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We discuss the recently proposed LDA'+DMFT approach providing consistent parameter free treatment of the so called double counting problem arising within the LDA+DMFT hybrid computational method for realistic strongly correlated materials.…

Strongly Correlated Electrons · Physics 2015-06-11 I. A. Nekrasov , N. S. Pavlov , M. V. Sadovskii

The systematic underestimation of band gaps is one of the most fundamental challenges in semilocal density functional theory (DFT). In addition to hindering the application of DFT to predicting electronic properties, the band gap problem is…

Chemical Physics · Physics 2024-08-27 Kyle Bystrom , Stefano Falletta , Boris Kozinsky

The electronic structure of selected rare-earth atoms adsorbed on a free-standing graphene was investigated using methods beyond the conventional density functional theory (DFT+U, DFT+HIA and DFT+ED). The influence of the electron…

Strongly Correlated Electrons · Physics 2016-09-12 Agnieszka L. Kozub , Alexander B. Shick , Frantisek Maca , Jindrich Kolorenc , Alexander I. Lichtenstein

The known and usable truly nonlocal functionals for exchange-correlation energy of the inhomogeneous electron gas are the ADA (average density approximation) and the WDA (weighted density approximation). ADA, by design, yields the correct…

Materials Science · Physics 2009-10-30 I. I. Mazin , D. J. Singh

We review recent developments in electronic structure calculations that go beyond state-of-the-art methods such as density functional theory (DFT) and dynamical mean field theory (DMFT). Specifically, we discuss the following methods: GW as…

Strongly Correlated Electrons · Physics 2017-07-27 J. M. Tomczak , P. Liu , A. Toschi , G. Kresse , K. Held

To address the impact of electron correlations in the linear and non-linear response regimes of interacting many-electron systems exposed to time-dependent external fields, we study one-dimensional (1D) systems where the interacting problem…

Other Condensed Matter · Physics 2011-08-17 N. Helbig , J. I. Fuks , I. V. Tokatly , H. Appel , E. K. U. Gross , A. Rubio

An overarching question in strongly correlated electron systems is how the landscape of quantum phases emerges from electron correlations. The method of extended dynamical mean field theory (EDMFT) has been developed for clean lattice…

Strongly Correlated Electrons · Physics 2022-10-26 Haoyu Hu , Lei Chen , Qimiao Si

Many of the fascinating and unconventional properties of several transition-metal compounds with partially filled d-shells are due to strong electronic correlations. While local correlations are in principle treated exactly within the frame…

Strongly Correlated Electrons · Physics 2017-07-13 F. Lechermann , A. I. Lichtenstein , M. Potthoff

Electrons on Fermi arcs (FAs), a hallmark of Weyl semimetals, exhibit chiral transport harboring chiral anomaly, negative magnetoresistance, and Majorana zero modes. While FAs were observed in exemplary Weyl semimetal TaAs and Co3Sn2S2, the…

Materials Science · Physics 2025-09-01 Yiran Peng , Rui Liu , Pengyu Zheng , Zhiping Yin

In the density-functional studies of materials with localized electronic states, the local/semilocal exchange-correlation functionals are often either combined with a Hubbard parameter $U$ as in the LDA+$U$ method or mixed with a fraction…

Materials Science · Physics 2014-07-24 Mehmet Aras , Çetin Kılıç

We investigate the construction of approximated exchange-correlation functionals by interpolating locally along the adiabatic connection between the weak- and the strong-coupling regimes, focussing on the effect of using approximate…

Chemical Physics · Physics 2017-04-05 Stefan Vuckovic , Lucas O. Wagner , Andrew M. Teale , Paola Gori-Giorgi

An oversight of several previous local density approximation (LDA) results appears to have led to an incomplete picture of the actual capability of density functional theory (DFT), with emphasis on LDA, to describe and to predict the band…

Materials Science · Physics 2010-12-16 D. Bagayoko , G. L. Zhao , L. Franklin , E. C. Ekuma

ARPES is a priori a technique of choice to measure the Fermi velocities vF in metals. In correlated systems, it is interesting to compare this experimental value to that obtained in band structure calculations, as deviations are usually…

Strongly Correlated Electrons · Physics 2012-11-20 V. Brouet , A. Nicolaou , M. Zacchigna , A. Taleb-Ibrahimi , P. Le Fèvre , F. Bertran

While methods based on density-functional perturbation theory have dramatically improved our understanding of electron-phonon contributions to transport in materials, methods for accurately capturing electron-electron scattering relevant to…

We report a detailed electronic structure calculation for Vanadium (V) using DFT, DFT+$U$, $G_0W_0$, $GW_0$ and DFT+DMFT methods. The calculated values of $W$, $U$ and $J$ by cRPA method are $\sim$1.1, $\sim$3.4 and $\sim$0.52 eV,…

Strongly Correlated Electrons · Physics 2020-01-22 Antik Sihi , Sudhir K. Pandey

An exchange-correlation energy functional beyond the local density approximation, based on the exchange-correlation kernel of the homogeneous electron gas and originally introduced by Kohn and Sham, is considered for electronic structure…

Condensed Matter · Physics 2016-08-31 Maurizia Palummo , Giovanni Onida , Rodolfo Del Sole

We describe an ab initio method for calculating the electronic structure, electronic transport, and forces acting on the atoms, for atomic scale systems connected to semi-infinite electrodes and with an applied voltage bias. Our method is…

Materials Science · Physics 2009-11-07 Mads Brandbyge , Jose-Luis Mozos , Pablo Ordejon , Jeremy Taylor , Kurt Stokbro

Pseudogap physics in strongly correlated systems is essentially scale dependent. We generalize the dynamical mean field theory (DMFT) by including into the DMFT equations dependence on correlation length of pseudogap fluctuations via…

Strongly Correlated Electrons · Physics 2007-05-23 E. Z. Kuchinskii , I. A. Nekrasov , M. V. Sadovskii

Sun et al. [J. Chem. Phys. 144, 191101 (2016)] suggested that common density functional approximations (DFAs) should exhibit large energy errors for excited states as a necessary consequence of orbital nodality. Motivated by…

Computational Physics · Physics 2022-11-09 Sebastian Schwalbe , Kai Trepte , Susi Lehtola

Half-metallicity, low magnetic damping and high curie temperature (TC) are crucial for application in spintronics and full Heusler alloys in this regard exhibit remarkable properties. Herein, we have considered Co2FeAl (CFA) and Fe2CoAl…

Computational Physics · Physics 2018-06-08 Lalrinkima , Gennady M. Mikhailov , D. P. Rai