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Advanced theoretical techniques that combine the linearized coupled-cluster method, configuration interaction method, and perturbation theory are used to calculate energy levels, ionization potentials, electron affinities, field isotope…

Atomic Physics · Physics 2025-08-05 V. A. Dzuba , V. V. Flambaum , G. K. Vong

Fully numerical mesh solutions of 2D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of atoms and…

Atomic Physics · Physics 2015-06-26 Mikhail V. Ivanov , Peter Schmelcher

We revisited the electronic structure parameters used to interpret the hyperfine structure of neutral polonium. We used a computational scheme that treats relativistic and high-order electronic correlation effects within the coupled cluster…

Atomic Physics · Physics 2024-03-08 Leonid V. Skripnikov , Anatoly E. Barzakh

Based upon elements of the modern Pseudoanalytic Function Theory, we analyse a new method for numerically approaching the solution of the Dirichlet boundary value problem, corresponding to the two-dimensional Electrical Impedance Equation.…

Mathematical Physics · Physics 2012-02-23 M. P. Ramirez T. , C. M. A. Robles G. , R. A. Hernandez-Becerril

We proposed a distributed approximating functional method for efficiently describing the electronic dynamics in atoms and molecules in the presence of the Coulomb singularities, using the kernel of a grid representation derived by using the…

Computational Physics · Physics 2016-04-05 Zhigang Sun

Novel equations for the electric dipole polarizability $\alpha_{_{E1}}$ of low-lying excited states in atomic nuclei -- and the related $(-2)$ moment of the total photo-absorption cross section, $\sigma_{_{-2}}$ -- are inferred in terms of…

Nuclear Theory · Physics 2024-03-12 José Nicolás Orce , Cebo Ngwetsheni

A simple method of variational calculations of the electronic structure of a two-electron atom/ion, primarily near the nucleus, is proposed. The method as a whole consists of a standard solution of a generalized matrix eigenvalue equation,…

Atomic Physics · Physics 2024-10-08 Evgeny Z. Liverts

We relax the usual diagonal constraint on the matrix representation of the eigenvalue wave equation by allowing it to be tridiagonal. This results in a larger solution space that incorporates an exact analytic solution for the non-central…

Chemical Physics · Physics 2009-11-13 A. D. Alhaidari

This study proposes an approach toward the first principles electronic structure calculation with the aid of symbolic-numeric solving. The symbolic computation enables us to express the Hartree-Fock-Roothaan equation and the molecular…

Symbolic Computation · Computer Science 2013-02-26 Akihito Kikuchi

We present a highly accurate method for solving single-active-electron (SAE) atomic eigenset in momentum space. The trouble of Coulomb kernel singularity is bypassed with numerical quadrature, which is simple but effective. The complicated…

Quantum Physics · Physics 2017-06-20 Shih-Da Jheng , Tsin-Fu Jiang

We study the interesting problem of interaction and identification of the hadronic molecules which seem to be deuteron-like structure. In particular, we propose a binding mechanism in which One Boson Exchange Potential plus Yukawa…

High Energy Physics - Phenomenology · Physics 2018-07-10 D. P. Rathaud , Ajay Kumar Rai

In (relativistic) electronic structure methods, the quaternion matrix eigenvalue problem and the linear response (Bethe-Salpeter) eigenvalue problem for excitation energies are two frequently encountered structured eigenvalue problems.…

Chemical Physics · Physics 2021-12-01 Zhendong Li

Vertical stacking of two-dimensional (2D) crystals, such as graphene and hexagonal boron nitride, has recently lead to a new class of materials known as van der Waals heterostructures (vdWHs) with unique and highly tunable electronic…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Kirsten Andersen , Simone Latini , Kristian S. Thygesen

Gausslets are one of the few basis constructions for electronic structure that combine locality, orthonormality, variable resolution, and an accurate diagonal approximation for the electron-electron interaction, but the original…

Chemical Physics · Physics 2026-05-07 Steven R. White

We propose a novel numerical algorithm for computing the electronic structure related eigenvalue problem of incommensurate systems. Unlike the conventional practice that approximates the system by a large commensurate supercell, our…

Numerical Analysis · Mathematics 2019-03-27 Yuzhi Zhou , Huajie Chen , Aihui Zhou

Using the Wentzel-Kramers-Brillouin method, we derive a modified form of the Thomas-Fermi approximation to electron density. This new result enables us to calculate the details of the self-consistent ion cores, as well as the ionization…

Materials Science · Physics 2009-02-23 Gregory C. Dente , Michael L. Tilton

We present an implicit solvent model for ab initio electronic structure calculations which is fully self-consistent and is based on direct solution of the nonhomogeneous Poisson equation. The solute cavity is naturally defined in terms of…

Computational Physics · Physics 2011-12-07 Jacek Dziedzic , Hatem H. Helal , Chris-Kriton Skylaris , Arash A. Mostofi , Mike C. Payne

The reduced-density-matrix method is an promising candidate for the next generation electronic structure calculation method; it is equivalent to solve the Schr\"odinger equation for the ground state. The number of variables is the same as a…

Strongly Correlated Electrons · Physics 2011-06-27 Maho Nakata , Mituhiro Fukuda , Katsuki Fujisawa

We revisit the three-body problem in quantum mechanics in two and three dimensions, generating both exact eigenvalues and eigenvectors of the Hamiltonian and a series of approximate solutions as calculated with a variety of different…

Recently we proposed an information entropy based method for electronic structure calculations within the density-matrix functional theory(DMFT) (Phys. Rev. Lett. 128, 013001), dubbed as $i$-DMFT. Comments have been raised regarding the…

Quantum Physics · Physics 2022-07-07 Jian Wang , Evert Jan Baerends