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Related papers: Lattice and Electronic properties of VO$_2$ with t…

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Results of first principles augmented spherical wave electronic structure calculations for niobium dioxide are presented. Both metallic rutile and insulating low-temperature NbO2, which crystallizes in a distorted rutile structure, are…

Strongly Correlated Electrons · Physics 2009-11-07 V. Eyert

VO2 features concomitant structural and metal-insulator transitions. This poses a challenge for understanding the underlying mechanism: is the transition triggered by a structural or by an electronic instability? The two scenarios are…

The quantum phase transition between a repulsive Luttinger liquid and an insulating Peierls state is studied in the framework of the one-dimensional spinless Holstein model. We focus on the adiabatic regime but include the full quantum…

Strongly Correlated Electrons · Physics 2011-03-08 Martin Hohenadler , Holger Fehske , Fakher F. Assaad

VO2 is renowned for its electric transition from an insulating monoclinic (M1) phase characterized by V-V dimerized structures, to a metallic rutile (R) phase above 340 Kelvin. This transition is accompanied by a magnetic change: the M1…

Materials Science · Physics 2023-10-10 Yubo Zhang , Da Ke , Junxiong Wu , Chutong Zhang , Baichen Lin , Zuhuang Chen , John P. Perdew , Jianwei Sun

We present a technique to calculate the transport properties through one-dimensional models of molecular wires. The calculations include inelastic electron scattering due to electron-lattice interaction. The coupling between the electron…

Condensed Matter · Physics 2009-10-31 H. Ness , S. A. Shevlin , A. J. Fisher

We present a spectroscopic study that reveals that the metal-insulator transition of strained VO$_2$ thin films may be driven towards a purely electronic transition, which does not rely on the Peierls dimerization, by the application of…

The importance of electronic correlation effects in the layered perovskite Sr$_2$RuO$_4$ is evidenced. To this end we use state-of-the-art LDA+DMFT (Local Density Approximation + Dynamical Mean-Field Theory) in the basis of Wannier…

Strongly Correlated Electrons · Physics 2007-05-23 Z. V. Pchelkina , I. A. Nekrasov , Th. Pruschke , A. Sekiyama , S. Suga , V. I. Anisimov , D. Vollhardt

Copper borate Cu$_3$(BO$_3$)$_2$ is a complex compound with a layered crystallographic structure in which the Jahn-Teller active and magnetic copper Cu$^{2+}$ ions occupy sixteen nonequivalent positions in the unit cell displaying…

The popular dual electronic (Mott) and structural (Peierls) transitions in VO2 are explored using x-ray absorption spectromicroscopy with high spatial and spectral resolutions. It is found that during both heating and cooling, the…

Strongly Correlated Electrons · Physics 2015-11-20 Suhas Kumar , John Paul Strachan , Matthew D. Pickett , Alexander Bratkovsky , Yoshio Nishi , R. Stanley Williams

We have investigated the charge dynamics of VO2 by optical reflectivity measurements. Optical conductivity clearly shows a metal-insulator transition. In the metallic phase, a broad Drude-like structure is observed. On the other hand, in…

Strongly Correlated Electrons · Physics 2009-11-11 K. Okazaki , S. Sugai , Y. Muraoka , Z. Hiroi

A theory of the metal-insulator transition in vanadium dioxide from the high-temperature rutile to the low- temperature monoclinic phase is proposed on the basis of cluster dynamical mean field theory, in conjunction with the density…

Strongly Correlated Electrons · Physics 2009-11-10 S. Biermann , A. Poteryaev , A. I. Lichtenstein , A. Georges

Heterostructuring provides different ways to manipulate the orbital degrees of freedom and to tailor orbital occupations in transition metal oxides. However, the reliable prediction of these modifications remains a challenge. Here, we…

Strongly Correlated Electrons · Physics 2022-04-27 P. Radhakrishnan , B. Geisler , K. Fürsich , D. Putzky , Y. Wang , G. Christiani , G. Logvenov , P. Wochner , P. A. van Aken , R. Pentcheva , E. Benckiser

Using density functional theory we investigate the lattice instability and electronic structure of recently discovered ferroelectric metal LiOsO$_3$. We show that the ferroelectric-like lattice instability is related to the Li-O distortion…

Materials Science · Physics 2015-03-19 Gianluca Giovannetti , Massimo Capone

We investigate the electronic structure of Sr$_2$FeMoO$_6$ combining photoemission spectroscopy with a wide range of photon energies and electronic structure calculations based on first-principle as well as model Hamiltonian approaches to…

Strongly Correlated Electrons · Physics 2007-05-23 Sugata Ray , Priya Mahadevan , Ashwani Kumar , D. D. Sarma , R. Cimino , M. Pedio , L. Ferrari , A. Pesci

The metal-insulator transition (MIT) in paramagnetic VO2 is studied within LDA+DMFT(IPT), which merges the local density approximation (LDA) with dynamical mean field theory (DMFT). With a fixed value of the Coulomb U=5.0eV, we show how the…

Strongly Correlated Electrons · Physics 2007-05-23 M. S. Laad , L. Craco , E. Müller-Hartmann

Using soft x-ray angle-resolved photoemission spectroscopy we probed the bulk electronic structure of Td MoTe2. We found that on-site Coulomb interaction leads to a Lifshitz transition, which is essential for a precise description of the…

Strongly Correlated Electrons · Physics 2018-09-27 N. Xu , Z. W. Wang , A. Magrez , P. Bugnon , H. Berger , C. E. Matt , V. N. Strocov , N. C. Plumb , M. Radovic , E. Pomjakushina , K. Conder , J. H. Dil , J. Mesot , R. Yu , H. Ding , M. Shi

We investigate the vibrational properties of VO2, particularly the low temperature M1 phase by first-principles calculations using the density functional theory as well as Raman spectroscopy. We perform the structural optimization using…

The electron-phonon interaction is of central importance for the electrical and thermal properties of solids, and its influence on superconductivity, colossal magnetoresistance, and other many-body phenomena in correlated-electron materials…

Using a first-principles approach based on density functional theory and dynamical mean field theory, we study the electronic properties of a new candidate polar metal SrEuMo$_2$O$_6$. Its electronic structure shares similarities with…

Strongly Correlated Electrons · Physics 2015-07-02 Gianluca Giovannetti , Danilo Puggioni , James M. Rondinelli , Massimo Capone

Recently, rutile RuO$_2$ has raised interest for its itinerant antiferromagnetism, crystal Hall effect, and strain-induced superconductivity. Understanding and manipulating these properties demands resolving the electronic structure and the…