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Spin excitations of magnetoelectric LiNiPO$_4$ are studied by infrared absorption spectroscopy in the THz spectral range as a function of magnetic field through various commensurate and incommensurate magnetically ordered phases up to…

We investigated the spin excitations of magnetoelectric $\text{LiFePO}_4$ by THz absorption spectroscopy in magnetic fields up to 33$\,$T. By studying their selection rules, we found not only magnetic-dipole, but also electric-dipole active…

Low-energy magnon excitations in magnetoelectric LiFePO$_4$ have been investigated by high-frequency high-field electron spin resonance spectroscopy in magnetic fields up to B = 58 T and frequencies up to f = 745 GHz. For magnetic fields…

Strongly Correlated Electrons · Physics 2021-05-06 J. Werner , C. Neef , C. Koo , A. Ponomaryov , S. Zvyagin , R. Klingeler

Inelastic neutron scattering (INS) experiments were performed to investigate the spin dynamics in magnetoelectric effect (ME) LiCoPO$_4$ single crystals. Weak dispersion was detected in the magnetic excitation spectra along the three…

Strongly Correlated Electrons · Physics 2013-08-14 Wei Tian , Jiying Li , Jeffrey W. Lynn , Jerel L. Zarestky , David Vaknin

Magnetic excitations are investigated for a hexagonal polar magnet Fe2Mo3O8 by terahertz spectroscopy. We observed magnon modes including an electric-field active magnon, electromagnon, in the collinear antiferromagnetic phase with spins…

Strongly Correlated Electrons · Physics 2017-01-09 T. Kurumaji , Y. Takahashi , J. Fujioka , R. Masuda , H. Shishikura , S. Ishiwata , Y. Tokura

We studied spin excitations of the multiferroic Ba2CoGe2O7 in high magnetic fields up to 33 T. In the electron spin resonance and far infrared absorption spectra we found several spin excitations beyond the two conventional magnon modes…

Strongly Correlated Electrons · Physics 2012-08-27 K. Penc , J. Romhányi , T. Rõõm , U. Nagel , Á. Antal , T. Fehér , A. Jánossy , H. Engelkamp , H. Murakawa , Y. Tokura , D. Szaller , S. Bordács , I. Kézsmárki

Temperature (5--250 K) and magnetic field (0--70 kOe) variations of the low-energy (1--10 meV) electrodynamics of spin excitations have been investigated for a complete set of light-polarization configurations for a ferroelectric magnet…

Materials Science · Physics 2009-11-13 N. Kida , Y. Ikebe , Y. Takahashi , J. P. He , Y. Kaneko , Y. Yamasaki , R. Shimano , T. Arima , N. Nagaosa , Y. Tokura

Elastic and inelastic neutron scattering studies reveal details of the antiferromagnetic tansition and intriguing spin-dynamics in the magneto-electric effect single crystal LiMnPO$_4$. The elastic scattering studies confirm the system is…

Strongly Correlated Electrons · Physics 2015-05-13 Jiying Li , Wei Tian , Ying Chen , Jerel L. Zarestky , Jeffrey W. Lynn , David Vaknin

We report the magnetic field dependence of the THz absorption and non-reciprocal directional dichroism spectra of BiFeO$_3$ measured on the three principal crystal cuts for fields applied along the three principal directions of each cut.…

Strongly Correlated Electrons · Physics 2021-12-01 D. G. Farkas , D. Szaller , I. Kézsmárki , U. Nagel , T. Rõõm , L. Peedu , J. Viirok , J. S. White , R. Cubitt , T. Ito , R. S. Fishman , S. Bordács

Antiferromagnetic (AFM) materials are considered as promising building blocks of novel data storage devices, still, detecting and manipulating AFM domains have remained challenging. Here, we demonstrate that the two antiphase domains of the…

Materials Science · Physics 2026-03-13 B. Tóth , V. Kocsis , Y. Tokunaga , Y. Taguchi , Y. Tokura , S. Bordács

Magnetic and magnetoelectric excitations in the multiferroic TbMnO_3 have been investigated at terahertz frequencies. Using different experimental geometries we can clearly separate the electro-active excitations (electromagnons) from the…

Strongly Correlated Electrons · Physics 2009-03-16 A. Pimenov , A. Shuvaev , A. Loidl , F. Schrettle , A. A. Mukhin , V. D. Travkin , V. Yu. Ivanov , A. M. Balbashov

Spin excitations were studied by absorption spectroscopy in CaBaCo4O7 which is a type-I multiferroic compound with the largest magnetic-order induced ferroelectric polarization ({\Delta}P=17mC/m2) reported, so far. We observed two optical…

Strongly Correlated Electrons · Physics 2016-01-05 S. Bordács , V. Kocsis , Y. Tokunaga , U. Nagel , T. Rõõm , Y. Takahashi , Y. Taguchi , Y. Tokura

We study the spin-dependent electronic excitations in alkali-metal nanoparticles. Using numerical and analytical approaches, we focus on the resonances in the response to spin-dependent dipole fields. In the spin-dipole absorption spectrum…

Mesoscale and Nanoscale Physics · Physics 2009-09-18 Yue Yin , Paul-Antoine Hervieux , Rodolfo A. Jalabert , Giovanni Manfredi , Emmanuel Maurat , Dietmar Weinmann

Magnetic structures are investigated by means of neutron diffraction to shine a light on the intricate details that are believed to be key to understanding the magnetoelectric effect in LiCoPO$_4$ . At zero field, a spontaneous spin canting…

Li-based phosphates are paradigmatic materials for magnetoelectricity. By means of first-principles calculations, we elucidate the microscopic origin of spin anisotropy and of magnetoelectric effects in LiNiPO4. The comparison with LiCoPO4…

Materials Science · Physics 2015-05-14 Kunihiko Yamauchi , Silvia Picozzi

We present the electron spin resonance study of the influence of an electric field on the low-field multiferroic magnetic state in LiCuVO4. The shift of the magnetic resonance spectra in the electric field has been observed experimentally.…

Strongly Correlated Electrons · Physics 2021-12-22 S. K. Gotovko , V. I. Marchenko , A. Prokofiev , L. E. Svistov

We show that strong electromagnon peaks can be found in absorption spectra of non-collinear magnets exhibiting a linear magnetoelectric effect. The frequencies of these peaks coincide with the frequencies of antiferromagnetic resonances and…

Materials Science · Physics 2009-07-20 M. A. van der Vegte , C. P. van der Vegte , M. Mostovoy

The angular and temperature dependences of single crystal ESR spectra at X-band frequency of quasi 1D spin 1/2 antiferromagnetic zigzag chain system {\beta}-TeVO4 are reported. Two resonance components in the ESR spectrum have been…

Strongly Correlated Electrons · Physics 2013-11-25 Yu. Savina , A. Bludov , V. Pashchenko , S. Gnatchenko , A. Stepanov , P. Lemmens

We report our combined experimental and theoretical study of magnetoelectric properties of an antiferromagnet Sr(TiO)Cu$_4$(PO$_4$)$_4$, in comparison with the isostructurals Ba(TiO)Cu$_4$(PO$_4$)$_4$ and Pb(TiO)Cu$_4$(PO$_4$)$_4$. The…

Magnetoelectric, dielectric and magnetic susceptibility tensors of multiferroic TbMnO3 with cycloidal antiferromagnetic structure in external electric and magnetic fields have been investigated with taking into account dynamics of spin,…

Materials Science · Physics 2013-04-17 Igor V. Bychkov , Dmitry A. Kuzmin , Sergey J. Lamekhov , Vladimir G. Shavrov
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