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Type-I clathrate solids have attracted significant interest due to their ultralow thermal conductivities and subsequent promise for thermoelectric applications, yet the mechanisms underlying these properties are not well understood. Here,…

Materials Science · Physics 2025-06-30 Dipti Jasrasaria , Timothy C. Berkelbach

Although extensive experimental and theoretical works have been conducted to understand the ballistic and diffusive phonon transport in nanomaterials recently, direct observation of temperature and thermal nonequilibrium of different phonon…

Mesoscale and Nanoscale Physics · Physics 2017-05-17 Tianli Feng , Wenjun Yao , Zuyuan Wang , Jingjing Shi , Chuang Li , Bingyang Cao , Xiulin Ruan

In this study, we use the transient thermal grating optical technique \textemdash a non-contact, laser-based thermal metrology technique with intrinsically high accuracy \textemdash to investigate room-temperature phonon-mediated thermal…

Recent experimental advances probing coherent phonon and electron transport in nanoscale devices at contact have motivated theoretical channel-based analyses of conduction based on the nonequilibrium Green's function formalism. The…

Mesoscale and Nanoscale Physics · Physics 2020-08-12 Prashanth S. Venkataram , Sean Molesky , Juan Carlos Cuevas , Alejandro W. Rodriguez

Understanding lattice dynamics and thermal transport in crystalline compounds with intrinsically low lattice thermal conductivity ($\kappa_L$) is crucial in condensed matter physics. In this work, we investigate the lattice thermal…

Materials Science · Physics 2025-02-26 Jincheng Yue , Yanhui Liu , Jiongzhi Zheng

Phonon modes and their dispersion relations in ultrathin homogenous dielectric membranes are calculated using elasticity theory. The approach differs from the previous ones by a rigorous account of the effect of the film surfaces on the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. Kühn , D. V. Anghel , J. P. Pekola , M. Manninen , Y. M Galperin

We investigate the effect of confinement and orientation on the phonon transport properties of ultra-thin silicon layers of thicknesses between 1 nm-16 nm. We employ the modified valence force field method to model the lattice dynamics and…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Hossein Karamitaheri , Neophytos Neophytou , Hans Kosina

We develop an accurate interlayer pairwise potential derived from the \textit{ab-initio} calculations and investigate the thermal transport of silicene bilayers within the framework of equilibrium molecular dynamics simulations. The…

Materials Science · Physics 2023-11-16 Sapta Sindhu Paul Chowdhury , Appalakondaiah Samudrala , Santosh Mogurampelly

Electron-phonon interactions play a key role in many branches of solid-state physics. Here, our focus is on the transport properties of one-dimensional systems, and we apply efficient real-time matrix-product state methods to compute the…

Strongly Correlated Electrons · Physics 2023-08-21 David Jansen , Fabian Heidrich-Meisner

Surface scattering is the key limiting factor to thermal transport in dielectric crystals as the length scales are reduced or when temperature is lowered. To explain this phenomenon, it is commonly assumed that the mean free paths of heat…

Materials Science · Physics 2017-08-17 Andrea Cepellotti , Nicola Marzari

Recent advances in our understanding of thermal transport in nanocrystalline systems are responsible for the integration of new technologies into advanced energy systems, including thermoelectric refrigeration systems and renewable energy…

Mesoscale and Nanoscale Physics · Physics 2019-08-12 Brian F. Donovan , Ronald J. Warzoha , R. Bharath Venkatesh , Nicholas T. Vu , Jay Wallen , Daeyeon Lee

Perturbative considerations account for the properties of conventional metals, including the range of temperatures where the transport scattering rate is $1/\tau_\text{tr} = 2\pi \lambda T$, where $\lambda$ is a dimensionless strength of…

Strongly Correlated Electrons · Physics 2023-05-16 Chaitanya Murthy , Akshat Pandey , Ilya Esterlis , Steven A. Kivelson

We compute the thermal conductivity of monolayer beryllene using the linearized phonon Boltzmann transport equation with interatomic force constants obtained from \textit{ab-initio} calculations. Monolayer beryllene exhibits an impressive…

Materials Science · Physics 2024-09-10 Sapta Sindhu Paul Chowdhury , Santosh Mogurampelly

Detailed understanding of vibrational heat transfer mechanisms between solids is essential for the efficient thermal engineering and control of nanomaterials. We investigate the frequency dependence of anharmonic scattering and interfacial…

Materials Science · Physics 2014-10-31 K. Sääskilahti , J. Oksanen , J. Tulkki , S. Volz

Boundary scattering in hierarchically disordered nanomaterials is an effective way to reduce the thermal conductivity of thermoelectric materials and increase their performance. In this work we investigate thermal transport in silicon based…

Materials Science · Physics 2019-02-27 Dhritiman Chakraborty , Laura de Sousa Oliveira , Neophytos Neophytou

Indium iodides, which adopt layered or molecular-crystal-like arrangements depending on composition, are expected to exhibit low lattice thermal conductivity because of their heavy constituent atoms and weak In-I bonding. In this work, we…

Materials Science · Physics 2026-01-06 Takuma Shiga , Yoshikazu Mizuguchi , Hiroshi Fujihisa

In this work, we investigate the microscopic mechanisms of anharmonic lattice dynamics and thermal transport in lead-free halide double perovskite Cs2AgBiBr6 from first principles. We combine self-consistent phonon calculations with bubble…

Materials Science · Physics 2024-02-09 Jiongzhi Zheng , Changpeng Lin , Chongjia Lin , Geoffroy Hautier , Ruiqiang Guo , Baoling Huang

We study the intrinsic scattering of phonons by a general quantum degree of freedom, i.e. a fluctuating "field" $Q$, which may have completely general correlations, restricted only by unitarity and translational invariance. From the induced…

Strongly Correlated Electrons · Physics 2023-01-04 Léo Mangeolle , Leon Balents , Lucile Savary

Many crystals, such as lanthanum zirconate (La2Zr2O7), exhibit a flat temperature dependence of thermal conductivity at elevated temperatures. This phenomenon has recently been attributed to the inter-band phonon tunneling (or diffuson)…

Materials Science · Physics 2024-04-30 Hao Zhou , Janak Tiwari , Tianli Feng

Ballistic transport and resonance phenomena are elucidated in the one-dimensional $\alpha$-Fermi-Pasta-Ulam-Tsingou (FPUT) model using an approach of computing thermal response functions. The existence of periodic oscillations in spatially…

Statistical Mechanics · Physics 2022-09-14 Nathaniel Bohm , Patrick K. Schelling