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Generation of high-order harmonics in gases enabled to probe the attosecond electron dynamics in atoms and molecules with unprecedented resolution. Extending the techniques developed originally for atomic and molecular gases to solid state…

Optics · Physics 2020-02-04 Mrudul M. S. , Nicolas Tancogne-Dejean , Angel Rubio , Gopal Dixit

The problem of harmonics generation in nanotargets is considered at the range of parameters (a nanotarget diameter and a pump laser intensity) when the oscillation amplitude of an electron in a target is much larger than the target width.…

Plasma Physics · Physics 2014-02-11 Philipp Korneev

The stability of graphene nanoribbons in the presence of typical atmospheric molecules is systematically investigated by means of density functional theory. We calculate the edge formation free energy of five different edge configurations…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 M. Vanin , J. Gath , K. S. Thygesen , K. W. Jacobsen

A quantum optical model for the high-order harmonic generation is presented, in which both the exciting field and the high harmonic modes are quantized, while the target material appears via parameters only. As a consequence, the model is…

The structural similarity between hexagonal boron nitride (h-BN) and graphene nanoribbons allows for the formation of heterojunctions with small chain stress. The combination of the insulation nature of the former and the quasi-metallic…

High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

Atomic Physics · Physics 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

We demonstrated nonperturbative high harmonics induced by intense mid-infrared light up to 18th order that well exceed the material bandgap in monolayer transition metal dichalcogenides. The intensities of the even-order high-harmonic…

Mesoscale and Nanoscale Physics · Physics 2019-08-20 Naotaka Yoshikawa , Kohei Nagai , Kento Uchida , Yuhei Takaguchi , Shogo Sasaki , Yasumitsu Miyata , Koichiro Tanaka

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

Optics · Physics 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

We present a high harmonic generation theory which generalizes the strong-field approximation to the resonant case, when the harmonic frequency is close to that of the transition from the ground to an autoionizing state of the generating…

Atomic Physics · Physics 2015-06-16 V. V. Strelkov , M. A. Khokhlova , N. Yu. Shubin

With the high-order harmonic generation (HHG) from plasma sur- faces it is possible to turn a laser pulse into a train of attosecond or even zeptosecond pulses in the backward radiation. These attosecond pulses may have amplitude several…

Plasma Physics · Physics 2016-11-03 Mykyta Cherednychek , Alexander Pukhov

High-harmonic spectroscopy driven by circularly-polarized laser pulses and their counter-rotating second harmonic is a new branch of attosecond science which currently lacks quantitative interpretations. We extend this technique to the…

Atomic Physics · Physics 2019-09-04 Denitsa Baykusheva , Simon Brennecke , Manfred Lein , Hans Jakob Wörner

A method is proposed for arbitrarily engineering the high-order harmonic generation phase achieved by shaping a laser pulse and employing xuv light or x rays for ionization. This renders the production of bandwidth-limited attosecond pulses…

Atomic Physics · Physics 2011-02-25 Markus C. Kohler , Christoph H. Keitel , Karen Z. Hatsagortsyan

We experimentally investigate the generation of above-threshold harmonics completely from argon atoms on an excited state using mid-infrared femtosecond laser pulses. The highly nonlinear dependences of the observed signal on the pulse…

Optics · Physics 2015-10-20 Guihua Li , Hongqiang Xie , Ziting Li , Jingpin Yao , Bin Zeng , Wei Chu , Ya Cheng

The enhancement and control of non-linear phenomena at a nanometer scale has a wide range of applications in science and in industry. Among these phenomena, high-harmonic generation in solids is a recent focus of research to realize next…

We develop the strong-field approximation for high-order harmonic generation in hydrogen molecules, including the vibrational motion and the laser-induced coupling of the lowest two Born-Oppenheimer states in the molecular ion that is…

Atomic Physics · Physics 2009-11-13 C. C. Chirila , M. Lein

High-order harmonics generated by bicircular laser field have helicities which alternate between $+1$ and $-1$. In order to generate circularly polarized high-harmonic pulses, which are important for applications, it is necessary to achieve…

Atomic Physics · Physics 2018-09-26 Dejan B. Milošević

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with…

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