Related papers: Quantum-classical nonadiabatic dynamics of Floquet…
When the coupled electron-nuclear dynamics are subjected to strong Floquet driving, there is a strong breakdown of the Born-Oppenheimer approximation. In this article, we derive a Fokker-Planck equation to describe non-adiabatic molecular…
We present a detailed derivation and numerical tests of a new mixed quantum-classical scheme to deal with non-adiabatic processes. The method is presented as the zero-th order approximation to the exact coupled dynamics of electrons and…
We propose to combine the Floquet formalism for systems in ac fields with the dynamical mean-field theory to study correlated electron systems periodically driven out of equilibrium by external fields such as intense laser light. This…
We present an approach for efficiently simulating strongly damped quantum systems subjected to periodic driving, employing a periodic matrix product operator representation of the influence functional. This representation enables the…
Much recent experimental effort has focused on the realization of exotic quantum states and dynamics predicted to occur in periodically driven systems. But how robust are the sought-after features, such as Floquet topological surface…
We propose mixed quantum-classical equations of motion that unify electronic coherence and phase evolution simultaneously within the exact factorization framework. Our derivation shows that incorporating the second-order electron-nuclear…
Quantum adiabaticity is the evolution of a quantum system that remains close to an instantaneous eigenstate of a time-dependent Hamiltonian. Using Floquet formalism, we derive a rigorous sufficient condition for adiabaticity in closed,…
We consider the dynamics of a two-level system (qubit) driven by strong and short resonant pulses in the framework of Floquet theory. First we derive analytical expressions for the quasienergies and Floquet states of the driven system. If…
We present a novel mixed quantum-classical approach to the coupled electron-nuclear dynamics based on the exact factorization of the electron-nuclear wave function, recently proposed in [A. Abedi, N. T. Maitra, and E. K. U. Gross, Phys.…
Periodically driven quantum systems can be used to realize quantum pumps, ratchets, artificial gauge fields and novel topological states of matter. Starting from the Keldysh approach, we develop a formalism, the Floquet-Boltzmann equation,…
In this manuscript, we introduce an exact expression for the response of a semi-classical two-level quantum system subject to arbitrary periodic driving. Determining the transition probabilities of a two-level system driven by an arbitrary…
With light-matter interaction extending into strong regime, as well as rapid development of laser technology, systems subjecting to a time-periodic perturbation are attracted broad attention. Floquet theorem and Floquet time-independent…
A novel mixed quantum-classical approach to simulating nonadiabatic dynamics of molecules at metal surfaces is presented. The method combines the numerically exact hierarchical equations of motion approach for the quantum electronic degrees…
We develop a Floquet surface hopping (FSH) approach to deal with nonadiabatic dynamics of molecules near metal surfaces subjected to time-periodic drivings from strong light-matter interactions. The method is based on a Floquet classical…
We present an efficient \textit{ab initio} algorithm for quantum dynamics simulations of interacting systems that is based on the conditional decomposition of the many-body wavefunction [Phys. Rev. Lett. 113, 083003 (2014)]. Starting with…
By directly using the probability formulas of quantum trajectories, we construct an auxiliary open quantum system for a periodically driven open quantum system whose dynamics is governed by the Floquet quantum master equation. This…
Periodically driven quantum systems, known as Floquet systems, have been a focus of non-equilibrium physics in recent years, thanks to their rich dynamics. Not only time-periodic systems exhibit symmetries similar to those in spatially…
We aim to give a pedagogic presentation of the open system dynamics of a periodically driven qubit in contact with a temperature bath. We are specifically interested in the thermodynamics of the qubit. It is well known that by combining the…
We present a new formulation of the correlated electron-ion dynamics (CEID) scheme, which systematically improves Ehrenfest dynamics by including quantum fluctuations around the mean-field atomic trajectories. We show that the method can…
We investigate the nonequilibrium dynamics of the $S=1$ quantum spin chain subjected to a time-dependent external drive, where the driving frequency is adiabatically decreased as a function of time (``Floquet adiabatic evolution''). We show…