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We investigate the transport characteristics of a redox system weakly coupled to leads in the Coulomb blockade regime. The redox system comprises a donor and acceptor separated by an insulating bridge in a solution. It is modeled by a…

Strongly Correlated Electrons · Physics 2010-09-08 Sabine Tornow , Gertrud Zwicknagl

With the progress of nano-technology, thermodynamics also has to be scaled down, calling for specific protocols to extract and measure work. Usually, such protocols involve the action of an external, classical field (the battery) of…

Quantum Physics · Physics 2016-08-09 Cyril Elouard , Maxime Richard , Alexia Auffèves

The methods of Nicholson and Shain and Randles-Sevcik are the paradigms of voltammetry of redox species. However, as they were originally developed for aqueous redox couples, they cannot be directly applied to solid redox films such as…

Chemical Physics · Physics 2025-03-20 Keyvan Malaie

As an alternative approach to ionic data transmission with hydrogel as substrate, this work explores the possible applications of liquid electrolyte filling cavity of a stretchable, flexible elastomeric tubing, which is the primary…

Systems and Control · Electrical Eng. & Systems 2023-07-06 Khoi Ly , Chong-Chan Kim , Robert Shepherd

We investigate both analytically and by numerical simulation the kinetics of a microscopic model of hard rods adsorbing on a linear substrate, a model which is relevant for compaction of granular materials. The computer simulations use an…

Statistical Mechanics · Physics 2009-10-31 J. Talbot , G. Tarjus , P. Viot

The results of molecular dynamics simulations of the properties of water in an aqueous ionic solution close to an interface with a model metallic electrode are described. In the simulations the electrode behaves as an ideally polarizable…

Statistical Mechanics · Physics 2014-09-09 Adam P. Willard , Stewart K. Reed , Paul A. Madden , David Chandler

Electroosmosis is a fascinating effect where liquid motion is induced by an applied electric field. Counter ions accumulate in the vicinity of charged surfaces, triggering a coupling between liquid mass transport and external electric…

Batteries are pivotal components in overcoming some of today's greatest technological challenges. Yet to date there is no self-consistent atomistic description of a complete battery. We take first steps toward modeling of a battery as a…

Materials Science · Physics 2013-08-16 Wolf B. Dapp , Martin H. Müser

We present two recent applications of lattice-gas modeling techniques to electrochemical adsorption on catalytically active metal substrates: urea on Pt(100) and (bi)sulfate on Rh(111). Both involve the specific adsorption of small…

Condensed Matter · Physics 2009-10-22 P. A. Rikvold , M. Gamboa-Aldeco , J. Zhang , M. Han , Q. Wang , H. L. Richards , A. Wieckowski

It has been known for a long time that the adsorption and condensation of gas cause elastic deformation of the porous matrix. The reversible formation of an adsorbed film, which precedes capillary condensation, results in an extension of…

Soft Condensed Matter · Physics 2008-09-04 Annie Grosman , Camille Ortega

Controlling the magnetization reversal process of magnetic elements is important for a wide range of applications that make use of magnetoresistive effects, but is difficult to achieve for devices that require adjacent thin film structures…

Mesoscale and Nanoscale Physics · Physics 2016-11-23 Gavin D. Scott , Ting-Chen Hu

Specific conductance and frequency-dependent resistance (impedance) data are widely utilized for understanding the physicochemical characteristics of aqueous and non-aqueous fluids and for evaluating the performance of chemical processes.…

Absorption of electromagnetic energy by a dissipative material is one of the most fundamental electromagnetic processes that underlies a plethora of applied problems, including sensing and molecular detection, radar detection, wireless…

Optics · Physics 2020-03-31 Alexey Proskurin , Andrey Bogdanov , Denis G. Baranov

Redox flow batteries (RFBs) have gained popularity as large-scale energy storage systems for wind and solar powered grids. Modern RFB systems are based on highly corrosive and/or flammable electrolytes. Organic redox active species for RFBs…

Materials Science · Physics 2021-06-22 Rohan Borah , Fraser R Hughson , Thomas Nann

We propose an equivalent circuit representation of the photogenerated charge separation and propagation in dye sensitized polycrystalline semiconductor in contact with a redox electrolyte. The suggested equivalent circuit for this type of…

Materials Science · Physics 2007-05-23 B. Vainas

Electrochemical impedance spectra for battery electrodes are usually interpreted using models that assume isotropic active particles, having uniform current density and symmetric diffusivities. While this can be reasonable for amorphous or…

Chemical Physics · Physics 2013-09-24 J. Song , M. Z. Bazant

A new global analytical model of the heat dissipation process that occurs in passively-cooled embedded systems is introduced, and we explicit under what circumstances the traditional assumption that exponential cooling laws apply in such…

Other Computer Science · Computer Science 2015-12-17 Karel De Vogeleer , Gerard Memmi , Pierre Jouvelot , Fabien Coelho

Electron transfer at electrode interfaces to molecules in solution or at the electrode surface plays a vital role in numerous technological processes. However, treating these processes requires a unified and accurate treatment of the…

Chemical Physics · Physics 2023-07-19 Kenneth A. Jung , Joseph Kelly , Thomas E. Markland

An analogy between electromagnetism and acoustics is presented in 2D. The propagation of sound in presence of absorbing material is modeled using an open boundary microwave package. Validation is performed through analytical and…

Classical Physics · Physics 2007-05-23 Laurent Nicolas , M. Furstoss , Marie-Annick Galland

A simple molecular thermodynamic approach is applied to the study of the adsorption of gases of chain molecules on solid surfaces. We use a model based on the Statistical Associating Fluid Theory for Variable Range (SAFT-VR) potentials [A.…

Computational Physics · Physics 2010-12-23 M. Castro , R. Martinez , A. Martinez , H. C. Rosu