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Selectively exciting target molecules to high vibrational states is inefficient in the liquid phase, which restricts the use of IR pumping to catalyze ground-state chemical reactions. Here, we demonstrate that this inefficiency can…

Chemical Physics · Physics 2022-12-27 Tao E. Li , Abraham Nitzan , Joseph E. Subotnik

Strong coupling between excitons and confined modes of light presents a promising pathway to tunable and enhanced energy transport in organic materials. By forming hybrid light-matter quasiparticles, exciton-polaritons, electronic…

Chemical Physics · Physics 2024-11-01 Niclas Krupp , Gerrit Groenhof , Oriol Vendrell

We show that strong electron-electron interactions in cavity-coupled quantum materials can enable collectively enhanced light-matter interactions with ultrastrong effective coupling strengths. As a paradigmatic example we consider a…

Strongly Correlated Electrons · Physics 2019-09-04 Martin Kiffner , Jonathan Coulthard , Frank Schlawin , Arzhang Ardavan , Dieter Jaksch

The ability to establish coherent communication channels is key for scaling up quantum devices. Here, we engineer interactions between distant polaritons, hybrid spin-photon excitations formed at different lumped-element superconducting…

The ultrafast non-radiative relaxation of a molecular ensemble coupled to a cavity mode is considered theoretically and by real-time quantum dynamics. For equal coupling strength of single molecules to the cavity mode, the non-radiative…

Chemical Physics · Physics 2018-12-26 Oriol Vendrell

We study the scattering problem of photon and polariton in a one-dimensional coupled-cavity system. Analytical approximate analysis and numerical simulation show that a photon can stimulate the photon emission from a polariton through…

Quantum Physics · Physics 2016-02-17 Ci. Li , Zhi. Song

We review the recent developments of the polariton physics in microcavities featuring the exciton-photon strong coupling at room-temperature, and leading to the achievement of room-temperature polariton condensates. Such cavities embed…

Mesoscale and Nanoscale Physics · Physics 2016-09-21 Thierry Guillet , Christelle Brimont

Ionization-excitation of an atom induced by the absorption of a single photon in the presence of a neighbouring atom is studied. The latter is, first, resonantly photoexcited and, afterwards, transfers the excitation energy radiationlessly…

Atomic Physics · Physics 2023-09-06 S. Kim , S. Steinhäuser , A. B. Voitkiv , C. Müller

We show that an exciton on a discrete chain of sites can be guided by effective measurements induced by an ambient, non-equilibrium medium that is synchronised to the exciton transport. For experimental verification, we propose a hybrid…

Quantum Physics · Physics 2024-08-16 K. Mukherjee , S. Wüster

Replacing independent single quantum wells inside a strongly-coupled semiconductor microcavity with double quantum wells produces a special type of polariton. Using asymmetric double quantum wells in devices processed into mesas allows the…

Between mirrors, the density of electromagnetic modes differs from the one in free space. This changes the radiation properties of an atom as well as the light forces acting on an atom. It has profound consequences in the strong-coupling…

Quantum Physics · Physics 2007-10-04 T. Puppe , I. Schuster , P. Maunz , K. Murr , P. W. H. Pinkse , G. Rempe

A model designed to mimic the implications of the collective optical response of molecular ensembles in optical cavities on molecular vibronic dynamics is investigated. Strong molecule-radiation field coupling is often reached when a large…

Chemical Physics · Physics 2022-10-05 Bingyu Cui , Abraham Nitzan

Vacuum-stimulated Raman transitions are driven between two magnetic substates of a rubidium-87 atom strongly coupled to an optical cavity. A magnetic field lifts the degeneracy of these states, and the atom is alternately exposed to laser…

Quantum Physics · Physics 2007-05-23 T. Wilk , S. C. Webster , H. P. Specht , G. Rempe , A. Kuhn

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

In this theoretical work, we study a double quantum dot interacting strongly with a microcavity, while undergoing resonant tunneling. Effects of interdot tunneling on the light-matter hybridized states are determined, and tunability of…

Quantum Physics · Physics 2018-11-08 Marlon S. Domínguez , David F. Macias-Pinilla , Hanz Y. Ramírez

We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. A quantum Langevin analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of…

Quantum Physics · Physics 2023-03-29 Zhedong Zhang , Xiaoyu Nie , Dangyuan Lei , Shaul Mukame

A tapered optical nanofiber simultaneously used to trap and optically interface of cold atoms through evanescent fields constitutes a new and well controllable hybrid quantum system. The atoms are trapped in two parallel 1D optical lattices…

Quantum Physics · Physics 2010-10-25 Hashem Zoubi , Helmut Ritsch

Multi-particle correlations of exciton-polaritons and reservoir-excitons in the strong light-matter coupling regime dictate the quantum dynamics of optical microcavities. In this letter, we examine the many-body exciton-polariton dynamics…

Collective strong coupling between a disordered ensemble of $N$ localized molecular vibrations and a resonant optical cavity mode gives rise to 2 polariton and $N-1\gg2$ dark modes. Thus, experimental changes in thermally-activated reaction…

Quantum Physics · Physics 2022-03-14 Matthew Du , Joel Yuen-Zhou

We investigate a cavity quantum electrodynamic effect, where the alignment of two-dimensional freely rotating optical dipoles is driven by their collective coupling to the cavity field. By exploiting the formal equivalence of a set of…

Quantum Physics · Physics 2017-08-02 Erika Cortese , Pavlos Lagoudakis , Simone De Liberato