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The phase behaviour of room-temperature ionic liquids (ILs) confined in disordered porous media is studied using a theoretical approach that combines an extension of scaled particle theory, Wertheim's thermodynamic perturbation theory, and…

Soft Condensed Matter · Physics 2025-03-12 T. Hvozd , T. Patsahan , O. Patsahan , Yu. Kalyuzhnyi , M. Holovko

Molecular dynamics simulations are a powerful tool to study diffusion processes in battery electrolyte and electrode materials. From a single molecular dynamics simulation many properties relevant to diffusion can be obtained, including the…

Chemical Physics · Physics 2018-07-09 Niek J. J. de Klerk , Eveline van der Maas , Marnix Wagemaker

Ionic liquids (ILs) gain much interest as possible electrolytes in the next generation of mixed-solid Li-ion batteries. However, such properties of ionic liquids as melting transition, diffusion, strength and structure of hydrogen bond…

Ionic liquids (ILs) are an exciting class of electrolytes finding applications in many areas from energy storage to solvents, where they have been touted as ``designer solvents'' as they can be mixed to precisely tailor the physiochemical…

Molecular dynamics simulations have been performed on pure liquid water, aqueous solutions of sodium chloride, and polymer solutions exposed to a strong external electric field with the goal to gain molecular insight into the structural…

Soft Condensed Matter · Physics 2016-08-08 I. Nezbeda , J. Jirsák , F. Moučka , W. R. Smith

Aqueous solid-liquid interfaces (SLI) are ubiquitous in nature and technology, often hosting molecular-level processes with macroscopic consequences. Molecular dynamics (MD) simulations offer a tool of choice to investigate interfacial…

Soft Condensed Matter · Physics 2025-08-12 Mahdi Tavakol , Kislon Voïtchovsky

The fundamental understanding of intermolecular interactions of ionic liquids with water represents a vital extent in predicting ionic liquid properties. Intermolecular or noncovalent interactions were studied for 1,3-dimethyl imidazolium…

Chemical Physics · Physics 2022-06-14 Oleg N. Starovoytov

Simulating liquid water to an accuracy that matches its wealth of available experimental data requires both precise electronic structure methods and reliable sampling of nuclear (quantum) motion. This is challenging because applying the…

Calorimetric determination of enthalpies of mixing ($\Delta$H$_{\rm mix}$) of multicomponent molten salts often employs empirical models that lack parameters with clear physical interpretation (e.g., coordination numbers, molar volumes, and…

In inertial confinement fusion (ICF), the dynamics of plasma mixing in hohlraums critically influence laser-plasma instabilities (LPI) and implosion performance. This study investigates the mixing of hohlraum ablated Au plasmas and filling…

Plasma Physics · Physics 2025-08-22 Xiaoran Li , Jie Qiu , Shuqing Zhang , Liang Hao , Shiyang Zou

This work describes the behaviour of water molecules in 1-butyl-3-methylimidazolium tetrafluoroborate ionic liquid under nanoconfinement between graphene sheets. By means of molecular dynamics simulations, an adsorption of water molecules…

Among other improvements, the Martini 3 coarse-grained force field provides a more accurate description of the solvation of protein pockets and channels through the consistent use of various bead types and sizes. Here, we show that the…

Soft Condensed Matter · Physics 2022-07-27 Balázs Fábián , Sebastian Thallmair , Gerhard Hummer

We study ionic liquids composed 1-alkyl-3-methylimidazolium cations and bis(trifluoromethyl-sulfonyl)imide anions ([C$_n$MIm][NTf$_2$]) with varying chain-length $n\!=\!2, 4, 6, 8$ by using molecular dynamics simulations. We show that a…

Soft Condensed Matter · Physics 2017-11-13 Benjamin Golub , Jan Neumann , Lisa-Marie Odebrecht , Ralf Ludwig , Dietmar Paschek

We develop a theory for the description of ionic liquids (ILs) confined in a porous medium formed by a matrix of immobile randomly placed uncharged particles. The IL is modelled as an electroneutral mixture of hardsphere anions and flexible…

Soft Condensed Matter · Physics 2024-07-03 T. Hvozd , T. Patsahan , Yu. Kalyuzhnyi , O. Patsahan , M. Holovko

Understanding of the molecular interaction between asphaltenes and other molecules, which may act as its solvents, provides insights into the nature of its stability in petroleum fluids and its phase transitions. Molecular dynamics…

Chemical Physics · Physics 2019-07-04 Salah Yaseen , G. Ali Mansoori

The standard model of enhanced ionic conductivities in solid electrolyte heterostructures follows from a continuum mean-field description of defect distributions that makes no reference to crystalline structure. To examine ionic transport…

Materials Science · Physics 2015-06-18 Benjamin J. Morgan , Paul A. Madden

Molecular dynamics simulations of ultrathin water film confined between atomically flat rigid diamond plates are described. Films with thickness of one and two molecular diameters are concerned and TIP4P model is used for water molecules.…

Statistical Mechanics · Physics 2009-03-25 A. V. Khomenko , N. V. Prodanov

A simulation study is performed to investigate the dynamics of coupled Langmuir waves (LWs) and ion-acoustic waves (IAWs) in an unmagnetized plasma. The effects of dispersion due to charge separation and the density nonlinearity associated…

Plasma Physics · Physics 2010-04-29 S. Banerjee , A. P. Misra , P. K. Shukla , L. Rondoni

We investigate nanoflows through dilute disordered media by means of joint lattice Boltzmann (LB) and molecular dynamics (MD) simulations -- when the size of the obstacles is comparable to the size of the flowing particles -- for randomly…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 J. Russo , J. Horbach , F. Sciortino , S. Succi

We propose a simplified version of local molecular field (LMF) theory to treat Coulomb interactions in simulations of ionic fluids. LMF theory relies on splitting the Coulomb potential into a short-ranged part that combines with other…

Statistical Mechanics · Physics 2009-11-13 Natalia A. Denesyuk , John D. Weeks