of ferroelectric walls can go well beyond the conventional Ising-type structure. N\'eel-,…

Polytypes of tetralayer graphene (TLG: Bernal, rhombohedral and mixed stacking) are crystalline structures with different symmetries. Among those, mixed-stacking tetralayers lack inversion symmetry, which allows for intrinsic spontaneous…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Patrick Johansen Sarsfield , Aitor Garcia-Ruiz , Vladimir I. Fal'ko

Ba{[Gax,Tax]Ti(1-2x)}O3 ceramics with x equal to 0, 0.0025, 0.005, 0.01, 0.025 and 0.05 have been prepared by conventional solid-state reaction. Structural and dielectric characterization have been performed to investigate the effect of…

The recent discovery of the spin supersolid candidate Na$_2$BaCo(PO$_4$)$_2$ stimulates numerous research interest on the triangular-lattice transition-metal phosphates. Here we report a comprehensive study on the structural, magnetic and…

Strongly Correlated Electrons · Physics 2024-04-30 Chuandi Zhang , Junsen Xiang , Quanliang Zhu , Longfei Wu , Shanfeng Zhang , Juping Xu , Wen Yin , Peijie Sun , Wei Li , Gang Su , Wentao Jin

Thin films of PbTiO3, a classical ferroelectric, have been grown under tensile strain on single-crystal substrates of DyScO3. The films, of only 5nm thickness, grow fully coherent with the substrate and show no crystallographic twin…

Materials Science · Physics 2009-11-11 G. Catalan , A. Janssens , G. Rispens , S. Csiszar , O. Seeck , G. Rijnders , D. H. A. Blank , B. Noheda

We investigated the electrical conductivity, thermal conductivity and thermopower as a function of Nb content (x) in Ba0.7Eu0.3Ti1-xNbxO3 (x = 0.001- 0.10) in the temperature range T = 400-2 K. The substitution of Nb destabilizes the…

Materials Science · Physics 2018-02-20 KmRubi , R. Mahendiran

The results of the magnetization studies on Pr_{5}Ge_{3}and Tb_{5}Ge_{3} single crystals are reported. Single Crystals of Pr_{5}Ge_{3} and Tb_{5}Ge_{3} compounds were successfully grown by Czochralski method. These compounds crystallize in…

Strongly Correlated Electrons · Physics 2009-11-13 Devang A. Joshi , A. Thamizhavel , S. K. Dhar

We report a detailed high-resolution powder neutron diffraction investigation of the structural behaviour of the multiferroic hexagonal polymorph of YMnO3 between room temperature and 1403 K. The study was aimed at resolving previous…

Materials Science · Physics 2015-05-19 Alexandra S. Gibbs , Kevin S. Knight , Philip Lightfoot